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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2005,Vol.21>> Issue(06)>> 653-657     doi: 10.3866/PKU.WHXB20050615         中文摘要
The Reaction Mechanism for the Synthesis of 1-methoxy-2-propanol on MgO Catalyst
ZHANG Wen-yu; DONG Qing-nian; ZHAO Ning; WEI Wei; SUN Yu-han
State Key Laboratory of Coal Conversion, Shanxi Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan 030001; Graduate School of the Chinese Academy of Sciences, Beijing 100049
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The addition of propylene oxide with methanol was carried out over MgO and a detailed mechanism of the reaction was investigated by using FT-IR method. In-situ FT-IR revealed that methanol dissociation into methoxide and proton took place readily on MgO, and propylene oxide adsorbed on MgO could generate propylenelike species via carbanion intermediate. As a result, methanol dissociated into adsorbed methoxide and reacted with the propylenelike species in antiMarkownikov fashion, which led to the high selectivity to 1-methoxy-2-propanol on MgO.

Keywords: Methanol   Poropylene oxide   IR   1-methoxy-2-propanol   MgO  
Received: 2004-12-20 Accepted: 2005-01-25 Publication Date (Web): 2005-06-15
Corresponding Authors: SUN Yu-han Email: yhsun@sxicc.ac.cn


Cite this article: ZHANG Wen-yu; DONG Qing-nian; ZHAO Ning; WEI Wei; SUN Yu-han. The Reaction Mechanism for the Synthesis of 1-methoxy-2-propanol on MgO Catalyst[J]. Acta Phys. -Chim. Sin., 2005,21 (06): 653-657.    doi: 10.3866/PKU.WHXB20050615
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91. ZHANG Qiang, QIAO Xiao-Jing, ZHANG Jian-Guo, ZUO Xiao-Li.Flash Pyrolysis of Trinitrophloroglucinol Metallic (Li, Na, K, Mg) Compounds[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1081-1087
92. NI Zhe-Ming, MAO Jiang-Hong, PAN Guo-Xiang, XU Qian, LI Xiao-Nian.Mechanism of Palladium-Catalyzed Methanol Decomposition for Hydrogen Production[J]. Acta Phys. -Chim. Sin., 2009,25(05): 876-882
93. DONG Lin-Mao, LI Xiao-Dong, YANG Rong-Jie.Thermal Decomposition of Hexanitrohexaazaisowurtzitane and Its Residues[J]. Acta Phys. -Chim. Sin., 2009,25(05): 981-986
94. WANG Jian-She, GUO Xun, SONG Cheng-Ying, WANG Liu-Cheng, ZHAO Jian-Hong, QIU Xin-Ping.Promoting Methanol Electro-Oxidation through Fabricating Pore Structure in Pt/CNTs Catalyst Layer by Dissolving Away Premixed La2O3 Particles[J]. Acta Phys. -Chim. Sin., 2009,25(04): 767-772
95. YANG Hong-Yan, GUO Pan-Pan, LI Wei-Shan.Electrodeposition Preparation and Activity of CO-Resistant Catalyst Pt-HxWO3 for Methanol Oxidation[J]. Acta Phys. -Chim. Sin., 2009,25(04): 719-723
96. XU Lei; WU Shu-Jie; ZHANG Wen-Xiang; JIA Ming-Jun; LIU Gang.Vapour Phase ortho-Selective Alkylation of Phenol with Methanol over Fe-Zr Oxide Catalysts[J]. Acta Phys. -Chim. Sin., 2009,25(02): 242-246
97. LI Lai-Cai; WANG Yi-Wei; TIAN An-Min.Adsorption of Methanol on the Pt-Mo(111)/C Surface[J]. Acta Phys. -Chim. Sin., 2008,24(11): 2013-2018
98. PAN Lei-Ming, ZHOU Zhi-You, CHEN De-Hun, SUN Shi-Gang.Electrochemical and In Situ FTIR Studies of Adsorption and Oxidation of Dimethyl Ether on Platinum Electrode[J]. Acta Phys. -Chim. Sin., 2008,24(10): 1739-1744
99. YU Jun, WU Gui-Sheng, MAO Dong-Sen, LU Guan-Zhong.Effect of La2O3 on Catalytic Performance of Au/TiO2 for CO Oxidation[J]. Acta Phys. -Chim. Sin., 2008,24(10): 1751-1755
100. CHANG Xiao-Tu, WANG Jian-Ming, SHAO Hai-Bo, WANG Jun-Bo, ZENG Xiao-Xu, ZHANG Jian-Qing, CAO Chu-Nan.Corrosion and Anodic Behaviors of Pure Aluminumin a Novel Alkaline Electrolyte[J]. Acta Phys. -Chim. Sin., 2008,24(09): 1620-1624
101. WANG Hong-Guo; JIANG Heng; XU Jing; SUN Zhao-Lin; ZHANG Xiao-Tong; ZHU He-Li; SONG Li-Juan.Effects of Benzene and 1-Octene on Desulfurization by Selective Adsorption with Ce(IV)Y[J]. Acta Phys. -Chim. Sin., 2008,24(09): 1714-1718
