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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2008,Vol.24>> Issue(09)>> 1714-1718     doi: 10.3866/PKU.WHXB20080933         中文摘要
Effects of Benzene and 1-Octene on Desulfurization by Selective Adsorption with Ce(IV)Y
WANG Hong-Guo; JIANG Heng; XU Jing; SUN Zhao-Lin; ZHANG Xiao-Tong; ZHU He-Li; SONG Li-Juan
College of Chemistry & Chemical Engineering, China University of Petroleum (East China), Dongying 257061, Shandong Province, P. R. China; Liaoning Key Laboratory of Petrochemical Engineering, Liaoning Shihua University, Fushun 113001, Liaoning Province, P. R. China
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Selective adsorptive desulfurization of model gasolines containing different amounts of aromatics and olefin compounds, such as benzene and 1-octene, on Ce(IV)Y zeolite was studied using a fixed-bed adsorption column, Fourier transform-infrared spectroscopy (FT-IR), and ultraviolet diffuse reflection spectroscopy (UV-DRS) techniques. It was found that both benzene and 1-octene had strong inhibiting effects on the desulfurization which could be detected by the decreases in the desulfurization capacities of the Ce(IV)Yin the presence of benzene and 1-octene in the model gasoline. The FT-IR and UV-DRS spectra of the Ce(IV)Y zeolites adsorbing the model gasolines revealed that benzene was desorbed easily because of the formation of π-complexes, while 1-octene was desorbed difficultly due to the strong interactions between the double-bond of 1-octene and the Ce4+ to form the π-complexes through the σ-π electron donations. Therefore, it could be concluded that the effect of benzene on the adsorptive removal of sulfur compounds could be ascribed to the competitive adsorption on the Ce(IV)Ybetween the aromatics and the organosulfur compounds in the fuels. While for the effect of 1-octene, the Ce(IV)Y zeolites adsorbed preferentially the 1-octene molecules onto adsorption sites, resulting in descending adsorptive selectivity for removing thiophene from the model fuel containing even minor amount of olefin.

Keywords: Zeolite   Selective adsorption   Desulfurization mechanism   FT-IR   UV-DRS  
Received: 2008-04-18 Accepted: 2008-05-23 Publication Date (Web): 2008-07-04
Corresponding Authors: SONG Li-Juan Email: lsong@lnpu.edu.cn


Cite this article: WANG Hong-Guo; JIANG Heng; XU Jing; SUN Zhao-Lin; ZHANG Xiao-Tong; ZHU He-Li; SONG Li-Juan. Effects of Benzene and 1-Octene on Desulfurization by Selective Adsorption with Ce(IV)Y[J]. Acta Phys. -Chim. Sin., 2008,24 (09): 1714-1718.    doi: 10.3866/PKU.WHXB20080933
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91. Dai Zhi-Hui;Ju Huang-Xian.Direct Electron Transfer of Protein Immobilized on Mesoporous Molecular Sieves Matrix[J]. Acta Phys. -Chim. Sin., 2004,20(10): 1262-1266
92. Ma Zhong-Yi;Xu Run;Yang Cheng;Wei Wei;Li Wen-Huai;Sun Yu-Han.Preparation and Surface Properties of Different Zirconia Polymorphs[J]. Acta Phys. -Chim. Sin., 2004,20(10): 1221-1225
93. Wang Fan;Yang Zhan-Lan;Zhang Li;Weng Shi-Fu;Wu Jin-Guang.FT-IR Study of the Interaction between Phosphatidylcholine and Bovine Serum Albumin[J]. Acta Phys. -Chim. Sin., 2004,20(10): 1186-1190
94. Lian Wen-Hao;Zheng Ying;Wang Xu-Xu;Fu Xian-Zhi.Preparation and Property of a MCM-41 Surface Neopentyl-titanium and Surface Titanium Oxides[J]. Acta Phys. -Chim. Sin., 2004,20(09): 1138-1143
95. Zhu Jian-Hua;Xu Yang;Wang Ying;Zhou Shi-Lu;Zhou Chun-Fang.Adsorption and Catalytic Degradation of Nitrosamines by Zeolites and Molecular Sieves[J]. Acta Phys. -Chim. Sin., 2004,20(08S): 946-952
96. Chen Hong-Lin;Shen Bao-Jian;Pan Hui-Fang.Physicochemical and Catalytic Properties of ZSM-5/Y Composite Zeolites Dealuminated by the Steaming[J]. Acta Phys. -Chim. Sin., 2004,20(08): 854-859
97. Liu Jie-Xiang;Dong Mei;Qin Zhang-Feng;Wang Jian-Guo.Molecular Simulation of Dichlorobenzene Sorption in AlPO4-5Molecular Sieves[J]. Acta Phys. -Chim. Sin., 2004,20(07): 696-700
