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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2007,Vol.23>> Issue(07)>> 1032-1036     doi: 10.3866/PKU.WHXB20070713         中文摘要
Structural Characterization of Nanocrystalline TiO2 fromIonic Liquid-Water Solvent Mixture and Its Photocatalytic Activity
YAN Zhi-Ying; WU Li-Yan; SUN Gui-Xiang; ZHANG Ning; ZHENG Wen-Jun
Department of Materials Chemistry, College of Chemistry, Nankai University, Tianjin 300071, P. R. China; Department of Applied Chemistry, Yunnan University, Kunming 650091, P. R. China
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Nanocrystalline TiO2 was synthesized by the low-temperature hydrothermal method using ionic liquid (1-ethyl-3-methyl-imidazole acetate)-water mixture as solvent; various studies such as X-ray diffraction, Brunauer-Emmett-Teller surface area, X-ray photoelectron spectra, UV-Vis spectroscopy were conducted. The products prepared from ionic liquid-water mixture possessed good anatase crystallinity and contained less brookite phase than that from pure water. The photocatalytic degradation of methyl orange in water was studied in photoreactor with UV lamp as light source. The product prepared from ionic liquid-water solvent for 24 h showed superior photocatalytic activity for the degradation of methyl orange compared to commercial TiO2, Degussa P25. The higher photocatalytic activity was attributed to the crystal phase, grain size, and specific surface area of the catalyst. Further, the effects of the catalyst amount and pH value of solution on the photocatalytic activity of the product were also investigated.



Keywords: TiO2   Ionic liquid   Low-temperature hydrothermal   Methyl orange   Photocatalytic activity  
Received: 2007-01-09 Accepted: 2007-03-13 Publication Date (Web): 2007-05-22
Corresponding Authors: ZHENG Wen-Jun Email: zhwj@nankai.edu.cn


Cite this article: YAN Zhi-Ying; WU Li-Yan; SUN Gui-Xiang; ZHANG Ning; ZHENG Wen-Jun. Structural Characterization of Nanocrystalline TiO2 fromIonic Liquid-Water Solvent Mixture and Its Photocatalytic Activity[J]. Acta Phys. -Chim. Sin., 2007,23 (07): 1032-1036.    doi: 10.3866/PKU.WHXB20070713
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92. LIU Yu-Sheng, FU Hai-Ying, TANG Zhong-Feng, HUANG Wei, WU Guo-Zhong.Melting Point and Structure of Ionic Liquid [EMIM][PF6] on the Surface of Nano-SiOx Particles[J]. Acta Phys. -Chim. Sin., 2011,27(07): 1725-1729
93. CONG Ye, QIN Yun, LI Xuan-Ke, DONG Zhi-Jun, YUAN Guan-Ming, CUI Zheng-Wei.Preparation and Visible Light Photocatalytic Activity of Titanium Dioxide Coated Multiwalled Carbon Nanotubes[J]. Acta Phys. -Chim. Sin., 2011,27(06): 1509-1515
94. LONG Jin-Xing, GUO Bin, LI Xue-Hui, WANG Fu-Rong, WANG Le-Fu.Catalytic Decomposition of Cellulose in Cooperative Ionic Liquids[J]. Acta Phys. -Chim. Sin., 2011,27(05): 995-999