102. ZHENG Bo; LI He-Xian; WANG Guo-Chang; LIU Kun; YUAN Wei; LI He; LIANG Bo.Supramolecular Complexation in Water-Methanol Mixtures[J]. Acta Phys. -Chim. Sin., 2008,24(08): 1503-1506
103. ZHENG Gen-Wen; GONG Chun-Li; WEN Sheng; XIE Xiao-Lin.Preparation and Performances of Sulfonated Poly(ether imide) and Poly (ether sulfone) Blends for Proton Exchange Membrane[J]. Acta Phys. -Chim. Sin., 2008,24(05): 855-860
104. ZHU Rong-Shu; GUO Ming-Xin; OUYANG Feng.Reaction of NO over Iridium Catalysts with Excess Oxygen[J]. Acta Phys. -Chim. Sin., 2008,24(05): 909-914
105. TIAN Ying; LI Zhe-Qi; XU Hong-Feng; WU Yan-Bo; YANG Feng-Lin.Effects of Different Electrolyte Solutions on Characteristics of Polypyrrole-Modified Films[J]. Acta Phys. -Chim. Sin., 2008,24(04): 612-618
106. LIANG Ying; LIAO Dai-Wei.Effects of pH on the PtRu/C Catalyst Prepared by Microwave-assisted Ethylene Glycol Process[J]. Acta Phys. -Chim. Sin., 2008,24(02): 317-322
107. LIU Fu-Guo; DU Min; ZHANG Jing; QIU Meng.Inhibition Mechanismof Imidazoline Derivative Inhibitor for Q235 Steel in Saltwater Saturated with CO2[J]. Acta Phys. -Chim. Sin., 2008,24(01): 138-142
108. RAMACHANDRAN K.; SIVAGURUNATHAN P.; DHARMALINGAN K.. MEHROTRA S. C..Dielectric Relaxation Study of Amide-Alcohol Mixtures by Using Time Domain Reflectometry[J]. Acta Phys. -Chim. Sin., 2007,23(10): 1508-1514
109. DENG Hui-Ning; WANG Yu-Xin.Preparation and Properties of Proton Conducting Composite Membranes from Sulfonated Poly(phthalazinone ether keton) and Phosphotungstic Acid[J]. Acta Phys. -Chim. Sin., 2007,23(08): 1235-1240
110. XU Hui-Yuan; CHU Wei; CI Zhi-Min.Effect of Glow Discharge Plasma on Copper-based Catalysts for Methanol Synthesis[J]. Acta Phys. -Chim. Sin., 2007,23(07): 1042-1046
111. YUE Qiao-Hong; SHAO Xiao-Hong; CAO Da-Peng.Separation of Hydrogen and Carbon Dioxide in Activated Mesocarbon Microbeads with High Specific Surface[J]. Acta Phys. -Chim. Sin., 2007,23(07): 1080-1084
112. ZHENG Hai-Tao; LI Yong-Liang; LIANG Jian-Ying; SHEN Pei-Kang.Methanol Oxidation on Pd-based Electrocatalysts[J]. Acta Phys. -Chim. Sin., 2007,23(07): 993-996
113. YAN Zong-Cheng; CHEN Li; WANG Hong-Lin.Glow Discharge Plasma Electrolysis of Methanol Solutions[J]. Acta Phys. -Chim. Sin., 2007,23(06): 835-840
114. LI Lan-Lan; WEI Zi-Dong; YAN Can; LUO Yi-Hui; YIN Guang-Zhi; SUN Cai-Xin.Methanol Oxidation on a Pt ElectrodeModified by Underpotential Deposition of Ru[J]. Acta Phys. -Chim. Sin., 2007,23(05): 723-727
115. ZHAO Wen-Xia; HU Man-Cheng; LI Shu-Ni; JIANG Yu-Cheng; ZHANG Xiao-Lei; HU Lei; CHEN Huai-Jun.The Solubility of Ternary SystemRbBr/CsBr-CH3OH/C2H5OH-H2O at Different Temperatures[J]. Acta Phys. -Chim. Sin., 2007,23(05): 695-700
116. TANG Yan-Jun; LI You-Ming; SONG Jing; PAN Zhi-Dong.Structural Characterization and Thermal Decomposition Behavior of Microsized and Nanosized CaCO3[J]. Acta Phys. -Chim. Sin., 2007,23(05): 717-722
117. WANG Huan-Ping; ZHANG Qi-Long; YANG Hui; SUN Hui-Ping.Synthesis and Microwave Dielectric Properties of (Ca1-xMgx)SiO3 Ceramic by Sol-Gel Process[J]. Acta Phys. -Chim. Sin., 2007,23(04): 609-613
118. WU Wei; CAO Jie-Ming; CHEN Yu; LU Tian-Hong.Preparation of High-alloying Pt-Ru/CMK-3 Catalysts in THF-H2O-EtOH Ternary Solution System[J]. Acta Phys. -Chim. Sin., 2007,23(04): 559-564
119. YIN Li-Song;CHEN Min-Tao;LI Ting;ZHOU Ke-Sheng;GAO Song-Hua.Preparation of Rhombic MgO Nanoflakes from Dolomites[J]. Acta Phys. -Chim. Sin., 2007,23(03): 433-437
120. ZHANG Cheng-Gen;LI Wen-Zuo;HUANG Ming-Bao.Reaction of Methyl Alcohol with Thionyl Chloride in Solution[J]. Acta Phys. -Chim. Sin., 2007,23(03): 399-403
121. HAO Zhi-Xian;LIU Hui;GUO Bin;LI Hong;ZHANG Jia-Wei;GAN Li-Hua;XU Zi-Jie;CHEN Long-Wu.Sol-Gel Synthesis of Alumina Using Inorganic Salt Precursor[J]. Acta Phys. -Chim. Sin., 2007,23(03): 289-294
