Article
Photocatalytic Degradation of Organic Pollutants on TiO2/Bentonite
LI Jing-Yi;SIQIN Gao-Wa;LIU Li-Na
Institute of Chemistry and Chemical Engineering, Inner Mongolia University, Hohhot 010021, P. R. China
Institute of Chemistry and Chemical Engineering, Inner Mongolia University, Hohhot 010021, P. R. China
A series of TiO2/bentonite catalysts (with different loadings and calcined at different temperatures) were prepared by sol-gel method. The prepared catalysts were employed to photocatalytically degrade organic dye Rhodamine B (RhB) under UV irradiation. The capabilities to degrade organic pollutants were studied by detecting the change of their absorbance and chemical oxygen demand (COD) under UV light irradiation. The results showed that they had a better catalytic reactivity when the loading was 50% and calcination temperature was 400 ℃ (Ti400). Their minerialization activity was slightly less than P25, when UV light irradiation time was 4 h, COD changes of P25 and TiO2/bentonite calcinated at 400 ℃ were 99.7% and 97.0%, respectively. But they were easier to be reused. Ti400 catalyst was employed to degrade RhB, and its photocatalytic activity was kept almost the same after recycling 7 times. The catalysts were further characterized by XRD, BET, and UV-Vis DRS. The experimental results showed that they would have a better activity when their BET surface area was larger.
Keywords: TiO2/bentonite catalysts Rhodamine B Photocatalytic degradation XRD BET UV-Vis DRS
Received: 2006-05-29 Accepted: 2006-07-26 Publication Date (Web): 2007-01-08
Corresponding Authors: LI Jing-Yi Email: lijingyicn@yahoo.com
Cite this article: LI Jing-Yi;SIQIN Gao-Wa;LIU Li-Na. Photocatalytic Degradation of Organic Pollutants on TiO2/Bentonite[J]. Acta Phys. -Chim. Sin., 2007,23 (01): 16-20. doi: 10.3866/PKU.WHXB20070104
Keywords: TiO2/bentonite catalysts Rhodamine B Photocatalytic degradation XRD BET UV-Vis DRS
Received: 2006-05-29 Accepted: 2006-07-26 Publication Date (Web): 2007-01-08
Corresponding Authors: LI Jing-Yi Email: lijingyicn@yahoo.com
Cite this article: LI Jing-Yi;SIQIN Gao-Wa;LIU Li-Na. Photocatalytic Degradation of Organic Pollutants on TiO2/Bentonite[J]. Acta Phys. -Chim. Sin., 2007,23 (01): 16-20. doi: 10.3866/PKU.WHXB20070104
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2． LI Song, LIU Fu-Feng, YU Lin-Ling, ZHAO Yan-Jiao, DONG Xiao-Yan.Dual Effect of Thioflavin T on the Nucleation Kinetics of Amyloid β-Protein 40[J]. Acta Phys. -Chim. Sin., 2016,32(6): 1391-1396
3． LIU Guo, LU Yuan-Yuan, ZHANG Jing, LI Zhi, FENG Zhao-Chi, LI Can.Phase Transformation and Photocatalytic Properties of Bi2O3 Prepared Using a Precipitation Method[J]. Acta Phys. -Chim. Sin., 2016,32(5): 1247-1256
