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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2004,Vol.20>> Issue(04)>> 424-427     doi: 10.3866/PKU.WHXB20040420         中文摘要
Study of Loaded Photocatalysts by Precious Metals on the Photocatalytic Reactivity
Zhang Jin-Long;Zhao Wen-Juan;Chen Hai-Jun;Xu Hua-Sheng;Chen Ai-Ping;Anpo Masa-Kazu
Institute of Fine Chemicals, East China University of Science and Technology, Shanghai 200237; 1Key Laboratory for Ultrofine Materials of Ministry of Education, East China University of Science and Technology, Shanghai 200237;Department of Applied Chemistry, Graduate School of Engineering, Osaka Prefecture University, 1-1 Gakuen-cho, Sakai,Osaka 599-8531, Japan
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The functional photocatalysts of high photocatalytic reactivity under visible light irradiation were prepared by loading precious metals on the vanadium ion implanted titanium oxide. The photocatalytic hydrolysis reaction of methylacetylene was studied under the visible light and solar beam. Those modified titanium oxides were used to construct conversion system of solar to chemical energy. It was found from experimental results that existence of precious metals on the V/TiO2 photocatalysts has the advantage of promotion of hydrogenation reaction in photocatalytic hydrolysis reaction of methylacetylene, and increase of propene product. The photocatalytic reactivities under visible light irradiation have a close relationship with oxidation states of the precious metals on titanium oxide and it is necessary for increasing photcatalytic reactivities that precious metals be reduced to 0 valence.

Keywords: Titanium oxide   Photocatalyst   Visible light   Precious metal loaded    Ion implant  
Received: 2003-09-12 Accepted: 2003-11-27 Publication Date (Web): 2004-04-15
Corresponding Authors: Zhang Jin-Long Email: jlzhang@ecust.edu.cn


Cite this article: Zhang Jin-Long;Zhao Wen-Juan;Chen Hai-Jun;Xu Hua-Sheng;Chen Ai-Ping;Anpo Masa-Kazu. Study of Loaded Photocatalysts by Precious Metals on the Photocatalytic Reactivity[J]. Acta Phys. -Chim. Sin., 2004,20 (04): 424-427.    doi: 10.3866/PKU.WHXB20040420
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90. GUO Qing-Lian, LI Ran, JIANG Feng-Lei, TU Jian-Cheng, LI Lin-Wei, LIU Yi.Characterization of the Interactions between Itraconazole and Human and Bovine Serum Albumins by a Spectroscopic Method[J]. Acta Phys. -Chim. Sin., 2009,25(10): 2147-2154
91. ZHANG Xiao-Yan, CUI Xiao-Li.Preparation and Photocatalytic Hydrogen Evolution Performance of C-N Co-doped Nano TiO2 Photocatalysts[J]. Acta Phys. -Chim. Sin., 2009,25(09): 1829-1834
92. DONG Xiang, TAO Jie, LI Ying-Ying, WANG Tao, ZHU Hong.Photoelectrochemical Properties of Three-Dimensional Network TiO2 Nanowire Film Prepared by Hydrothermal Method[J]. Acta Phys. -Chim. Sin., 2009,25(09): 1874-1882
93. DU Wei-Ping, LI Zhen, LENG Wen-Hua, XU Yi-Ming.Photocatalytic Reduction of Silver Ions on Ferric Oxides and Ferric Hydroxides[J]. Acta Phys. -Chim. Sin., 2009,25(08): 1530-1534
94. LI Chang-Yu, LIU Shou-Xin, MA Yue.Preparation of Visible-Light Response Cu-Cu2+1O Composites by a One-Step Hydrothermal Method[J]. Acta Phys. -Chim. Sin., 2009,25(08): 1555-1560
95. WANG Qi-Zhao, JIANG Li, LIU Hui, YUAN Jian, CHEN Ming-Xia, SHI Jian-Wei, SHANGGUAN Wen-Feng.Preparation and Characterization of Bi1-xGdxVO4 Photocatalyst and Its Application toWater Splitting[J]. Acta Phys. -Chim. Sin., 2009,25(08): 1703-1707
96. FENG Li-Li, ZHAO Wei, LIU Yang, JIAO Liang, LI Xing-Guo.Photocatalytic Degradation of Rhodamine B by Nanocrystalline TiO2 Loaded into MCM-41 Molecular Sieves[J]. Acta Phys. -Chim. Sin., 2009,25(07): 1347-1351
97. WEI Xian-Jun, LI Hui-Zhen, LI Jing, ZHOU Neng, TANG Hong-Wei.Vis-Spectrum Investigation of Thermo-Solvatochromic Behaviors of a Mixed Diamine and β-Diketonate Ligand Ni(II) Complex in Different Alcoholic Solutions[J]. Acta Phys. -Chim. Sin., 2009,25(07): 1449-1454
98. LEI Jian-Fei, LI Wei-Shan.Photoelectrocatalytic Performance of Arrayed Porous TiO2/Ti[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1173-1178