122. ZHANG Shu-Dong;ZHU Xiang-Jun;WANG Yan;KONG Xiang-He.Multiphoton Ionization Mass Spectrum of Methanol Clusters and Ab Initio Calculations[J]. Acta Phys. -Chim. Sin., 2007,23(03): 379-383
123. SIVAGURUNATHAN P.;RAMACHANDRAN K.;DHARMALINGAM K..FTIR Spectroscopic Studies on Molecular Interaction between Alcohols and N,N-dimethylacetamide[J]. Acta Phys. -Chim. Sin., 2007,23(03): 295-298
124. DENG Hui-Ning;WANG Yu-Xin .Sulfonated Poly(phthalazinones) Membranes For Direct Methanol Fuel Cell[J]. Acta Phys. -Chim. Sin., 2007,23(02): 187-191
125. HUANG Mian-Yan;CHEN Hua-Yan;GUO Jian-Zhao;WANG Zhi-Tao;XU Li;WANG Yu-Xin.Methanol Resistant Poly(Ether Sulfone)/Sulfonated Poly(Ether Ether Ketone) Blend Proton Exchange Membrane for DMFC[J]. Acta Phys. -Chim. Sin., 2007,23(01): 44-49
126. SHEN Pei-Kang;WANG Sheng-Long;HU Zhi-Yi;LI Yong-Liang;ZENG Rong;HUANG Yue-Qiang.Hydrogen Production by Alcohol Electrolysis[J]. Acta Phys. -Chim. Sin., 2007,23(01): 107-110
127. LIN Cui-Ying;ZHAO Jian-Xi.Effect of NaBr on the Ability of C12-s-C12•2Br Reverse Micelles for Solubilizing Water in Chloroform[J]. Acta Phys. -Chim. Sin., 2006,22(12): 1501-1505
128. RAMACHANDRAN Krishnamurthy;DHARMALINGAM Kurunthu;SIVAGURUNATHAN Periyasamy.Hydrogen Bonding Interaction between N-methylformamide and Alcohols[J]. Acta Phys. -Chim. Sin., 2006,22(12): 1560-1562
129. GUO Hao;DAI Shu-Xi;SUN Cheng-Feng;WU Chao;HUANG Ya-Bin;DU Zu-Liang.In situ Raman Spectroscopy of Langmuir Monolayers at Air-Water Interface[J]. Acta Phys. -Chim. Sin., 2006,22(09): 1061-1064
130. HU Ji-Ming;HOU Yan-Yuan;WANG Xiao-Mei;ZHANG Jian-Qing;CAO Chun-Nan .Effect of Calcination Procedure on the Electrocatalytic Activities of Ti/IrO2 Electrodes in Acidic Aqueous Solution[J]. Acta Phys. -Chim. Sin., 2006,22(08): 1010-1014
131. LI Ai-Ping;KAN Cheng-You;DU Yi;LIU De-Shan.Study on the Evolvement of Structure in Synthesis of Urea-Formaldehyde Resins by FTIR[J]. Acta Phys. -Chim. Sin., 2006,22(07): 873-877
132. GUAN Hong-Bo;WANG Pei;WANG Hui;ZHAO Bi-Ying;ZHU Yue-Xiang;XIE You-Chang.Preparation of Nanometer Magnesia with High Surface Area and Study on the Influencing Factors of the Preparation Process[J]. Acta Phys. -Chim. Sin., 2006,22(07): 804-808
133. JIN Guo-Jie;GUO Yang-Long;LIU Xiao-Hui;YAO Wei;GUO Yun;WANG Yun-Song;YUAN Fang;LU Guan-Zhong.In situ FT-IR Study on the Direct Gas Phase Epoxidation of Propylene over Ag-MoO3 Catalyst[J]. Acta Phys. -Chim. Sin., 2006,22(07): 809-814
134. ZHANG Xue-Hong;TANG Xing-Hua;CHENG Xin-Sun.Synthesis and Application of Ce-doped Mesoporous TiO2[J]. Acta Phys. -Chim. Sin., 2006,22(05): 532-537
135. LI Hui-Juan;JIANG Xiao-Yuan;ZHENG Xiao-Ming.Synthesis of TiO2/[[gamma]]r-Al2O3 and Effect of CuO Loading on NO Reduction[J]. Acta Phys. -Chim. Sin., 2006,22(05): 584-589
136. CHEN Ling; WANG Xin-dong; GUO Min.The Effect of NdOx as Co-catalyst for the Electro-oxidation of Methanol on PtRu/C[J]. Acta Phys. -Chim. Sin., 2006,22(02): 141-145
137. CHEN Yu; TANG Ya-wen; Kong Ling-yong; LIU Chang-peng; XING Wei; LU Tianhong.Effect of Surface Modification Extent of Carbon Nanotubes on Electrocatalytic Performance of Carbon Nanotubes Supported Pt catalyst[J]. Acta Phys. -Chim. Sin., 2006,22(01): 119-123
138. LIN Heng; CHEN Guo-liang; ZHENG Zi-shan; ZHOU Jian-zhang; CHEN Sheng-pei; LIN Zhong-hua.The Adsorption and Oxidation of Isopropanol at Platinum Electrode in Alkaline Media[J]. Acta Phys. -Chim. Sin., 2005,21(11): 1280-1284
139. WANG Zhen-bo; YIN Ge-ping; SHI Peng-fei.The Influence of Three Groups of Pt-Ru/C Catalyst’s Precursors on Its Performance for Direct Methanol Fuel Cell[J]. Acta Phys. -Chim. Sin., 2005,21(10): 1156-1160
140. GUAN Hong-bo; LIANG Jian; ZHU Yue-xiang; ZHAO Bi-ying; XIE You-chang.Structure Characterization and Monolayer Dispersion Phenomenon of MgO-ZrO2 Prepared by Co-precipitation[J]. Acta Phys. -Chim. Sin., 2005,21(09): 1011-1016
