维度调控策略提升铂基纳米晶氧还原催化研究进展

doi:10.3866/PKU.WHXB201708312

Acta Phys. -Chim. Sin. ›› 2018, Vol. 34 ›› Issue (4): 361-376.doi: 10.3866/PKU.WHXB201708312

Special Issue: 高被引科学家特刊

• REVIEW • Previous Articles Next Articles

Boosting Oxygen Reduction Catalysis by Tuning the Dimensionality of Pt-based Nanostructures

Mingchuan LUO¹,Yingjun SUN^1,³,Yingnan Yingjun^1,³,Yong YANG¹,Dong WU⁴,Shaojun GUO^1,^2,*()

¹ Department of Materials Science & Engineering, College of Engineering, Peking University, Beijing 100871, P. R. China
² BIC-ESAT, College of Engineering, Peking University, Beijing 100871, P. R. China
³ College of Chemistry and Molecular Engineering, Qingdao University of Science and Technology, Qingdao 266042, Shandong Province, P. R. China
⁴ Academy for Advanced Interdisciplinary Studies, Peking University, Beijing 100871, P. R. China

Received:2017-06-30 Published:2018-01-02
Contact: Shaojun GUO E-mail:guosj@pku.edu.cn
Supported by:
the National Natural Science Foundation of China(51671003);the China Postdoctoral Science Foundation(2017M610022);the National Basic Research Program of China(2016YFB0100201);the Open Project Foundation of State Key Laboratory of Chemical Resource Engineering, the start-up supports from Peking University;the Young Thousand Talented Program, China

Abstract

Abstract:

The past decade has witnessed tremendous progress in the improvement of the electrocatalytic efficiency of the oxygen reduction reaction (ORR), which is important for the widespread adoption of fuel cells. This review provides an overview of the recent advances in the rational structural design and construction of Pt-based nanocatalysts to achieve higher ORR activity, with an emphasis on tuning the dimensionalities of Pt-based nanocrystals. The advantages and disadvantages of each dimensional catalyst have been discussed. In particular, we focus on a contemporary understanding of the structure-performance relationships based on the combined theoretical and experimental evidence, which can be further applied to guide the search for more exciting catalytic systems. The review concludes with a personal perspective for future research directions.

Key words: Fuel cells, Oxygen reduction reaction, Platinum-based nanocrystals, Dimensionality tuning

MSC2000:

O646

Mingchuan LUO,Yingjun SUN,Yingnan Yingjun,Yong YANG,Dong WU,Shaojun GUO. Boosting Oxygen Reduction Catalysis by Tuning the Dimensionality of Pt-based Nanostructures[J].Acta Phys. -Chim. Sin., 2018, 34(4): 361-376.

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Boosting Oxygen Reduction Catalysis by Tuning the Dimensionality of Pt-based Nanostructures

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