水电解制氢非贵金属催化剂的研究进展

doi:10.3866/PKU.WHXB201604291

Abstract

Abstract:

Because of its zero-carbon emission energy, hydrogen energy is considered the cleanest energy. The greatest challenge is to develop a cost-effective strategy for hydrogen generation. Water electrolysis driven by renewable resource-derived electricity and direct solar-to-hydrogen conversion are promising pathways for sustainable hydrogen production. All of these techniques require highly active noble metal-free hydrogen and oxygen evolution catalysts to make the water splitting process energy efficient and economical. In this review, we highlight recent research efforts toward synthesis and performance optimization of noble metal-free electrocatalysts in our institute over the last 3 years. We focus on (1) hydrogen evolution catalysts, including transition metal phosphide, sulfides, selenides, and carbides; (2) oxygen evolution catalysts, including transition metal phosphide, sulfide, and oxide/hydroxides; and (3) bifunctional catalysts, mainly comprising transition metal phosphides, selenides, sulfides, and so on. Finally, we summarize the challenges and prospective for future development of non-noble metal catalysts for water electrolysis.

Key words: Water electrolysis, Hydrogen energy, Non-noble catalyst, Hydrogen evolution reaction, Oxygen evolution reaction

MSC2000:

O646

Jin-Fa CHANG,Yao XIAO,Zhao-Yan LUO,Jun-Jie GE,Chang-Peng LIU,Wei XING. Recent Progress of Non-Noble Metal Catalysts in Water Electrolysis for Hydrogen Production[J].Acta Phys. -Chim. Sin., 2016, 32(7): 1556-1592.

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Recent Progress of Non-Noble Metal Catalysts in Water Electrolysis for Hydrogen Production

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