141. WU Xiao-ping; LIU Zhi-ping.Computer Simulation Study of the Mixtures of Room Temperature Ionic Liquid [bmim][BF4] and Water[J]. Acta Phys. -Chim. Sin., 2005,21(09): 1036-1041
142. LANG; Xu-qing; MA Hong-qin; TAN Xin; ZHU Hui-ming.Surface Activation and Graft of the Ultrafine PTFE Particles[J]. Acta Phys. -Chim. Sin., 2005,21(07): 703-706
143. LI Yong-Xin; GUO Yu-Hua; JI Yong-Qiang.Catalytic Activity of M/(MgO)y(CeO2)1-y (M=Ni, Co, Cu) Catalysts for Methane Combustion[J]. Acta Phys. -Chim. Sin., 2005,21(05): 468-473
144. CHEN Yu; TANG Ya-Wen; LIU Chang-Peng; XING Wei; LU Tian-Hong.Research Progress on Proton Exchange Membranes for Direct Methanol Fuel Cell[J]. Acta Phys. -Chim. Sin., 2005,21(04): 458-462
145. JIA Yu-Xiang; GUO Xiang-Yun.Monte Carlo Simulation of Adsorption Process of CO and H2 in Supercritical Fluids[J]. Acta Phys. -Chim. Sin., 2005,21(03): 306-309
146. MA Zhong-Yi;YANG Cheng;DONG Qing-Nian;WEI Wei;LI Wen-Huai;SUN Yu-Han.A Study of CO2/H2 Adsorption on Zirconia Polymorphs[J]. Acta Phys. -Chim. Sin., 2005,21(02): 225-228
147. ZHANG Tao;GU Ting-Kun;QI Yuan-Hua.Evolvement on the Microstructure of Molten Compound AuCu3 in Rapid Cooling[J]. Acta Phys. -Chim. Sin., 2005,21(02): 173-176
148. Li Xue-Hui; Zhang Lei; Li Qiong; Geng Wei-Guo; Ye Yu-Jia; Wang Le-Fu.TGA-FTIR Study of 1-n-butyl-3-methylimidazolium Bromide Ionic Liquid[J]. Acta Phys. -Chim. Sin., 2004,20(12): 1465-1468
149. Deng Hui-Ning;Li Lei;Xu Li;Wang Yu-Xin.Comparison on Properties of Membranes for Direct Methanol Fuel Cell[J]. Acta Phys. -Chim. Sin., 2004,20(11): 1372-1375
150. Ma Zhong-Yi;Xu Run;Yang Cheng;Wei Wei;Li Wen-Huai;Sun Yu-Han.Preparation and Surface Properties of Different Zirconia Polymorphs[J]. Acta Phys. -Chim. Sin., 2004,20(10): 1221-1225
151. Wang Fan;Yang Zhan-Lan;Zhang Li;Weng Shi-Fu;Wu Jin-Guang.FT-IR Study of the Interaction between Phosphatidylcholine and Bovine Serum Albumin[J]. Acta Phys. -Chim. Sin., 2004,20(10): 1186-1190
152. Wang Hai-Shui;Wang Yi-Bing;Xi Shi-Quan.A Review for the Preparation and Structural Characterization of Thin Films of Charge-Transfer Complexes[J]. Acta Phys. -Chim. Sin., 2004,20(10): 1281-1286
153. Sun Shi-Gang.Enhanced IR Absorption and Abnormal IR Effects of Low-dimensional Nanomaterials[J]. Acta Phys. -Chim. Sin., 2004,20(08S): 1017-1023
154. Cao Jiang-Lin;Leng Wen-Hua;Zhang Jian-Qing;Cao Chu-Nan.Adsorption Behavior and Photooxidation Kinetics of OH- at TiO2 Thin Film Electrodes[J]. Acta Phys. -Chim. Sin., 2004,20(07): 735-739
155. Hu Ji-Ming;Zhang Jian-Qing;Zhang Jin-Tao;Cao Chu-Nan.Electrochemical Activities of IrO2 Electrodes in Small Organic Molecules Containing Aqueous Solutions[J]. Acta Phys. -Chim. Sin., 2004,20(07): 740-744
156. Yun Hong;Chen Jian-Hua;Zhang Hui;Lin Jing-Dong;Chen Hong-Bo;Lin Chang-Jian.The Effects of ZrO2 on Cu-ZnO-ZrO2 Catalysts for Hydrogen Generation by Steam Reforming of Methanol[J]. Acta Phys. -Chim. Sin., 2004,20(05): 550-553
157. Yun Hong;Zhang Hui;Chen Jian-Hua;Chen Hong-Bo;Lin Chang-Jian.The Intermediate State and Mechanism of the Steam Reforming of Methanol over CuO-ZnO-ZrO2 Catalysts[J]. Acta Phys. -Chim. Sin., 2004,20(05): 524-528
158. Peng Cheng;Cheng Xuan;Zhang Ying;Chen Ling;Fan Qing-Bai.Comparison of Methanol Electrooxidation on Carbon Supported Pt and PtRu Catalysts[J]. Acta Phys. -Chim. Sin., 2004,20(04): 436-439
159. Chen You-Jiang;Sun Shi-Gang;Gong Hui;Chen Sheng-Pei;Zhou Zhi-You;Li Jun-Tao.Nanostructured Films Prepared on Pt Microelectrode through Square Wave Oxidation-reduction Cycles and Their Particular IR Properties[J]. Acta Phys. -Chim. Sin., 2004,20(02): 129-133