95. LI Huan-Huan, CHEN Run-Feng, MA Cong, ZHANG Sheng-Lan, AN Zhong-Fu, HUANG Wei.Titanium Oxide Nanotubes Prepared by Anodic Oxidation and Their Application in Solar Cells[J]. Acta Phys. -Chim. Sin., 2011,27(05): 1017-1025
96. JIANG Jing-Jing, LONG Ming-Ce, WU De-Yong, CAI Wei-Min.Preparation of F-Modified Nanosized TiO2 and Its Methyl Orange Photodegradation Mechanism[J]. Acta Phys. -Chim. Sin., 2011,27(05): 1149-1156
97. CHEN Jin-Yi, LI Nian, LI Jing, ZHU Liang, PENG Chang-Jun.Synthesis and Visible Light Photocatalytic Activity of Cross-Linked Sodium Rectorite/Cu2O Nanocomposites[J]. Acta Phys. -Chim. Sin., 2011,27(04): 932-938
98. ZHU Guang-Lai, WU Guo-Zhong, CUI Zhi-Feng, XU Xin-Sheng.Transient Absorption Spectroscopy of the Effects of the Ionic Liquid [bmim][BF4] on the Photochemical Reactions of Benzil[J]. Acta Phys. -Chim. Sin., 2011,27(04): 971-976
99. ZHANG Qi-Bo, HUA Yi-Xin.Effect of Alkylimidazolium Ionic Liquids on the Corrosion Inhibition of Copper in Sulfuric Acid Solution[J]. Acta Phys. -Chim. Sin., 2011,27(03): 655-663
100. LAO Chun-Feng, CHU Zeng-Ze, ZOU De-Chun.Self-Assembly of 3-Aminopropyltrimethoxysilane to Improve the Efficiency of Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2011,27(02): 419-424
101. LIU Jia, YANG Hao-Tian, ZHANG Jing-Bo, ZHOU Xiao-Wen, LIN Yuan.Room Temperature Synthesis of Rutile TiO2 and Its Application in Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2011,27(02): 408-412
102. CUI Wen-Yu, AN Mao-Zhong, YANG Pei-Xia, ZHANG Jin-Qiu.Cathodic and Thermal Stabilities of the P(VdF-HFP)-Based Ionic Liquid Composite Polymer Electrolyte[J]. Acta Phys. -Chim. Sin., 2011,27(01): 78-84
103. ZHANG Qi-Bo, HUA Yi-Xin.Effect of the Ionic Liquid Additive-[BMIM]HSO4 on the Kinetics of Oxygen Evolution during Zinc Electrowinning[J]. Acta Phys. -Chim. Sin., 2011,27(01): 149-155
104. WU Tao, TAO Jie, DENG Jie, TANG Yu-Xin, ZHU Hong, GAO Peng.Preparation and Characterization of One-Dimensional TiO2 Nanowire Films on a Flexible Stainless Steel Substrate[J]. Acta Phys. -Chim. Sin., 2010,26(11): 3087-3094
105. ZHANG Li-Qun, LI Hao-Ran.Progress of Investigations on Structures and Interactions of Ionic Liquids by Infrared Spectroscopy and Raman Spectroscopy[J]. Acta Phys. -Chim. Sin., 2010,26(11): 2877-2889
106. ZHANG Xiao-Ru, LIN Yan-Hong, ZHANG Jian-Fu, HE Dong-Qing, WANG De-Jun.Photoinduced Charge Carrier Properties and Photocatalytic Activity of N-Doped TiO2 Nanocatalysts[J]. Acta Phys. -Chim. Sin., 2010,26(10): 2733-2738
107. QIAN Di-Feng, ZHANG Qing-Hong, WAN Jun, LI Yao-Gang, WANG Hong-Zhi.Enhancing the Photovoltaic Performance of Dye Sensitized Solar Cells with the TiO2 Sol Infiltrated Nanocrystalline Electrode[J]. Acta Phys. -Chim. Sin., 2010,26(10): 2745-2751
108. PAN Shan-Fei, HU Gui-Xiang, LV Yang, ZOU Jian-Wei, YU Qing-Sen.QSPRModel Analysis on the Solubility of Organic Compounds in Ionic Liquids[J]. Acta Phys. -Chim. Sin., 2010,26(09): 2494-2502
