Article
Photocatalytic Properties of Composite of SiO2 and Pt-Cd0.53Zn0.47S Solid Solutions
HU Yuan-Fang; LI Yue-Xiang; PENG Shao-Qin; LV Gong-Xuan; LI Shu-Ben
Department of Chemistry, Nanchang University, Nanchang 330031, P. R. China; State Key Laboratory for Oxo Synthesis and Selective Oxidation, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, P. R. China
Department of Chemistry, Nanchang University, Nanchang 330031, P. R. China; State Key Laboratory for Oxo Synthesis and Selective Oxidation, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, P. R. China
Cd0.53Zn0.47S was prepared by a coprecipitation method. Pt was loaded onto Cd0.53Zn0.47S by photodeposition method. SiO2 was deposited onto Cd0.53Zn0.47S by hydrolysis of the tetraethylorthosilicate (TEOS), and the effect of the hydrolysis pH on the activity of the catalysts was studied. The samples were characterized by X-ray diffraction (XRD), BET surface area, photoluminescence (PL), UV-Vis diffusive reflectance spectroscopy (UV-Vis DRS), and scanning electron microscope (SEM) techniques. The composite SiO2 prevented effectively photocorrosion and coalescence of Pt-Cd0.53Zn0.47S nanoparticles during the photocatalytic reaction, and improved the charge separation of photogenerated electrons and holes. Therefore, the stability and the activity of Pt-Cd0.53Zn0.47S for photocatalytic hydrogen generation
under visible light irradiation were improved greatly.
Keywords: Photocatalyst SiO2/Pt-Cd0.53Zn0.47S Hydrogen production Solid solution
Received: 2008-05-04 Accepted: 2008-07-01 Publication Date (Web): 2008-09-26
Corresponding Authors: LI Yue-Xiang Email: liyx@ncu.edu.cn
Cite this article: HU Yuan-Fang; LI Yue-Xiang; PENG Shao-Qin; LV Gong-Xuan; LI Shu-Ben. Photocatalytic Properties of Composite of SiO2 and Pt-Cd0.53Zn0.47S Solid Solutions[J]. Acta Phys. -Chim. Sin., 2008,24 (11): 2071-2076. doi: 10.3866/PKU.WHXB20081123
under visible light irradiation were improved greatly.
Keywords: Photocatalyst SiO2/Pt-Cd0.53Zn0.47S Hydrogen production Solid solution
Received: 2008-05-04 Accepted: 2008-07-01 Publication Date (Web): 2008-09-26
Corresponding Authors: LI Yue-Xiang Email: liyx@ncu.edu.cn
Cite this article: HU Yuan-Fang; LI Yue-Xiang; PENG Shao-Qin; LV Gong-Xuan; LI Shu-Ben. Photocatalytic Properties of Composite of SiO2 and Pt-Cd0.53Zn0.47S Solid Solutions[J]. Acta Phys. -Chim. Sin., 2008,24 (11): 2071-2076. doi: 10.3866/PKU.WHXB20081123
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15． ZHOU He-Gen, WEN Xing-Wei, FANG Zhen-Xing, Li Yi, DING Kai-Ning, HUANG Xin, ZHANG Yong-Fan.Electronic Structures and Optical Properties of AgGa(S1-xSex)2 Solid Solutions[J]. Acta Phys. -Chim. Sin., 2013,29(05): 920-928
16． ZHAO Jian, ZHOU Wei, XU Jun-Ke, MA Jian-Xin.Effect of Pretreatment Routes on the Performance and Structure of Ni-Co Bimetallic Catalysts[J]. Acta Phys. -Chim. Sin., 2013,29(04): 806-812
17． YUAN Wen-Hui, LIU Xiao-Chen, LI Li.Improving Photocatalytic Performance for Hydrogen Generation over Co-Doped ZnIn2S4 under Visible Light[J]. Acta Phys. -Chim. Sin., 2013,29(01): 151-156
18． TAO Jing-Liang, XIONG Yuan-Quan.Hydrogen Production from the Decomposition of Ethanol Aqueous Solution Using Glow Discharge Plasma Electrolysis[J]. Acta Phys. -Chim. Sin., 2013,29(01): 205-211
19． ZHENG Hua-Rong, ZHANG Jin-Shui, WANG Xin-Chen, FU Xian-Zhi.Modification of Carbon Nitride Photocatalysts by Copolymerization with Diaminomaleonitrile[J]. Acta Phys. -Chim. Sin., 2012,28(10): 2336-2342
20． CAO Hong-Yan, WANG Jian-Li, YAN Sheng-Hui, LIU Zhi-Min, GONG Mao-Chu, CHEN Yao-Qiang.Effect of Doping M (M = Mn, Y) into Ce0.50Zr0.50O2 on the Properties of MnOx/Ce0.50-zZr0.50-zM2zOy/Al2O3 for Catalytic Combustion of Ethyl Acetate[J]. Acta Phys. -Chim. Sin., 2012,28(08): 1936-1942
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22． XIONG Li-Long, XU You-Long, ZHANG Cheng, TAO Tao.Doping-Coating Surface Modification of Spinel LiMn2O4 Cathode Material with Al3+ for Lithium-Ion Batteries[J]. Acta Phys. -Chim. Sin., 2012,28(05): 1177-1182
23． WANG Zhao, WU Feng, SU Yue-Feng, BAO Li-Ying, CHEN Lai, LI Ning, CHEN Shi.Preparation and Characterization of xLi2MnO3·(1-x)Li[Ni1/3Mn1/3Co1/3]O2 Cathode Materials for Lithium-Ion Batteries[J]. Acta Phys. -Chim. Sin., 2012,28(04): 823-830
24． JIANG Li-Long, MA Yong-De, CAO Yan-Ning, YANG Yang, WEI Ke-Mei.Modified Bauxite Supported Ruthenium Catalysts for Hydrogen Evolution in the Water-Gas Shift Reaction[J]. Acta Phys. -Chim. Sin., 2012,28(03): 674-680
25． CHEN Xiao-Yun, LU Dong-Fang, HUANG Jin-Feng, LU Yan-Feng, ZHENG Jian-Qiang.Preparation and Properties of N-F Co-Doped TiO2 Photocatalyst with Wide Range Light Response and Multipore Structure from Ionic Liquid-Water Mixture Solvent[J]. Acta Phys. -Chim. Sin., 2012,28(01): 161-169
26． LI Ben-Xia, WANG Yan-Fen, LIU Tong-Xuan.Adjustable Synthesis and Visible-Light Responsive Photocatalytic Performance of V2O5·xH2O-BiVO4 Nanocomposites[J]. Acta Phys. -Chim. Sin., 2011,27(12): 2946-2952
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