160. Zhou Hai-Hui;Jiao Shu-Qiang;Chen Jin-Hua;Wei Wan-Zhi;Kuang Ya-Fei.Electrocatalytic Oxidation of Methanol on Nano-fibular Polyaniline Electrode Modified with Pt Microparticles[J]. Acta Phys. -Chim. Sin., 2004,20(01): 9-14
161. Zhang Li;Liu Hong-Guo;Kang Shi-Zhao;Zhang Ren-Jie;Mou Ying-Di;Qian Dong-Jin;Feng Xu-Sheng.The Fabrication of New Luminescent Thin Films of Europium Complex/TiO2/AA by Langmuir-Blodgett Technique[J]. Acta Phys. -Chim. Sin., 2003,19(12): 1146-1149
162. Liu Ji-Xin;Xie You-Chang.Single-wall Carbon Nanotubes Produced by Decomposition of CH4 on W-Fe-MgO Catalysts[J]. Acta Phys. -Chim. Sin., 2003,19(11): 1093-1096
163. Xu Yi-Jun;Li Jun-Qian;Zhang Yong-Fan.O2 Adsorption on MgO(001) Surface with Oxygen and Magnesium Vacancies[J]. Acta Phys. -Chim. Sin., 2003,19(09): 815-818
164. Xu Yi-Jun;Li Jun-Qian;Zhang Yong-Fan;Chen Wen-Kai.Theoretical Study of O2 Adsorption on Perfect and Defect Sites of MgO(001) Surface[J]. Acta Phys. -Chim. Sin., 2003,19(05): 414-418
165. Chen Wei;Sun Shi-Gang;Si Di;Chen Sheng-Pei.Electrocatalytic Properties of Agglomerates of Pt Nanoparticles in Methanol Oxidation[J]. Acta Phys. -Chim. Sin., 2003,19(05): 441-444
166. Li Xu-Guang;Han Fei;Xing Wei;Tang Ya-Wen;Lu Tian-Hong.Influence of Methanol on the Kinetics of Oxygen Reduction on Pt/C and CoPcTc/C[J]. Acta Phys. -Chim. Sin., 2003,19(04): 380-384
167. Sheng Xia;Fang Kun;Zou Gang;He Ping-Sheng;Lü Wei-Xing.Component-controllable Monolayer of Ru Chelate Complex[J]. Acta Phys. -Chim. Sin., 2003,19(03): 237-241
168. Zhen Chun-Hua;Fan Chun-Jie;Gu Yan-Juan;Chen Sheng-Pei;Sun Shi-Gang.Adsorption and Oxidation of Glycine on Au Film Electrodes in Alkaline Solutions[J]. Acta Phys. -Chim. Sin., 2003,19(01): 60-64
169. Zhang Xin-Rong;Shi Peng-Fei.Catalytic Production of Hydrogen from Steam Reforming of Methanol on CeO2 Promoted Cu/Al2O3 Catalysts[J]. Acta Phys. -Chim. Sin., 2003,19(01): 85-89
170. Wang Jin;Chen Hong-Bo;Yun Hong;Lin Jing-Dong;Yi Jun;Zhang Hong-Bin;Liao Dai-Wei.Study on Rh-ZnO/MWNTs Catalyst for Methanol Synthesis[J]. Acta Phys. -Chim. Sin., 2003,19(01): 65-69
171. Chen Song-Zhe;Zhong Shun-He.The Photo Stimulated Surface Reaction of Synthesis of Methanol from Carbon Dioxide and Water on Cu/TiO2-NiO[J]. Acta Phys. -Chim. Sin., 2002,18(12): 1099-1103
172. Wei Zi-Dong;Miki Atsushi;Ohmori Tadayoshi;Osawa Masatoshi.Methanol Electroxidation on Upd - Sn Modified Platinum Electrodes[J]. Acta Phys. -Chim. Sin., 2002,18(12): 1120-1124
173. Shao Min-Hua;Huang Ruo-Shuang;Hu Rong-Gang;Lin Chang-Jian.Fabrication of Composite Scanning Micro pH Electrode and Its Application in Localized Corrosion[J]. Acta Phys. -Chim. Sin., 2002,18(10): 934-937
174. Xu Yong-Xiang;Yan Chuan-Wei;Gao Yan-Min;Cao Chu-Nan.Diffusion and Existing Form of Water Vapour in Organic Coatings[J]. Acta Phys. -Chim. Sin., 2002,18(07): 649-652
175. Guo Xia;Xu Hui;Guo Rong.The Fluorescence Quenching of Anthracene by Phenothiazine in Sodium Dodecyl Sulfate / Benzyl Alcohol / Water Microemulsion[J]. Acta Phys. -Chim. Sin., 2002,18(06): 500-503
176. Gao Hong-Wen;Zi Yan-Qin;Li Yu-Cheng.Langmuir Aggregation of Polychrome Blue on Nucleic Acids[J]. Acta Phys. -Chim. Sin., 2002,18(06): 540-544
177. Gong Hai-Ning;Shen Hua;Huang Hui-Zhong;Wu Nian-Zu.Preliminary Exploration of Touggard′s Method Used for the Background[J]. Acta Phys. -Chim. Sin., 2002,18(04): 326-331
178. Yang Cheng;Dong Qing-Nian;Zhang Jing;Ren Jie;Sun Yu-Han;Xie Ya-Ning;Hu Tian-Dou.The Structural Effect of CeO2 and La2O3 Modified Pd/γ-Al2O3 Catalysts[J]. Acta Phys. -Chim. Sin., 2002,18(02): 170-174
179. Zhou Ling-Ping;Deng Liang;Kou Yuan;Li Xuan-Wen.Studies on Acidity and Basicity and Adsorption of Modified Y Zeolites[J]. Acta Phys. -Chim. Sin., 2002,18(02): 142-146
180. Xi Jing-Yu;Wang Zhi-Fei;Wang Wei-Ping;Lü Gong-Xuan.In-situ XPS Study for Reaction Mechanism of Methanol Decomposition over Cu-Ni/Zn Catalyst[J]. Acta Phys. -Chim. Sin., 2002,18(01): 82-86