4． GAO Sha, LAN Wen-Bo, LIN Ying-Wu, LIAO Li-Fu, NIE Chang-Ming.Molecular Recognition of α,β-Unsaturated Carbonyl Compounds and Chiral Guests by Uranyl-Salophen Receptors[J]. Acta Phys. -Chim. Sin., 2016,32(3): 683-690
5． TONG La-Ga, LIU Jin-Yan, WANG Cen-Chen, RONG Hua, LI Wei.Preparation of Micro/Nano ZnO Pompons and Their Catalytic Activity for the Solar Degradation of Organic Dyes[J]. Acta Phys. -Chim. Sin., 2015,31(8): 1615-1620
6． ZHANG Jun-Wei, ZHOU Jun-Gang, Lü Hong, HUANG Qiang.Molecular Dynamics Simulation of Active-Sites of Retaining and Inverting β-Xylosidases[J]. Acta Phys. -Chim. Sin., 2015,31(6): 1169-1178
7． QIAN Hai-Cheng, KANWAL Shahid, JIA Qing-Zhu, WANG Qiang, JI Hui-Fen, ZHU Zhi-Chen, XIA Shu-Qian, MA Pei-Sheng.Norm Index-Based Quantitative Structure-Activity Relationship to Predict β-Cyclodextrin Complex Binding Constants[J]. Acta Phys. -Chim. Sin., 2015,31(5): 893-898
8． HU Long-Xing, XU Dan-Dan, ZOU Lian-Pei, YUAN Hang, HU Xing.Heterogeneous Fenton Oxidation of Refractory Dye Rhodamine B in Aqueous Solution with Mesoporous Fe/SBA-15[J]. Acta Phys. -Chim. Sin., 2015,31(4): 771-782
9． ZHOU Han-Yang, YU Tian-Lin, AO Yin-Yong, PENG Jing, ZHAI Mao-Lin.Crystal Structure and Radiation Stability of Sr(NO3)2·DCH18C6 Complex[J]. Acta Phys. -Chim. Sin., 2014,30(8): 1581-1586
10． GU Yong-Qin, WANG Bo, GU Xiu-Quan, ZHAO Yu-Long, QIANG Ying-Huai, ZHANG Shuang, ZHU Lei.Preparation and Characterization of Co3(PO4)2/Ag3PO4 Nanocomposites for Visible-Light Photocatalysis[J]. Acta Phys. -Chim. Sin., 2014,30(10): 1909-1915
11． DONG Li-Li, WANG Ying-Yong, TONG Xi-Li, JIN Guo-Qiang, GUO Xiang-Yun.Synthesis and Characterization of Boron-Doped SiC for Visible Light Driven Hydrogen Production[J]. Acta Phys. -Chim. Sin., 2014,30(1): 135-140
12． XING Wei-Nan, NI Liang, YAN Xue-Sheng, LIU Xin-Lin, LUO Ying-Ying, LU Zi-Yang, YAN Yong-Sheng, HUO Peng-Wei.Preparation of C@CdS/Halloysite Nanotube Composite Photocatalyst Using One-Step Pyrolytic Method and Its Photodegradation Properties[J]. Acta Phys. -Chim. Sin., 2014,30(1): 141-149
13． YANG Cheng-Xu, JU Jing, ZHAO Shi-Di, XU Hang-Yu, LIU Meng, LIAO Fu-Hui, LI Guo-Bao, LIN Jian-Hua.Synthesis of β-FeSe by Salt-Flux Method under Air Atmosphere[J]. Acta Phys. -Chim. Sin., 2013,29(12): 2661-2666
14． SHAN Sheng-Sheng, YAN Chao, XU Liang.Dihedral Dynamics Analyses of the Polymorphic Properties of Zn2+-Bound Amyloid β40 (Aβ40) and β42 (Aβ42)[J]. Acta Phys. -Chim. Sin., 2013,29(12): 2630-2638
15． LIU Ying, MENG Xiang-Guang, YU Wei-Feng, LI Xiao-Hong, PENG Xiao.Hydrolysis of Methyl-β-D-cellobioside Catalyzed by Functional Micelles with Glutamic Acid under Mild Conditions[J]. Acta Phys. -Chim. Sin., 2013,29(10): 2263-2270
16． WANG Xiao-Xia, XU Hua-Long, SHEN Wei, RUHLMANN Laurent, QIN Feng, SORGUES Sébastien, COLBEAU-JUSTIN Christophe.Synthesis of Ternary Hybrid TiO2-SiO2-POM Catalysts and Its Application in Degrading Rhodamine B under Visible Light Illumination[J]. Acta Phys. -Chim. Sin., 2013,29(09): 1837-1841