109. LIU Yu-Liang, YOU Cui-Rong, LI Yang, HE Tao, ZHANG Xiang-Qin, SUO Zhang-Huai.Preparation of Au@TiO2 Catalyst Using Escherichia Coil as the Template and Its Oxidation Reaction Activity toward CO[J]. Acta Phys. -Chim. Sin., 2010,26(09): 2455-2460
110. SONG Hua,GUO Yun-Tao, LI Feng ,YU Hong-Kun.Preparation, Hydrodesulfurization and Hydrodenitrogenation Performance of a Ni2P/TiO2-Al2O3 Catalyst[J]. Acta Phys. -Chim. Sin., 2010,26(09): 2461-2467
111. XU Ping-Chang, LIU Yang, WEI Jian-Hong, XIONG Rui, PAN Chun-Xu, SHI Jing.Solvothermal Preparation of Ag/TiO2 Nanoparticles and Their Photocatalytic Activity[J]. Acta Phys. -Chim. Sin., 2010,26(08): 2261-2266
112. CAO Hai, JIANG Jian, ZHU Xue-Feng, DUAN Peng-Fei, LIU Ming-Hua.Interfacial Assembly of Diethyl Ester Glutamic Acid Terminated Bolaamphiphile at the Air/Water Interface: Chiral Interaction and Morphology[J]. Acta Phys. -Chim. Sin., 2010,26(07): 1842-1846
113. LIU Qing-Shan, YANG Miao, TAN Zhi-Cheng, WELZ-BIERMANN Urs.Estimation and Prediction of the Physicochemical Properties of Imidazolium-Based Ionic Liquids[J]. Acta Phys. -Chim. Sin., 2010,26(06): 1463-1467
114. LIANG Rui, YANG Mei-Rong, ZHOU Qing-Xiang.Thermal Stability, Equilibrium Vapor Pressure and Standard Enthalpy of Vaporization of 1-Butyl-3-methylimidazolium Tetrafluoroborate[J]. Acta Phys. -Chim. Sin., 2010,26(06): 1468-1472
115. ZHAO Di, HUANG Qing, JIN Xian-Bo, WEI Xian-Jun, CHEN George Z..Capacitance at the Electrode/Ionic Liquid Interface[J]. Acta Phys. -Chim. Sin., 2010,26(05): 1239-1248
116. LI Li, LU Dan, JI Yuan, ZHAO Yue-Hong.Preparation of Nanocomposite Ag/TiO2-ZrO2 and the Microwave Enhanced Photocatalytic Degradation of Methyl Orange[J]. Acta Phys. -Chim. Sin., 2010,26(05): 1323-1329
117. LI Xue-Liang, CHEN Jie-Jie, LUO Mei, CHEN Xiang-Ying, LI Pei-Pei.Quantum Chemical Calculation of Hydroxyalkyl Ammonium Functionalized Ionic Liquids for Absorbing SO2[J]. Acta Phys. -Chim. Sin., 2010,26(05): 1364-1372
118. CUI Wen-Yu, AN Mao-Zhong, YANG Pei-Xia.Preparation of an Ionic Liquid Gel Polymer Electrolyte and Its Compatibility with a LiFePO4 Cathode[J]. Acta Phys. -Chim. Sin., 2010,26(05): 1233-1238
119. WANG Wei, LV Rong, YU An-Chi.Low Frequency Spectrumof Ionic Liquid [bmim][PF6] Studied by Femtosecond Optically Heterodyne-Detected Optical Kerr Effect Spectroscopy and Low Frequency Raman Spectroscopy[J]. Acta Phys. -Chim. Sin., 2010,26(04): 964-970
120. YUAN Li-Yong, PENG Jing, LI Jiu-Qiang, ZHAI Mao-Lin.Radiation-Induced Changes of Phase Behavior and Fluorescence Properties of the Ionic Liquids [C4mim][PF6] and [C4mim][NTf2][J]. Acta Phys. -Chim. Sin., 2010,26(04): 981-987
121. YUAN Xiao, LOU Shu-Jie, KOU Yuan.Ionic Liquid and Water: Making Nanoparticle Catalysis More Efficient and Greener[J]. Acta Phys. -Chim. Sin., 2010,26(04): 908-914