181. Wang Jue;Zhao Bi-Ying;Xie You-Chang.Correlations between the Dispersion State of MgO and Catalytic Behavior of[J]. Acta Phys. -Chim. Sin., 2001,17(11): 966-971
182. Xi Jing-Yu;Lv Gong-Xuan;Wang Zhi-Fei.Partial Oxidation of Methanol to Hydrogen over Cu/Zn and Cu/Zn/Ni Catalysts[J]. Acta Phys. -Chim. Sin., 2001,17(07): 655-658
183. Li Han-Sheng;Zhong Shun-He;Wang Jian-Wei;Xiao Xiu-Fen.Effect of K2O on Properties of Cu-Ni/V2O5-SiO2 Catalyst for the Synthesis of Dimethyl Carbonate[J]. Acta Phys. -Chim. Sin., 2001,17(06): 552-554
184. Lin Zhong-Yu;Fu Jin-Kun;Wu Jian-Ming;Liu Yue-Ying;Cheng Hu.Preliminary Study on the Mechanism of Nonenzymatic Bioreduction of Precious Metal Ions[J]. Acta Phys. -Chim. Sin., 2001,17(05): 477-480
185. Chen Ping, Zheng Xiao-Ming, Meyer S, Temps F.FTIR Study of Kinetics of the Reaction between HCO Radicals and NO2[J]. Acta Phys. -Chim. Sin., 2000,16(11): 1043-1047
186. Sun Ying, Yang Zhan-Lan, Zhang Li, Weng Shi-Fu, Wu Jin-Guang.Interaction of Ca2+、La3+ and Eu3+ with NaDC Micelle[J]. Acta Phys. -Chim. Sin., 2000,16(10): 873-878
187. Feng Wen-Hui, Wang Bao-Shan, Wang Hui, Kong Fan-Ao.Reaction of C2H3+NO Studied by Time-Resolved Emission Spectroscopy[J]. Acta Phys. -Chim. Sin., 2000,16(09): 776-778
188. Zhong Shun-He, Gao Feng, Ye Xiu-Qiang, Xiao Xiu-Fen.Study on Laser Stimulated Surface Reaction of Methanol Oxidative Coupling[J]. Acta Phys. -Chim. Sin., 2000,16(07): 601-607
189. Zhong Shun-He, Li Han-Sehng, Wang Jian-Wei, Xiao Xiu-Fen.Cu-Ni/V2O5-SiO2 Catalyst for the Direct Synthesis of Dimethyl Carbonate from Carbon Dioxide and Methanol[J]. Acta Phys. -Chim. Sin., 2000,16(03): 226-231
190. Jiang De-En, Zhao Bi-Ying, Xie You-Chang.Thermal Decomposition Behavior of Mg(NO3)2 on γ-Al2O3 and Basicity of MgO/γ-Al2O3[J]. Acta Phys. -Chim. Sin., 2000,16(02): 105-110
191. Shen Yu-Hua, Yang Zhan-Lan, Wu Jin-Guang.FT-IR for the Soluble Complexes of Bovine Serum Albumin Reacted with Calcium Hydroxyapatites[J]. Acta Phys. -Chim. Sin., 1999,15(12): 1064-1069
192. Cai Li-Rong, Sun Shi-Gang, Xia Sheng-Qing, Chen Fang, Zheng Ming-Sen, Chen Sheng-Pei, Lu Guo-Qiang.Particular Properties and Structure of Electrochemically Prepared Pd Film Nano-materials[J]. Acta Phys. -Chim. Sin., 1999,15(11): 1023-1029
193. Zhang Xiao-Gang, Li Yong-Wang, Zhong Bing, Peng Shao-Yi.Molecular Simulation in Hydrogen,Carbon Monoxide,Methanol and Hexane System[J]. Acta Phys. -Chim. Sin., 1999,15(11): 1036-1040
194. Liu Fu-Yi, Sheng Liu-Si, Qi Fei, Wu Guo-Hua, Gao Hui, Zhou Wei-Dong, Zhang Yun-Wu.Photoionization/Dissociation Channels and Mechanism of 1,2-Propylene Oxide[J]. Acta Phys. -Chim. Sin., 1999,15(09): 845-849
195. Deng Guo-Yang, Jes Henningsen.Quantitative Measurement of Adsorption of CH3OH on Commonly Used Mterials by Photoacoustic Method[J]. Acta Phys. -Chim. Sin., 1999,15(08): 764-768
196. Zhang Rong, Sun Yu-Han, Peng Shao-Yi.Effect of Surface Properties on the Catalytic Performance of Cu/SiO2 Catalysts[J]. Acta Phys. -Chim. Sin., 1999,15(07): 652-656
197. Yang Ji-Xin, Su Hong-Mei, Mao Wen-Tao, Zhong Jin-Xian, Kong Fan-Ao.TR-FTIR Study of the Reaction CH2(X3B1)+NO[J]. Acta Phys. -Chim. Sin., 1999,15(07): 643-646
198. Wu Gui-Sheng, Ren Jie, Sun Yu-Han.The Effect of Calcination Temperature on The Performance of Cu/ZrO2 and Cu-La2O3/ZrO2[J]. Acta Phys. -Chim. Sin., 1999,15(06): 564-567
199. Su Hong-Mei, Wu Cheng-Yin, Yang Ji-Xin, Zhong Jin-Xian, Kong Fan-Ao.Study of the Reaction CH2(X 3B1)+N2O[J]. Acta Phys. -Chim. Sin., 1999,15(06): 560-563
200. Zeng Hong-Xia, Li Zhi-Ping, Wang Han-Qing.Physical Chemistry Property of Water/TX-100/Hexanol/Octane Reverse Microemulsion[J]. Acta Phys. -Chim. Sin., 1999,15(06): 522-527
201. Wang Wen-Jun, Xu Jian-Hua, Lu Xing-Ze, Han Kui, Wang Gong-Ming, Wang Wen-Cheng, Cai Zhi-Gang, Yang Pei-Qing, Zhou Jian-Ying.Influence of the Interlayer Interactions on Aggregates in Organic Molecular Films[J]. Acta Phys. -Chim. Sin., 1999,15(05): 471-475
