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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2007,Vol.23>> Issue(12)>> 1899-1904     doi: 10.3866/PKU.WHXB20071213         中文摘要
Hydrogen Production from Water Splitting Using Perylene Dye-Sensitized Pt/TiO2 Photocatalyst
LIU Fu-Sheng; JI Ren; WU Min; SUN Yue-Ming
School of Chemistry and Chemical Engineering, Southeast University, Nanjing 210096, P. R. China; Department of Chemistry and Materials Science, Nanjing Forestry University, Nanjing 210037, P. R. China
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The photocatalyst (DPPBI/Pt/TiO2)was prepared using N,N’-di(4-pyridyl)-3,4,9,10-perylene tetracarboxylic acid bisimide (DPPBI) sensitized Pt/TiO2 and characterized by infrared spectroscopy(IR), UV-Vis diffuse reflectance spectroscopy (UV-Vis DRS), scanning electron microscopy(SEM), X-ray photoelectron spectroscopy(XPS), and X-ray diffraction (XRD). The results of characterizationshowedthat the crystal form of TiO2was anatase, Ptwas highly dispersed on the surface of TiO2 and DPPBI was adsorbed on the surface of Pt/TiO2 in DPPBI/Pt/TiO2. Hydrogen production from water splitting using photocatalyst (DPPBI/Pt/TiO2) was studied. It has been found that the rate of hydrogen evolution reaches 6.69 滋 mol·h-1·g-1 under visible light irradiation for 8 h with 300 W Xe-lamp cold light source when 250 mL reactive liquid contains 0.8 g·L-1 photocatalyst (0.1%DPPBI/0.4%Pt/TiO2) and 0.2 mol·L-1 KI.

Keywords: Perylene   Dye   Photocatalyst   Hydrogen production  
Received: 2007-06-25 Accepted: 2007-09-19 Publication Date (Web): 2007-10-11
Corresponding Authors: SUN Yue-Ming Email: sun@seu.edu.cn


Cite this article: LIU Fu-Sheng; JI Ren; WU Min; SUN Yue-Ming. Hydrogen Production from Water Splitting Using Perylene Dye-Sensitized Pt/TiO2 Photocatalyst[J]. Acta Phys. -Chim. Sin., 2007,23 (12): 1899-1904.    doi: 10.3866/PKU.WHXB20071213
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