122. ZHANG Qiong, HE Yun-Qiu, CHEN Xiao-Gang, HU Dong-Hu, LI Lin-Jiang, YIN Ting, JI Ling-Li.Intercalated Structure and Photocatalytic Properties of TiO2-Graphite Oxide Composite[J]. Acta Phys. -Chim. Sin., 2010,26(03): 654-662
123. WANG Meng-Ye, WANG Cheng-Lin, XIE Kun-Peng, SUN Lan, LIN Chang-Jian.Fabrication of a Spongelike Nanostructured TiO2 Filmand Its Photocatalytic Activity[J]. Acta Phys. -Chim. Sin., 2009,25(12): 2475-2480
124. WANG Wei-Bin, YIN Jian-Zhong, SUN Li-Hua, FENG En-Min.Molecular Dynamics Simulation of Thermodynamic Properties for CO2/Ionic Liquid Systems[J]. Acta Phys. -Chim. Sin., 2009,25(11): 2291-2295
125. ZHANG Xiao-Yan, CUI Xiao-Li.Preparation and Photocatalytic Hydrogen Evolution Performance of C-N Co-doped Nano TiO2 Photocatalysts[J]. Acta Phys. -Chim. Sin., 2009,25(09): 1829-1834
126. DONG Xiang, TAO Jie, LI Ying-Ying, WANG Tao, ZHU Hong.Photoelectrochemical Properties of Three-Dimensional Network TiO2 Nanowire Film Prepared by Hydrothermal Method[J]. Acta Phys. -Chim. Sin., 2009,25(09): 1874-1882
127. DU Wei-Ping, LI Zhen, LENG Wen-Hua, XU Yi-Ming.Photocatalytic Reduction of Silver Ions on Ferric Oxides and Ferric Hydroxides[J]. Acta Phys. -Chim. Sin., 2009,25(08): 1530-1534
128. LI Chang-Yu, LIU Shou-Xin, MA Yue.Preparation of Visible-Light Response Cu-Cu2+1O Composites by a One-Step Hydrothermal Method[J]. Acta Phys. -Chim. Sin., 2009,25(08): 1555-1560
129. WU Yang, ZHANG Tian-Tian, YU Ning.Interaction between 1-Ethyl-3-Methyl-Imidazolium Cation and Asparagine Anion[J]. Acta Phys. -Chim. Sin., 2009,25(08): 1689-1696
130. FENG Li-Li, ZHAO Wei, LIU Yang, JIAO Liang, LI Xing-Guo.Photocatalytic Degradation of Rhodamine B by Nanocrystalline TiO2 Loaded into MCM-41 Molecular Sieves[J]. Acta Phys. -Chim. Sin., 2009,25(07): 1347-1351
131. LEI Jian-Fei, LI Wei-Shan.Photoelectrocatalytic Performance of Arrayed Porous TiO2/Ti[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1173-1178
132. CAO Yong-Qiang, LONG Hui-Jin, CHEN Yong-Mei, CAO Ya-An.Photocatalytic Activity of TiO2 Films with Rutile/Anatase Mixed Crystal Structures[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1088-1092
133. ZHAI Cui-Ping, LIU Xue-Jun, ZHAO Yang, WANG Jian-Ji.NMR Study on the Aggregation of [C4mim][BF4] in D2O and CDCl3[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1185-1189
134. YU Zhi-Yong; ZHANG Wei; MA Ming; CUI Xiao-Li.Visible Light Photoelectrochemical Response of Nitrogen-Doped TiO2 Thin Films Prepared by Anodic Oxidation of Titanium Nitride Films[J]. Acta Phys. -Chim. Sin., 2009,25(01): 35-40
135. YAN Chao-Qun, WAN Hui, GUAN Guo-Feng.Prediction of Melting Points for 1,3-Disubstituent Imidazolium Ionic Liquids[J]. Acta Phys. -Chim. Sin., 2008,24(12): 2198-2202
136. WANG Xiao-Lu; WAN Hui; GUAN Guo-Feng.Structure and Interaction of Ion-Pairs of [EPy]Cl and [EPy]Br in Gas and Liquid Phases[J]. Acta Phys. -Chim. Sin., 2008,24(11): 2077-2082