17． LIN Xue, YU Li-Li, Yan Li-Na, GUAN Qing-Feng, Yan Yong-Sheng, ZHAO Han.Controllable Synthesis and Photocatalytic Activity of Spherical, Flowerlike and Threadlike Bismuth Vanadates[J]. Acta Phys. -Chim. Sin., 2013,29(08): 1771-1777
18． YANG Han-Pei, ZHANG Ying-Chao, FU Xiao-Fei, SONG Shuang-Shuang, WU Jun-Ming.Surface Modification of CNTs and Improved Photocatalytic Activity of TiO2-CNTs Heterojunction[J]. Acta Phys. -Chim. Sin., 2013,29(06): 1327-1335
19． HUANG Hai-Feng, JIA Jian-Ming, LU Han-Feng, ZHANG Hong-Hua, PAN Lie-Qun.Effect of Designed Zr/Ti Molar Ratio on the Photocatalytic Activity of Sr-Zr-Ti Mixed Oxide Catalysts under Visible Light[J]. Acta Phys. -Chim. Sin., 2013,29(06): 1319-1326
20． SHAO Zhi-Cheng, SONG Le-Xin, TENG Yue, DANG Zheng, XIA Juan.Increased Water Solubility of Molybdenum Trioxide Induced by β-Cyclodextrin[J]. Acta Phys. -Chim. Sin., 2013,29(03): 460-466
21． LIN Xue, GUAN Qing-Feng, LIU Ting-Ting, ZHANG Yao, ZOU Chun-Jie.Controllable Synthesis and Photocatalytic Activity of Bi4Ti3O12 Particles with Different Morphologies[J]. Acta Phys. -Chim. Sin., 2013,29(02): 411-417
22． WANG Bi-Yao, TAN Ning-Xin, YAO Qian, LI Ze-Rong, LI Xiang-Yuan.Accurate Calculation of the Reaction Barriers and Rate Constants of the Pyrolysis of Alkyl Radicals in the β Position Using the Isodesmic Reaction Method[J]. Acta Phys. -Chim. Sin., 2012,28(12): 2824-2830
23． FAN Hai-Bin, ZHANG Dong-Feng, GUO Lin.Fabrication, Formation Mechanism and the Photocatalytic Properties of Hierarchical Porous Hematite Networks[J]. Acta Phys. -Chim. Sin., 2012,28(09): 2214-2220
24． JI Ping-Li, WANG Jin-Gang, ZHU Xiao-Li, KONG Xiang-Zheng.Preparation of Silver Doped TiO2 Hollow Nanoparticles and Characterization of Their Structures and Photocatalytic Properties[J]. Acta Phys. -Chim. Sin., 2012,28(09): 2155-2161
25． LIN Xue, Lü Peng, GUAN Qing-Feng, LI Hai-Bo, LI Hong-Ji, CAI Jie, ZOU Yang.Visible Light Photocatalytic Properties of Bi3.25La0.75Ti3O12 Nanowires[J]. Acta Phys. -Chim. Sin., 2012,28(08): 1978-1984
26． ZHOU Liang-Chun, MENG Xiang-Guang, LI Jian-Mei, HU Wei, LIU Bo, DU Juan.Kinetics and Thermodynamics of Adsorption of Chlorophenols onto β-Cyclodextrin Modified Chitosan[J]. Acta Phys. -Chim. Sin., 2012,28(07): 1615-1622
27． LIN Xue, GUAN Qing-Feng, LI Hai-Bo, LI Hong-Ji, BA Chun-Hua, DENG Hai-De.Bi3.25Nd0.75Ti3O12 Nanostructures: Controllable Synthesis and Visible-Light Photocatalytic Activities[J]. Acta Phys. -Chim. Sin., 2012,28(06): 1481-1488
28． WU Qi, SU Yu-Feng, SUN Lan, WANG Meng-Ye, WANG Ying-Ying, LIN Chang-Jian.Preparation and Visible Light Photocatalytic Activity of Fe-N Codoped TiO2 Nanotube Arrays[J]. Acta Phys. -Chim. Sin., 2012,28(03): 635-640