99. CHEN Wei, DONG Xin-Fa, CHEN Zhi-Shan, CHEN Sheng-Zhou, LIN Wei-Ming.Effect of Fe3+ Doping on Photocatalytic Activity of K2La2Ti3O10 for Water Decomposition to Hydrogen under Visible Light[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1107-1110
100. CHEN Qi-Feng, JIANG Dong, XU Yao, WU Dong, SUN Yu-Han.Visible Region Photocatalysis of Ce-Si/TiO2 Synthesized Using Sol-Gel-Hydrothermal Method[J]. Acta Phys. -Chim. Sin., 2009,25(04): 617-623
101. YU Zhi-Yong; ZHANG Wei; MA Ming; CUI Xiao-Li.Visible Light Photoelectrochemical Response of Nitrogen-Doped TiO2 Thin Films Prepared by Anodic Oxidation of Titanium Nitride Films[J]. Acta Phys. -Chim. Sin., 2009,25(01): 35-40
102. HU Yuan-Fang; LI Yue-Xiang; PENG Shao-Qin; LV Gong-Xuan; LI Shu-Ben.Photocatalytic Properties of Composite of SiO2 and Pt-Cd0.53Zn0.47S Solid Solutions[J]. Acta Phys. -Chim. Sin., 2008,24(11): 2071-2076
103. LI Xiao-Hui, LIU Shou-Xin.Characterization of Visible Light Response N-F Codoped TiO2 Photocatalyst Prepared by Acid Catalyzed Hydrolysis[J]. Acta Phys. -Chim. Sin., 2008,24(11): 2019-2024
104. YAO Hui-Jun; MO Dan; DUAN Jing-Lai; CHEN Yan-Feng; ZHANG Ling; LIU Jie; HOU Ming-Dong; SUN You-Mei.Preparation and Optical Properties of Gold Nanowire Arrays[J]. Acta Phys. -Chim. Sin., 2008,24(10): 1922-1926
105. CHANG Guo-Qing, ZHENG Xi, CHEN Ri-Yao, CHEN Xiao, CHEN Li-Qin, CHEN Zhen.Silver Nanoparticles Filling in TiO2 Hollow Nanofibers by Coaxial Electrospinning[J]. Acta Phys. -Chim. Sin., 2008,24(10): 1790-1796
106. CHEN Yu-Juan; HU Zhong-Hua; WANG Xiao-Jing; ZHAO Guo-Hua; LIU Ya-Fei; LIU Wei.Influence of Pore Size and Surface Area of Activated Carbon on the Performance of TiO2/AC Photocatalyst[J]. Acta Phys. -Chim. Sin., 2008,24(09): 1589-1596
107. LI Hai-Long; LUO Wu-Lin; CHEN Tao; TIAN Wen-Yu; SUN Mao; LI Chun; ZHU Di; LIU Ran-Ran; ZHAO Yu-Liang; LIU Chun-Li.Preparation and Photocatalytic Performance of Titania Nanotubes Loaded with Ag Nanoparticles[J]. Acta Phys. -Chim. Sin., 2008,24(08): 1383-1386
108. SHI Jian; LI Jun; CAI Yun-Fa.Fabrication of C, N-Codoped TiO2 Nanotube Photocatalysts with Visible Light Response[J]. Acta Phys. -Chim. Sin., 2008,24(07): 1283-1286
109. PAN Hai-Bo; WANG Fang; HUANG Jin-Ling; CHEN Nai-Sheng.Binding Characteristics of CoPc/SnO2 by In-situ Process and Photocatalytic Activity under Visible Light Irradiation[J]. Acta Phys. -Chim. Sin., 2008,24(06): 992-996
110. LUO Da-Chao; ZHANG Lan-Lan; LONG Hui-Jin; CHEN Yong-Mei; CAO Ya-An.Effect of Surface Modification by Ni2+ on Photocatalysis Activity of TiO2[J]. Acta Phys. -Chim. Sin., 2008,24(06): 1095-1099
111. FENG Cai-Xia; WANG Yan; JIN Zhen-Sheng; ZHANG Shun-Li.Kinetic Behavior of Visible Light Photocatalytic Oxidation of Propylene for N-Doped Nano-TiO2[J]. Acta Phys. -Chim. Sin., 2008,24(04): 633-638
112. WU Yu-Cheng; LIU Xiao-Lu; YE Min; XIE Ting; HUANG Xin-Min.Preparation and Properties of Carbon Nanotube-TiO2 Nanocomposites[J]. Acta Phys. -Chim. Sin., 2008,24(01): 97-102
113. ZHANG Jun-Jie; WU Min; QIN Yan-Tao; CHEN Rui; JIANG Yin-Hua; SUN Yue-Ming; YANG Zhao-Hui.Study on Zn(II) Tetracarboxy Phthalocyanine Doped TiO2 Electrode Using Electrochemical Impedance Spectrum[J]. Acta Phys. -Chim. Sin., 2008,24(01): 79-84
114. LI Jing; YUN Hong; LIN Chang-Jian.The Fe-doped TiO2 Nanotube Arrays as a Photoanode for Cathodic Protection of Stainless Steel[J]. Acta Phys. -Chim. Sin., 2007,23(12): 1886-1892
115. LIU Fu-Sheng; JI Ren; WU Min; SUN Yue-Ming.Hydrogen Production from Water Splitting Using Perylene Dye-Sensitized Pt/TiO2 Photocatalyst[J]. Acta Phys. -Chim. Sin., 2007,23(12): 1899-1904
116. CHEN Qi-Yuan; TONG Hai-Xia; YIN Zhou-Lan; HU Hui-Ping; LI Jie; LIU Liang-Liang.Preparation, Characterization and Photo-catalytic Behavior of TiO2 Catalysts with Oxygen Vacancies[J]. Acta Phys. -Chim. Sin., 2007,23(12): 1917-1921
117. MAN Yi; ZONG Rui-Long; ZHU Yong-Fa.Preparation and Photoelectrochemical Properties of Bi2MoO6 Films[J]. Acta Phys. -Chim. Sin., 2007,23(11): 1671-1676
118. ZHU Lei; CUI Xiao-Li; SHEN Jie; YANG Xi-Liang; ZHANG Zhuang-Jian.Visible Light Photoelectrochemical Response of Carbon-doped TiO2 Thin Films Prepared by DC Reactive Magnetron Sputtering[J]. Acta Phys. -Chim. Sin., 2007,23(11): 1662-1666
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