137. YANG Pei-Xia; AN Mao-Zhong; SU Cai-Na; WANG Fu-Ping.Electrodeposition Behaviors of Pure Cobalt in Ionic Liquid[J]. Acta Phys. -Chim. Sin., 2008,24(11): 2032-2036
138. ZHENG Yong-Jun; ELI Wumanjiang.Phase Behavior of Tween80/BmimPF6/Alcohol/Toluene Systems[J]. Acta Phys. -Chim. Sin., 2008,24(11): 2143-2148
139. CHANG Guo-Qing, ZHENG Xi, CHEN Ri-Yao, CHEN Xiao, CHEN Li-Qin, CHEN Zhen.Silver Nanoparticles Filling in TiO2 Hollow Nanofibers by Coaxial Electrospinning[J]. Acta Phys. -Chim. Sin., 2008,24(10): 1790-1796
140. LI Hai-Long; LUO Wu-Lin; CHEN Tao; TIAN Wen-Yu; SUN Mao; LI Chun; ZHU Di; LIU Ran-Ran; ZHAO Yu-Liang; LIU Chun-Li.Preparation and Photocatalytic Performance of Titania Nanotubes Loaded with Ag Nanoparticles[J]. Acta Phys. -Chim. Sin., 2008,24(08): 1383-1386
141. ZHANG Xu-Zhi; JIAO Kui.Single-Walled Carbon Nanotubes and RoomTemperature Ionic Liquid Composite Film Modified Electrode[J]. Acta Phys. -Chim. Sin., 2008,24(08): 1439-1444
142. SHI Jian; LI Jun; CAI Yun-Fa.Fabrication of C, N-Codoped TiO2 Nanotube Photocatalysts with Visible Light Response[J]. Acta Phys. -Chim. Sin., 2008,24(07): 1283-1286
143. GAO Li-Xia; WANG Li-Na; QI Tao; LI Yu-Ping; CHU Jing-Long; QU Jing-Kui.Electrodeposition of Aluminium from AlCl3/Et3NHCl Ionic Liquids[J]. Acta Phys. -Chim. Sin., 2008,24(06): 939-944
144. LUO Da-Chao; ZHANG Lan-Lan; LONG Hui-Jin; CHEN Yong-Mei; CAO Ya-An.Effect of Surface Modification by Ni2+ on Photocatalysis Activity of TiO2[J]. Acta Phys. -Chim. Sin., 2008,24(06): 1095-1099
145. LI Wei; RONG Hua; WU Xin-Min; CHEN Zhong-Yuan.Microwave Synthesis, Characterization and Theoretical Study of para-Toluenesulfonic Acid Threonine Salt and Its Ester Derivatives[J]. Acta Phys. -Chim. Sin., 2008,24(05): 868-872
146. FENG Cai-Xia; WANG Yan; JIN Zhen-Sheng; ZHANG Shun-Li.Kinetic Behavior of Visible Light Photocatalytic Oxidation of Propylene for N-Doped Nano-TiO2[J]. Acta Phys. -Chim. Sin., 2008,24(04): 633-638
147. LU Han-Feng; ZHOU Ying; XU Bo-Qing; CHEN Yin-Fei; LIU Hua-Zhang.Effect of Gold Doping on the Photocatalytic Activity of the Anatase TiO2[J]. Acta Phys. -Chim. Sin., 2008,24(03): 459-464
148. LIU Shou-Xin; CHEN Xiao-Yun.Effect of Pore Structure of Activated Carbon on the Photocatalytic Activity of TiO2/AC Composite Photocatalyst[J]. Acta Phys. -Chim. Sin., 2008,24(03): 533-538
149. WU Yu-Cheng; LIU Xiao-Lu; YE Min; XIE Ting; HUANG Xin-Min.Preparation and Properties of Carbon Nanotube-TiO2 Nanocomposites[J]. Acta Phys. -Chim. Sin., 2008,24(01): 97-102
150. ZHANG Jun-Jie; WU Min; QIN Yan-Tao; CHEN Rui; JIANG Yin-Hua; SUN Yue-Ming; YANG Zhao-Hui.Study on Zn(II) Tetracarboxy Phthalocyanine Doped TiO2 Electrode Using Electrochemical Impedance Spectrum[J]. Acta Phys. -Chim. Sin., 2008,24(01): 79-84
151. SUN Guo-Hua; LI Kai-Xi; FAN Hui; GU Jian-Yu; LI Qiang; LIU Yue.Eelectrochemical Performance of Capacitors Using [BMIm]BF4/Fc as Electrolyte[J]. Acta Phys. -Chim. Sin., 2008,24(01): 103-108