29． CHEN Zhan.Molecular Structures of Buried Polymer Interfaces and Biological Interfaces Detected by Sum Frequency Generation Vibrational Spectroscopy[J]. Acta Phys. -Chim. Sin., 2012,28(03): 504-521
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31． SUN Hao, JIANG Yong-Jun, YU Qing-Sen, GAO Hui.Molecular Dynamics Simulations on the Role of Structural Mg2+ Ions in Phosphoryl Transfer Catalyzed by GSK-3β[J]. Acta Phys. -Chim. Sin., 2011,27(01): 207-212
32． LIU Shu-Ping, YUE Ming-Bo, WANG Yi-Meng.One-Step Synthesis of Mesoporous Beta Zeolite Using Phosphate[J]. Acta Phys. -Chim. Sin., 2010,26(08): 2224-2228
33． DANG Zheng, SONG Le-Xin.Powder X-Ray Diffraction Analyses for Molecule-Ion Adducts of β-Cyclodextrin with a Series of Inorganic Salts[J]. Acta Phys. -Chim. Sin., 2010,26(07): 1837-1841
34． MAO Xiao-Bo, WANG Chen-Xuan, LIU Lei, MA Xiao-Jing, NIU Lin, YANG Yan-Lian, WANG Chen.Study on the Fine Structure of Polypeptides at Solid-Liquid Interfaces by Scanning Tunneling Microscopy[J]. Acta Phys. -Chim. Sin., 2010,26(04): 850-861
35． HE Gui-Ping, ZHANG Jiang, YAO Ruo-He.Preparation, Structure and Photoluminescence of Er3+ and Ce3+/Ce4+ Doped β-BaB2O4 Nanorods[J]. Acta Phys. -Chim. Sin., 2010,26(03): 685-690
36． FENG Li-Li, ZHAO Wei, LIU Yang, JIAO Liang, LI Xing-Guo.Photocatalytic Degradation of Rhodamine B by Nanocrystalline TiO2 Loaded into MCM-41 Molecular Sieves[J]. Acta Phys. -Chim. Sin., 2009,25(07): 1347-1351
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38． DANG Zheng, SONG Le-Xin, PAN Shu-Zhen, WANG Mang.Preparation, Spectral Properties and Decomposition Behavior of a Novel β-Cyclodextrin and Sodium Arsenite Adduct Formed by Stirring[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1059-1064
39． SUN Xiu-Liang, HUANG Chong-Pin, ZHANG Jie, CHEN Biao-Hua.Location of Al and Acid Strength of Brφnsted Acid in Beta Zeolite[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1136-1142
40． WEI Zhuo, ZHANG Huai, CUI Wei, JI Ming-Juan.Molecular Docking and 3D-QSAR on Maleimide Derivatives as Glycogen Synthase Kinase-3β Inhibitors[J]. Acta Phys. -Chim. Sin., 2009,25(05): 890-896
41． CHEN Qi-Feng, JIANG Dong, XU Yao, WU Dong, SUN Yu-Han.Visible Region Photocatalysis of Ce-Si/TiO2 Synthesized Using Sol-Gel-Hydrothermal Method[J]. Acta Phys. -Chim. Sin., 2009,25(04): 617-623
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43． CHEN Ran, GONG Yan-Jun, LI Qiang, DOU Tao, ZHAO Zhen, XU Qing-Hu.Direct Synthesis and Characteristics of NH4-βZeolite with Hierarchical Pore Structure[J]. Acta Phys. -Chim. Sin., 2009,25(03): 539-544
44． LI Jun, FENG Jie, LI Wen-Ying, CHANG Hai-Zhou, XIE Ke-Chang.Determining Influences of the Aggregative State of Deoxidized Coal on Its Extraction by Molecular Mechanics and Molecular Dynamics Analysis[J]. Acta Phys. -Chim. Sin., 2008,24(12): 2297-2303