202. Zhao Qi, Han Xiu-Wen, Liu Xiu-Mei, Zhai Run-Sheng, Lin Li-Wu, Bao Xin-He, Guo Xin-Wen, Li Gang, Wang Xiang-Sheng.Studies on the TS-1 Zeolites Synthesized by Tetrapropylammonium Bromide as Template[J]. Acta Phys. -Chim. Sin., 1998,14(10): 906-912
203. Su Hong-Mei, Mao Wen-Tao, He Yong, Xu Li-Jin, Sun Ya, Kong Fan-Ao.Study of the Reaction CH2(X 3B1)+O2[J]. Acta Phys. -Chim. Sin., 1998,14(07): 597-600
204. Chen Hong-Bo, Yu La-Jia, Liao Dai-Wei, Lin Guo-Dong, Zhang Hong-Bin, Cai Qi-Rui.The Effect of Cr2O3 over Copper-based Catalysts for Methanol Synthesis[J]. Acta Phys. -Chim. Sin., 1998,14(06): 534-539
205. Zhao Qi, Han Xiu-Wen, Liu Xiu-Mei, Liu Xian-Chun, Zhai Run-Sheng, Bao Xin-He, Lin Li-Wu, Guo Xin-Wen, Zhang Fa-Zhi, Wang Xiang-Sheng.Structure of Highly Siliceous ZSM-5 Zeolites and Ti-ZSM-5 Zeolites Obtained by Indirect Synthesis[J]. Acta Phys. -Chim. Sin., 1998,14(04): 320-326
206. Wang Gui-Chang, Sun Yu-Han, Zhong Bing.Simulation to the Structure Sensitive of Cu Based catalyst for Methanol Synthesis[J]. Acta Phys. -Chim. Sin., 1998,14(04): 337-342
207. Li Ji-Tao, Zhang Wei-De, Qu Ze-Tang.Effect of CO on Methanol Synthesis from CO2 Hydrogenation[J]. Acta Phys. -Chim. Sin., 1998,14(03): 275-277
208. Zhong Chong-Min, Wang-De-Zheng, Takashi Ushikubo, Keisuke Wada.The Adsorption of Methanol,Water and Ethylene on a Niobium Oxide Thin Film[J]. Acta Phys. -Chim. Sin., 1998,14(03): 219-225
209. Yang Chun, Xu Qin-Hua.States and Assignment of Aluminium in Zeolite β[J]. Acta Phys. -Chim. Sin., 1998,14(02): 169-172
210. Zhang Xiao-Gang,Guo Xiang-Yun,Zhong Bing,Peng Shao-Yi.Monte Carlo Study of Methanol Clusters in Supercritical Cyclohexane System[J]. Acta Phys. -Chim. Sin., 1997,13(10): 898-903
211. Yang Chun,Wang Jian,Xu Qin-Hua.Basicities of Aluminated Zeolites β:An FTIR Study of Chemisorbed Pyrrole[J]. Acta Phys. -Chim. Sin., 1997,13(10): 957-960
212. Jiang Ming,Fu Yi-Lu.Characterization of Cu(I)Y Zeolites Prepared by Solid-state Ion Exchange[J]. Acta Phys. -Chim. Sin., 1997,13(09): 822-826
213. Li Li,He Tian-Jing,Wang Xiu-Yan,Liu Fan-Zhen.ESR Shift Induced by a Circularly Polarized Laser Beam and Antisymmetric Polarizability of [IrBr6]2-[J]. Acta Phys. -Chim. Sin., 1997,13(08): 685-692
214. Li Ji-Tao,Gao Li-Zhen,Zhang Wei-De.CO Adsorption and Hydrogenation on Crystalline YBa2Cu3Ox Thin Films[J]. Acta Phys. -Chim. Sin., 1997,13(08): 700-705
215. Hao Jing-Cheng,Wang Han-Qing,Ge Jin-Huan.Studies on the Sturctures of Microemulsions[J]. Acta Phys. -Chim. Sin., 1997,13(07): 593-597
216. Yang Hui,Li Chang-Zhi,Lu Tian-Hong,Xue Kuan-Hong,Sun Shi-Gang,Lu Guo-Qiang,Chen.Electrocatalytic Oxidation of Methanol on Polythionine Film Modified with Pt Microparticles[J]. Acta Phys. -Chim. Sin., 1997,13(06): 542-547
217. Yu Gang,Wang Kai-Xuan,Huang Jian-Bin,Zhao Bi-Ying.Low Frequency Raman Scattering of CdS Nanocrystallites Embedded in Silicate Glasses[J]. Acta Phys. -Chim. Sin., 1997,13(03): 230-235
218. Zhou Ya-Ping,Zhou Li.Study on the Adsorption Isotherms of Supercritical Hydrogen on Activatied Carbon[J]. Acta Phys. -Chim. Sin., 1997,13(02): 119-127
219. Wu Li-Ming,Li Zong-He,Liu Ruo-Zhuang.Theoretical Studies of Reaction F+H-C≡C-H→HF+C≡C-H[J]. Acta Phys. -Chim. Sin., 1996,12(11): 1018-1021
220. Li Xing-Lin,She Yi-Min,Guo Jun,Jiang Da-Zhen.XPS Study of the Interaction between Layers and Pillars of Layered Double Hydroxides Pillared with Heteroplyanion(II)[J]. Acta Phys. -Chim. Sin., 1996,12(10): 929-932
221. Xu Yong-Sheng,Han Kui,Xu Jian-Hua,Zhou Guang-Peng,Lu Xing-Ze.Studies on Azimuthal Orientation of Hemicyanine Molecules in LB Films[J]. Acta Phys. -Chim. Sin., 1996,12(09): 836-840