152. CHEN Qi-Yuan; TONG Hai-Xia; YIN Zhou-Lan; HU Hui-Ping; LI Jie; LIU Liang-Liang.Preparation, Characterization and Photo-catalytic Behavior of TiO2 Catalysts with Oxygen Vacancies[J]. Acta Phys. -Chim. Sin., 2007,23(12): 1917-1921
153. MA Chun-An; WANG Xiao-Juan; LI Guo-Hua; LI Mei-Chao; CHEN Song.Electroreduction Characteristics of Nitromethane in Ionic Liquid BMImBF4[J]. Acta Phys. -Chim. Sin., 2007,23(11): 1719-1722
154. LEI Sheng; ZHANG Jing; HUANG Jian-Bin.Promotion of the Surface Activity and Aggregation Ability of Sodium Dodecylsulfate in Aqueous Solution by Ionic Liquid 1-butyl-3-methyl-imidazolium Tetrafluoroborate[J]. Acta Phys. -Chim. Sin., 2007,23(11): 1657-1661
155. ZHU Lei; CUI Xiao-Li; SHEN Jie; YANG Xi-Liang; ZHANG Zhuang-Jian.Visible Light Photoelectrochemical Response of Carbon-doped TiO2 Thin Films Prepared by DC Reactive Magnetron Sputtering[J]. Acta Phys. -Chim. Sin., 2007,23(11): 1662-1666
156. WANG Jin-Bo; MING Fang-Yong; JIANG Wei-Dong; FAN Guang-Yin; LIU De-Rong; CHEN Hua; LI Xian-Jun.Asymmetric Hydrogenation of Acetophenone and Its Derivatives Catalyzed by Ruthenium Nanoparticles in Ionic Liquid Media[J]. Acta Phys. -Chim. Sin., 2007,23(09): 1381-1386
157. SUN Wei; GAO Rui-Fang; WANG Dan-Dan; JIAO Kui.Direct Electrochemistry of Hemoglobin at Room Temperature Ionic Liquid [BMIM]PF6 Modified Carbon Paste Electrode[J]. Acta Phys. -Chim. Sin., 2007,23(08): 1247-1251
158. YANG Hui; SHEN Qian-Hong; GAO Ji-Wei.Morphology Control of Anatase TiO2 Films Prepared at Low Temperature Using 4,4’-isopropylidenediphenol[J]. Acta Phys. -Chim. Sin., 2007,23(08): 1269-1274
159. TIAN Bao-Zhu; TONG Tian-Zhong; CHEN Feng; ZHANG Jin-Long.Effect of Water Washing Treatment on the Photocatalytic Activity of Au/TiO2 Catalysts[J]. Acta Phys. -Chim. Sin., 2007,23(07): 978-982
160. HUANG Dong-Sheng; ZENG Ren-Jie; CHEN Chao-Feng; LI Yu-Hua.Hydrophilicity of TiO2 Thin Films Codoped with Iron and Nitrogen[J]. Acta Phys. -Chim. Sin., 2007,23(07): 1037-1041
161. LI Shu; LIU Lei; CAO Zhen; WANG Ji-Qiang; YAN Tian-Ying.Molecular Dynamics Simulation on a Eutectic Systemof LiTFSI/Urea[J]. Acta Phys. -Chim. Sin., 2007,23(07): 983-986
162. WU Yan; YAO Wen-Qing; ZHU Yong-Fa.Interfacial Structure of Ta2O5/Si Filmand Photoactivity[J]. Acta Phys. -Chim. Sin., 2007,23(05): 625-629
163. MA Chun-An; CHEN Song; CHU You-Qun; MAO Xin-Biao.Electrochemical Reduction of Nitrobenzene in Ionic Liquid BMimBF4-H2O[J]. Acta Phys. -Chim. Sin., 2007,23(04): 575-580
164. DING Ying-Ying; LI Kui-Ying.Photoacoustic and Surface Photovoltaic Characters of Nanocrystalline TiO2[J]. Acta Phys. -Chim. Sin., 2007,23(04): 569-574
165. YAN Shan-Shan;WU Lian-Di;CHEN Feng;ZHANG Jin-Long.Low-temperature Preparation and Characterization of TiO2 Thin Films with a Bicrystalline Framework[J]. Acta Phys. -Chim. Sin., 2007,23(03): 414-418
