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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2008,Vol.24>> Issue(04)>> 633-638     doi: 10.3866/PKU.WHXB20080415         中文摘要
Kinetic Behavior of Visible Light Photocatalytic Oxidation of Propylene for N-Doped Nano-TiO2
FENG Cai-Xia; WANG Yan; JIN Zhen-Sheng; ZHANG Shun-Li
College of Chemistry and Chemical Engineering, Henan University, Kaifeng 475004, Henan Province, P. R. China; Functional Material Research Center, Kaifeng University, Kaifeng 475004, Henan Province, P. R. China
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N-doped TiO2 (anatase) with high visible light photocatalytic activity was prepared by treating nanotube titanic acid (NTA) in NH3 flowat different temperatures. The crystalline structure of N-doped TiO2 determined by XRD was anatase when the treating temperature was higher than 400 ℃, however, a newphase (TiN) emerged at 700 ℃. The UV-Vis diffuse reflectance spectra (DRS) display that N-doped TiO2 has a continuous absorption at λ=400 nm. The photocatalytic activity of the N-doped TiO2 was determined by the photocatalytic oxidation of propylene under visible light irradiation. The highest photocatalytic activity was obtained for the catalyst treated at 600 ℃ in NH3 flow, which was active even under λ=500 nm, its kinetic behavior was accordant with the first order reaction formula.

Keywords: Nanotube titanic acid   Dioxide titanium   Nitrogen doped   Visible light photocatalysis  
Received: 2007-08-22 Accepted: 2007-12-26 Publication Date (Web): 2007-03-03
Corresponding Authors: JIN Zhen-Sheng Email: zhenshengjin@henu.edu.cn


Cite this article: FENG Cai-Xia; WANG Yan; JIN Zhen-Sheng; ZHANG Shun-Li. Kinetic Behavior of Visible Light Photocatalytic Oxidation of Propylene for N-Doped Nano-TiO2[J]. Acta Phys. -Chim. Sin., 2008,24 (04): 633-638.    doi: 10.3866/PKU.WHXB20080415
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