222. Han Kui,Xu Yong-Sheng,Ma Shi-Hong,Wang Guo-Yi,Luo Long-Gen,Lu Xing-Ze.Studies on Optical Nonlinear Anisotropy in Hemicyanine LB Multilayers[J]. Acta Phys. -Chim. Sin., 1996,12(07): 589-593
223. Cao Xiao-Yan,Li Zong-He,Liu Ruo-Zhuang.State-selected Reaction Studies on H2 + CN(n=0,1)→H + HCN[J]. Acta Phys. -Chim. Sin., 1996,12(03): 239-244
224. Zhang Suo-Jiang,Han Shi-Jun,Jin Yin-Dong.Molar Conductances of NaCl and KCl in Aqueous Methanol Mixtures at 298.15K[J]. Acta Phys. -Chim. Sin., 1996,12(01): 75-80
225. Ma Shi-Hong, Han Kui, Lu Xing-Ze, Wang Gong-Ming, Zheng Jia-Biao, Wang Wen-Cheng, Yao Zhong-Qi.Second Harmonic Generation from Langmuir-Blodgett Multilayers of Hemicyanine Derivative Interleaved with a Novel Spacer[J]. Acta Phys. -Chim. Sin., 1995,11(07): 650-653
226. Li Qing-Shui, Lin Yu-Qin, Liao Yuan-Yan.Studies on Catalytic Dehydrogenation of Methanol to Formaldehyde[J]. Acta Phys. -Chim. Sin., 1995,11(05): 442-446
227. Gao Zhi-Ming, Wu Tong-Hao, Peng Shao-Yi.Preparation and Structural Features of Ultrafine Spinel Magnesium Ferrites[J]. Acta Phys. -Chim. Sin., 1995,11(05): 395-400
228. Li Zong-He, Wu Jun-Nan, Liu Ruo-Zhuang, Ma Si-Yu, Feng Wen-Lin, Wang Mei-Tian.Dynamics and Product Vibrational State Distributions of the Reaction of the F-N=C→F-C≡N[J]. Acta Phys. -Chim. Sin., 1994,10(12): 1075-1080
229. Zhang Hong-Yu, Wei Yu.Head Group Effect on Molecular Dynamics Simulation of Labgmuir Monolayers[J]. Acta Phys. -Chim. Sin., 1994,10(11): 998-1003
230. Xiao Feng-Shou.Catalytic Performance in Ethylene Hydroformylation over Silica Supported Ru-Co Bimetallic Carbonyl Cluster-Derived Catalysts[J]. Acta Phys. -Chim. Sin., 1994,10(08): 724-727
231. Zhang Ya-Ming, Wang Yan-Ru, Shi Jun.Enthalpies of Dilution of Calcium Chloride in Aqueous Solution of Alcohols[J]. Acta Phys. -Chim. Sin., 1994,10(06): 555-559
232. Xu Bai-Qing, Yamaguchi Tsutomu, Tanabe Kozo, Liang Juan, Zheng Lu-Bin.Characterization of Acid-base Property of ZrO2 by Thermal Desorption: I. TPD Studies of Acid and Base Probes[J]. Acta Phys. -Chim. Sin., 1994,10(02): 107-113
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234. Li Qing-Ming; Fu Xiao-Yuan; Zhang Jing-Chang; Cao Wei-Liang.The Topological Characteristics of the Structures in the Vicinity of Transition State of HCN→HNC Isomerization[J]. Acta Phys. -Chim. Sin., 1992,8(06): 724-727
235. Wang Yi-Xuan; Zhao Jian-Ping; Dai Ming.Vapor-Liquid Equilibrium for Some Polar Aprotic Solvents with Methanol or 1,2-Dichloroethane[J]. Acta Phys. -Chim. Sin., 1992,8(05): 636-641
236. Zhou Zhi-Hua; Hu Wei-Dong; Lu Wen-Qing; Zhou Yi-Ming; Xue Kuan-Hong.Effect of Supporting Electrolyte on the Electrochemical Oxidation Pathways of Anhydrous Methanol at Gold Electrode[J]. Acta Phys. -Chim. Sin., 1992,8(05): 707-711
237. Sun Shi-Gang; Yang Dong-Fang; Tian Zhao-Wu.IN-SITU FTIR Studies on Adsorption and Oxidation of 1,2-Propanediol at a Platinum Electrode in Acid Solutions[J]. Acta Phys. -Chim. Sin., 1992,8(01): 59-63
238. Xu Bai-Qing; Liang Juan; Zheng Lu-Bin; Yamaguchi Tsutomua; Tanabe Kozoa.TPD and IR Studies on the Decomposition of Formic Acid Adsorbed on ZrO2[J]. Acta Phys. -Chim. Sin., 1991,7(06): 712-715
239. Su Wen-Duan; Zhou Shao-Min; Zhou Xiao-Lin.Statistical Mechanical Treatment of Adsorbed Monolayer at Electrode/Solution Interface III. The Structure of Inner Layer Formed at the Interface of Hg/(H2O+CH3OH) Solution[J]. Acta Phys. -Chim. Sin., 1991,7(04): 443-448
240. Liang Ying-Qiu; Jiang Yu-Tao; Tian Yong-Chi.FT-IR Spectroscopic Study on Langmuir-Blodgett Films of Stearic Acid[J]. Acta Phys. -Chim. Sin., 1991,7(01): 72-76
241. CHENG Xiao-Meng, LI Yu, CHEN Zong, LI Hong-Ping, ZHENG Xiao-Fang.A Comparative Study on the NMR Relaxation of Methanol in Sub- and Super-critical Mixtures of CO2 and Methanol[J]. Acta Phys. -Chim. Sin., 0,(): 0-0
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