166. LIN Qi;FU Hai-Yan;YUAN Mao-Lin;CHEN Hua;LI Xian-Jun.Carbonylation of Aryl Halide Catalyzed by Active-carbon Supported Ionic Liquid-phase Palladium Catalyst[J]. Acta Phys. -Chim. Sin., 2006,22(10): 1272-1276
167. GU Hong;XU Bo-Lian;ZHOU Jing;LI Yuan-Zhi;FAN Yi-Ning.Catalytic Properties of Supported Pd/TiO2 and Pd-Ag/TiO2 Catalysts for Selective Hydrogenation of Acetylene[J]. Acta Phys. -Chim. Sin., 2006,22(06): 712-715
168. LI Xue-Hui;JIANG Yan-Bin;ZHANG Lei;LI Rong.Synthesis and Characterization of N-ester Appended Pyridine Task-specific Ionic Liquids[J]. Acta Phys. -Chim. Sin., 2006,22(06): 747-751
169. Ding Yun-Sheng;Wang Seng-Shan;Zha Min;Wang Zhi-Gang.Adsorption and Aggregative Structures of an Organic Cation [C18mim] of the Ionic Liquid in the Interlayer of Montmorillonite[J]. Acta Phys. -Chim. Sin., 2006,22(05): 548-551
170. ZHANG Xue-Hong;TANG Xing-Hua;CHENG Xin-Sun.Synthesis and Application of Ce-doped Mesoporous TiO2[J]. Acta Phys. -Chim. Sin., 2006,22(05): 532-537
171. LI Xue-Hui;ZHANG Lei;WANG Le-Fu;TANG Ying-Biao.Characterization of N-carboxyl Appended Pyridine Task-Specific Ionic Liquids[J]. Acta Phys. -Chim. Sin., 2006,22(04): 430-435
172. LIN Qi;FU Hai-Yan;XUE Fang;YUAN Mao-Lin;CHEN Hua;LI Xian-Jun.Hydroformylation of Long-chain Olefins Catalyzed by Rhodium-Phosphine Complexes in New Ionic Liquids[J]. Acta Phys. -Chim. Sin., 2006,22(04): 465-469
173. ZHAI Cui-Ping;WANG Jian-Ji;XUAN Xiao-Peng;WANG Han-Qing.NMR Study on the Interactions of Ionic Liquid with Acetone[J]. Acta Phys. -Chim. Sin., 2006,22(04): 456-459
174. WANG Peng; CHEN Dong; LIU Jian-Shu; TANG Fang-Qiong.Synthesis and Characterization of Monodisperse TiO2 Colloid Particles[J]. Acta Phys. -Chim. Sin., 2006,22(03): 365-368
175. GENG Wei-guo; LI Xue-hui; WANG Le-fu; DUAN Hong-li; PAN Wei-ping.Acidic Characterization of Polycarboxyl Imidazolium Ionic Liquids[J]. Acta Phys. -Chim. Sin., 2006,22(02): 230-233
176. TONG Jing; ZHANG Qing-guo; HONG Mei; YANG Jia-zhen.Thermodynamic Properties of Ionic Liquid BMIAlCl4[J]. Acta Phys. -Chim. Sin., 2006,22(01): 71-75
177. WU Xiao-ping; LIU Zhi-ping; WANG Wen-chuan.Molecular Dynamics Simulation of Gas Solubility in Room Temperature Ionic Liquids[J]. Acta Phys. -Chim. Sin., 2005,21(10): 1138-1142
178. WU Xiao-ping; LIU Zhi-ping.Computer Simulation Study of the Mixtures of Room Temperature Ionic Liquid [bmim][BF4] and Water[J]. Acta Phys. -Chim. Sin., 2005,21(09): 1036-1041
179. CAO Jie-ming; WANG Jun; FANG Bao-qing; ZHENG Ming-bo; LU Hong-xia; CHANG Xin; WANG Hai-yan.Synthesis and Characterization of ZnO Nanomaterials with Different Morphologies in Ionic Liquids[J]. Acta Phys. -Chim. Sin., 2005,21(06): 668-672
180. PAN Xu; DAI Song-yuan; WANG Kong-jia; SHI Cheng-wu; GUO Li.Development and Application of Electrolyte based on Ionic Liquid in Dye-sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2005,21(06): 697-702