45． XIAO Li-Hua, SUN Kun-Peng, XU Xian-Lun.Catalytic Combustion of Methane over CeO2-MOx (M=La3+, Ca2+) Solid Solution Promoted Pd/γ-Al2O3 Catalysts[J]. Acta Phys. -Chim. Sin., 2008,24(11): 2108-2113
46． LI Jing-Yi; MA Jun-Hua; BAI Tu-Ya; SUYOU Le-Ma.Effect of Fluoride Ion on the Photocatalytic Degradation of Sulforhodamine B on TiO2/Bentonite[J]. Acta Phys. -Chim. Sin., 2007,23(08): 1213-1218
47． YAO Su-Wei; SONG Zhen-Xing; WANG Hong-Zhi.Fabrication and Magnetic Properties of Co/Cu Multilayer Nanowire Arrays[J]. Acta Phys. -Chim. Sin., 2007,23(08): 1306-1310
48． FENG Chun-Bo;DU Zhi-Ping;Zhao Yong-Hong;TAI Xiu-Mei;LI Qiu-Xiao .Photocatalytic Activity of Au Modified Nano-TiO2 for NPE-10 Degradation[J]. Acta Phys. -Chim. Sin., 2006,22(08): 953-957
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52． HE Mai; FANG Ping; XIE Guan-qun; XIE Yun-long; YAN Zong-lan; LUO Meng-fei.Characterization of CuO Species in CuO/CeO2-Al2O3 Catalysts by In-situ XRD, Raman Spectroscopy and TPR[J]. Acta Phys. -Chim. Sin., 2005,21(09): 997-1000
53． XIONG Yu-hua; LI Feng-yi.Degradation of Polyethylene Film by Fe3+/TiO2 Photocatalyst[J]. Acta Phys. -Chim. Sin., 2005,21(06): 607-611
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56． Ren Da-Sen;Bei Zong-Min;Huang Li;Shen Jie;Cui Xiao-Li;Yang Xi-Liang;Zhang Zhuang-Jian.The Effect of Dopant Sb on the Superhydrophilicity and the Microstructure of the Nanoscale TiO2 Thin Film[J]. Acta Phys. -Chim. Sin., 2004,20(04): 414-416
57． Wang Yin-Jie;Qi-Lu.The Influencing Factor for CO2 Absorption of Li2ZrO3 at High Temperature[J]. Acta Phys. -Chim. Sin., 2004,20(04): 364-367
58． Han Shi-Tong;Xi Hai-Ling;Fu Xian-Zhi;Wang Xu-Xu;Ding Zheng-Xin;Lin Zhi-Cong;Su Wen-Yue.Study on the Photocatalytic Degradation of a Simulate Agent (2-CEES) of Mustard Gas[J]. Acta Phys. -Chim. Sin., 2004,20(03): 296-301
59． Guo Hui-Fen;Zhang Xing-Tang;Liu Bing;Li Yun-Cai;Huang Ya-Bin;Du Zu-Liang.Preparation of Nanometer-sized BaTiO3 Crystallites by Sol-gel Method and Size Effects on Structure[J]. Acta Phys. -Chim. Sin., 2004,20(02): 164-168
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61． Niu Zhen-Jiang;Wu Ting-Hua;Li Ze-Lin.In situ XRD Investigation on the Crystallization Behaviors of Electroless High-Phosphorous Ni-P Alloys[J]. Acta Phys. -Chim. Sin., 2003,19(08): 705-708
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63． Guo Min;Diao Peng;Ren Yan-Jie;Wang Bin;Cai Sheng-Min.Preparation and Characterization of Highly Oriented ZnO Single Crystal Submicrorod Arrays[J]. Acta Phys. -Chim. Sin., 2003,19(05): 478-480
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65． Wei Shi-Qiang;Zhang Xin-Yi;Liu Wen-Han;Wang Xiao-Guang;Yang Hong-Wei;Yan Wen-Sheng.Structural Study of Ni-B Ultrafine Amorphous Alloy during Annealed Crystallization[J]. Acta Phys. -Chim. Sin., 2001,17(08): 750-752
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