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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2003,Vol.19>> Issue(10)>> 917-921     doi: 10.3866/PKU.WHXB20031007         中文摘要
Electrochemical Properties of Methanofullerenes
Ning Bin;Fan Lou-Zhen;Zheng Li-Ping;Cao Yong;Guo Zhi-Xin
Department of Chemistry, Beijing Normal University, Beijing 100875; Institute of Polymer Optoelectronic Materials and Devices, South China University of Technology, Guangzhou 510640;Institute of Chemistry, Chinese Academy of Sciences, Beijing 100080
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11 methanofullerenes have been investigated using cyclic voltammetry(CV) systematically and comparatively. The influence of the nature of groups introduced and chain length of substituents on the electron-accepting ability of methanofullerenes was observed. It was found that introducing electron-donating groups, such as alkyls, weaken the electron- accepting ability of C60 and make its first reduction wave shifted to more negative position. Introducing electron-withdrawing groups, such as carboxylic ester groups, compensate part of negative shift of the reduction wave due to the effect of the saturation of a fullerene double bond. It was also found that increasing the chain length of substituents would not obviously change the electron-accepting ability of C60. Furthermore, the split of reduction peaks of some methanofullerenes induced by electrochemical isomerization was explained.

Keywords: Fullerene   Methanofullerene   Cyclic voltammetry(CV)   Electrochemical properties   Isomerization  
Received: 2003-04-08 Accepted: 2003-06-02 Publication Date (Web): 2003-10-15
Corresponding Authors: Fan Lou-Zhen Email: lzfan@bnu.edu.cn


Cite this article: Ning Bin;Fan Lou-Zhen;Zheng Li-Ping;Cao Yong;Guo Zhi-Xin. Electrochemical Properties of Methanofullerenes[J]. Acta Phys. -Chim. Sin., 2003,19 (10): 917-921.    doi: 10.3866/PKU.WHXB20031007
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