铈基催化剂用于NH3选择性催化还原NOx的研究进展

doi:10.3866/PKU.WHXB201503253

Abstract

Abstract:

Nitrogen oxides (NO_x), which are emitted from stationary sources (such as coal-fired power plant flue gases) and mobile sources (such as motor vehicle exhausts), cause serious atmospheric pollution. As a result, it is very important to control the emissions of NO_x. Some studies have suggested that NH₃-selective catalytic reduction (NH₃-SCR) of NO_x is one of the best techniques for this purpose. Ceria-based catalysts are widely used in the NH₃-SCR reaction because of their good redox ability, suitable surface acidity, high oxygen storage or release capacity, and rich resource reserves. Investigating the role of ceria component in this reaction is important to understand the nature of the related catalytic process, and provides a valuable scientific reference for the optimization of existing catalysts and the design of novel catalysts. Based on the different roles of ceria in NH₃-SCR catalysts, we have performed a systematic review of the latest research progress of ceria-based catalysts in the NH₃-SCR reaction for the following aspects: CeO₂ used as supports, ceria-based mixed oxides, surface loading components (additives and active species), and ceria-based catalysts with special structures. Finally, we discuss the future directions of this field.

Key words: Ceria-based catalyst, Nitrogen oxide, Selective catalytic reduction by NH₃, Support, Mixed oxide, Surface loading component, Special structure

MSC2000:

O643

YAO Xiao-Jiang, GONG Ying-Tao, LI Hong-Li, YANG Fu-Mo. Research Progress of Ceria-Based Catalysts in the Selective Catalytic Reduction of NO_x by NH₃[J].Acta Phys. -Chim. Sin., 2015, 31(5): 817-828.

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Research Progress of Ceria-Based Catalysts in the Selective Catalytic Reduction of NO_x by NH₃

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Research Progress of Ceria-Based Catalysts in the Selective Catalytic Reduction of NOx by NH3

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Research Progress of Ceria-Based Catalysts in the Selective Catalytic Reduction of NO_x by NH₃