181. WANG Yong; LI Hao-Ran; WU Tao; WANG Cong-Min; HAN Shi-Jun.Reaction Mechanism Study for the Synthesis of Alkylimidazolium-based Halide Ionic Liquids[J]. Acta Phys. -Chim. Sin., 2005,21(05): 517-522
182. WANG Xiao-Hua; TAO Guo-Hong; WU Xiao-Mu; KOU Yuan.Investigation of the Acidity of Ionic Liquids by IR Spectroscopy[J]. Acta Phys. -Chim. Sin., 2005,21(05): 528-533
183. PU Min; CHEN Biao-Hua; LI Hui-Ying; LIU Kun-Hui.DFT Studies on Reaction Mechanism of the Double Bond Isomerization of Butene Catalyzed by 1-ethyl-3-methyl-imidazolium of the Ionic Liquid (II)[J]. Acta Phys. -Chim. Sin., 2005,21(04): 383-387
184. LI Zhi-Jie; HOU Bo; XU Yao; WU Dong; SUN Yu-Han.Preparation and Characterization of Silica-modified Titanium Dioxide Nanoparticles by Co-precipitation Method[J]. Acta Phys. -Chim. Sin., 2005,21(03): 229-233
185. YAN Qing-Zhi;SU Xin-Tai;ZHOU Yan-Ping;GE Chang-Chun.Controlled Synthesis of TiO2 Nanometer Powders by Sol-gel Auto-igniting Process and Their Structural Property[J]. Acta Phys. -Chim. Sin., 2005,21(01): 57-62
186. Li Yue-Xiang; Wang Tian-Hui; Peng Shao-Qin1 Lü Gong-Xuan; Li Shu-Ben.Synergistic Effect of Eu3+ and Si4+ Co-doping on Photocatalytic Activity of Titanium Dioxide[J]. Acta Phys. -Chim. Sin., 2004,20(12): 1434-1439
187. Li Xue-Hui; Zhang Lei; Li Qiong; Geng Wei-Guo; Ye Yu-Jia; Wang Le-Fu.TGA-FTIR Study of 1-n-butyl-3-methylimidazolium Bromide Ionic Liquid[J]. Acta Phys. -Chim. Sin., 2004,20(12): 1465-1468
188. Zhang Zhi-Heng; Guan Wei; Yang Jia-Zhen; Tan Zhi-Cheng; Sun Li-Xian.The Standard Molar Enthalpy of Formation of Room Temperature Ionic Liquid EMIES[J]. Acta Phys. -Chim. Sin., 2004,20(12): 1469-1471
189. Shen Jie;Wo Song-Tao;Cui Xiao-Li;Cai Zhen-Wei;Yang Xi-Liang;Zhang Zhuang-Jian.Photoelectrochemical Characteristics of Nano-Titanium Dioxide Thin Films Prepared by RF Magnetron Sputtering[J]. Acta Phys. -Chim. Sin., 2004,20(10): 1191-1195
190. Piao Ling-Yu;Han Yang;Kou Yuan.The Reuse of Acidic Ionic Liquids as Catalysts in Diphenyl Oxide Alkylation with Dodecene[J]. Acta Phys. -Chim. Sin., 2004,20(09): 1083-1088
191. Pu Min;Liu Kun-Hui;Li Hui-Ying;Chen Biao-Hua.DFT Studies on Reaction Mechanism of the Double Bond Isomerization of Butene Catalyzed by 1-ethyl-3-methyl-lmidazolium of the Ionic Liquid[J]. Acta Phys. -Chim. Sin., 2004,20(08): 826-830
192. Zhang Sheng-Mao;Zhang Chun-Li;Zhang Jing-Wei;Zhang Zhi-Jun;Dang Hong-Xin;Wu Zhi-Shen;Liu Wei-Min.Preparation of Silver Nanoparticles in Room Temperature Ionic Liquids[J]. Acta Phys. -Chim. Sin., 2004,20(05): 554-556
193. Zhang Qi;Li Xin-Jun;Li Fang-Bai;Chang Jie.Investigation on Visible -light Activity of WOx/TiO2 Photocatalyst[J]. Acta Phys. -Chim. Sin., 2004,20(05): 507-511
194. Liu Shou-Xin;Sun Cheng-Lin.Mechanism of Silver Modification for the Enhanced Photocatalytic Activity of Cr(VI) Reduction on TiO2 Photocatalyst[J]. Acta Phys. -Chim. Sin., 2004,20(04): 355-359
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