Acta Phys. -Chim. Sin. ›› 2021, Vol. 37 ›› Issue (10): 2001025.doi: 10.3866/PKU.WHXB202001025
• ARTICLE • Previous Articles Next Articles
Ping An1, Yu Fu2, Danlei Wei1, Yanglong Guo2, Wangcheng Zhan2,*(), Jinshui Zhang1,*(
)
Received:
2020-01-07
Published:
2020-02-28
Contact:
Wangcheng Zhan,Jinshui Zhang
E-mail:jinshui.zhang@fzu.edu.cn;zhanwc@ecust.edu.cn
About author:
Emails: zhanwc@ecust.edu.cn (W.Z.); +86-13818212466 (W.Z.)Supported by:
MSC2000:
Ping An, Yu Fu, Danlei Wei, Yanglong Guo, Wangcheng Zhan, Jinshui Zhang. Hollow Nitrogen-Rich Carbon Nanoworms with High Activity for Metal-Free Selective Aerobic Oxidation of Benzyl Alcohol[J].Acta Phys. -Chim. Sin., 2021, 37(10): 2001025.
"
Sample | SBET/(m2?g?1) | Pore volume/(cm3?g?1) | Concentration (%, atomic fraction) | Graphitic N/Pyridinic N | ||||
Total C | Total O | Total N | Graphitic N | Pyridinic N | ||||
h-NCNWs0.5 | 440 | 1.40 | 88.37 | 3.49 | 8.14 | 4.96 | 3.18 | 1.56 |
h-NCNWs1 | 351 | 0.66 | 89.37 | 3.50 | 7.13 | 4.68 | 2.45 | 1.91 |
h-NCNWs1.5 | 459 | 0.59 | 93.52 | 3.72 | 2.76 | 2.02 | 0.74 | 2.73 |
"
Catalyst | Temperature (℃) | Conversion (%) | Selectivity (%) b |
blank | 120 | – | – |
C-RF | 120 | 1.73 | > 99 |
h-NCNWs0.5 | 60 | 3.36 | > 99 |
h-NCNWs0.5 | 80 | 10.1 | > 99 |
h-NCNWs0.5 | 100 | 18.7 | > 99 |
h-NCNWs0.5 | 120 | 24.9 | > 99 |
h-NCNWs1 | 120 | 20.2 | > 99 |
h-NCNWs1.5 | 120 | 13.1 | > 99 |
h-NCNWs0.5 c | 120 | 8.32 | > 99 |
h-NCNWs0.5 d | 120 | 8.83 | > 99 |
h-NCNWs0.5 e | 120 | 9.01 | > 99 |
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