98. Shi Xi-E;Zhai Shang-Ru;Dai Li-Yi;Shan Yong-Kui;He Ming-Yuan;Wei Wei;Wu Dong;Sun Yu-Han.Synthesis of Mesoporous Aluminosilicate Nanoparticles and Its Performance in Catalytic Cracking[J]. Acta Phys. -Chim. Sin., 2004,20(03): 265-270
99. Nie Chun-Fa;Suo Ji-Shuan.Synthesis,Characterization and Catalytic Applications of Asymmetric Hydrogenation Catalyst Immobilized on Hybrid MCM-41[J]. Acta Phys. -Chim. Sin., 2004,20(02): 149-153
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101. Zheng Jun-Lin;Zhang Ye;Wei Wei; Wu Dong;Sun Yu-Han;Deng Feng;Luo Qing;Yue Yong.Hydrothermally Stable Mesoporous Aluminosilicates with Strongly Acidic Sites[J]. Acta Phys. -Chim. Sin., 2003,19(10): 907-912
102. Cheng Zhi-Lin;Chao Zi-Sheng;Wan Hui-Lin.Nanosized NaY Zeolite Synthesized Rapidly by Microwave Induction[J]. Acta Phys. -Chim. Sin., 2003,19(06): 487-491
103. Zhu Jian-Hua;Xu Yang;Zhou Chun-Fang;Zhou Shi-Lu;Ma Li-Li.Investigation on the Insertion-adsorption of N-nitrosamines on the Zeolite with Small Pore[J]. Acta Phys. -Chim. Sin., 2003,19(03): 221-225
104. Wang Zhe-Ming;Yan Zi-Feng.Skeletal Isomerization of Butene on Si, Zr-substituted Aluminum Phosphate Zeolites[J]. Acta Phys. -Chim. Sin., 2003,19(03): 216-220
105. Zhai Shang-Ru;Pu Min;Zhang Ye;Wu Dong;Sun Yu-Han.High-Yield Synthesis of MCM-48 Using Mixed Surfactants and Adjusting pH Route[J]. Acta Phys. -Chim. Sin., 2003,19(02): 167-170
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107. Song Chun-Min;Yan Zi-Feng;Max Lu.Synthesis and Characterization of Supersurface MCM-41 Zeolites[J]. Acta Phys. -Chim. Sin., 2002,18(03): 279-283
108. Yao Yun-Feng;Zhang Mai-Sheng;Yang Yan-Sheng.Synthesis of Nano-sized MCM-41 Mesoporous Molecular Sieve by[J]. Acta Phys. -Chim. Sin., 2001,17(12): 1117-1121
109. Liu Zhen-Lin;Meng Ming;Fu Yi-Lu;Jiang Ming;Hu Tian-Dou;Xie Ya-Ning;Liu Tao.Structure Characterization of γ-Mo2N and Mo Nitrides Supported on Zeolites[J]. Acta Phys. -Chim. Sin., 2001,17(07): 631-635
110. Liu Xin-Mei;Yan Zi-Feng;Wang Huai-Ping.Optimization of Zeolite for Producing Lighter Olefin and Diesel in FCC Process[J]. Acta Phys. -Chim. Sin., 2001,17(06): 547-551
111. Xin Jing;Suo Ji-Shuan;Zhang Xiao-Ming;Ren Tong;Yan Liang;Zhang Han-Peng.Novel Templating Route to Mesoporous Silica Molecular Sieves[J]. Acta Phys. -Chim. Sin., 2001,17(03): 193-195
112. Lu An-Hui;Li Wen-Cui;Zheng Jing-Tang.Preparation of PANbased Molecular Sieve ACF and Study of Surface Structure by XPS[J]. Acta Phys. -Chim. Sin., 2001,17(03): 216-221
113. Wang Xu-Xu;Fu Xian-Zhi.Reaction of Surface Hydroxyl Group of MCM41 with Tetraneopentylzirconium[J]. Acta Phys. -Chim. Sin., 2001,17(02): 165-168
114. Gong Yan-Jun;Li Zhi-Hong;Wu Dong;Sun Yu-Han.Interface Characteristics of Organo-MSU-x Silica[J]. Acta Phys. -Chim. Sin., 2001,17(01): 1-4
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117. Zeng Hong-Xia, Li Zhi-Ping, Wang Han-Qing.Physical Chemistry Property of Water/TX-100/Hexanol/Octane Reverse Microemulsion[J]. Acta Phys. -Chim. Sin., 1999,15(06): 522-527
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119. Qiu Shi-Lun, Zhai Qing-Zhou, Xiao Feng-Shou, Zhang Zong-Tao, Han Yu.The Developments of the Studies of New Type Zeolite Molecular Sieve Host-nanoguest Composite Materials[J]. Acta Phys. -Chim. Sin., 1998,14(12): 1116-1122
120. Zhao Qi, Han Xiu-Wen, Liu Xiu-Mei, Zhai Run-Sheng, Lin Li-Wu, Bao Xin-He, Guo Xin-Wen, Li Gang, Wang Xiang-Sheng.Studies on the TS-1 Zeolites Synthesized by Tetrapropylammonium Bromide as Template[J]. Acta Phys. -Chim. Sin., 1998,14(10): 906-912
121. Yang Peng-Cheng, Ye Xue-Qi, Ji Ming-Juan, Zhao Zhu-Liu, Zhang Zhuo-Ya, Hou Ting-Jun, Xu Xiao-Jie.The Study of Non-framework Cation Position in Zeolite Model[J]. Acta Phys. -Chim. Sin., 1998,14(09): 817-820
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123. Yin Dong-Hong, Yin Du-Lin.Study on the Solid-state Reaction of ZnCl2 and Y Zeolites under Microwave lrradiation[J]. Acta Phys. -Chim. Sin., 1998,14(05): 448-452
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