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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2011,Vol.27>> Issue(07)>> 1560-1566     doi: 10.3866/PKU.WHXB20110629         中文摘要
THERMODYNAMICS, KINETICS, AND STRUCTURAL CHEMISTRY
Influence of Methanol Addition on the Two Stage Combustion of a Dimethyl Ether/Air Mixture
ZHANG Li-Zhi1,2,3, YANG Hao-Lin1,2, ZHAO Dai-Qing1,2, JIANG Li-Qiao1,2
1. Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou 510640, P. R. China;
2. Key Laboratory of Renewable Energy and Gas Hydrate, Chinese Academy of Sciences, Guangzhou 510640, P. R. China;
3. Graduate University of Chinese Academy of Sciences, Beijing 100049, P. R. China
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A numerical study was performed to determine the effects of methanol addition on the two stage oxidation of a dimethyl ether/air mixture and on the production of formaldehyde and formic acid in a micro-flow reactor with a fixed temperature profile. The results indicate that methanol addition influences the reaction pathway for dimethyl ether oxidation at low velocity and this results in the low temperature reactions of dimethyl ether being suppressed. The low temperature reactions of dimethyl ether nearly vanish when methanol is added in the same mass fraction as dimethyl ether. The major cause of this is a decrease in the OH radical concentration. With increasing the amount of methanol the emission index of formic acid decreases sharply but the emission index of formaldehyde increases slightly at first, and then it decreases gradually. Therefore, appropriate methanol addition can result in the reduction of the emission indexes of formic acid and formaldehyde.



Keywords: Dimethyl ether   Methanol   Low-temperature oxidation   Non-regulated pollutants  
Received: 2011-01-19 Accepted: 2011-03-24 Publication Date (Web): 2011-05-09
Corresponding Authors: ZHAO Dai-Qing Email: zhaodq@ms.giec.ac.cn

Fund: The project was supported by the National Natural Science Foundation of China (50806079) and Natural Science Foundation of Guangdong Province, China (8151007006000014).

Cite this article: ZHANG Li-Zhi, YANG Hao-Lin, ZHAO Dai-Qing, JIANG Li-Qiao. Influence of Methanol Addition on the Two Stage Combustion of a Dimethyl Ether/Air Mixture[J]. Acta Phys. -Chim. Sin., 2011,27 (07): 1560-1566.    doi: 10.3866/PKU.WHXB20110629

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74. YANG Hong-Yan, GUO Pan-Pan, LI Wei-Shan.Electrodeposition Preparation and Activity of CO-Resistant Catalyst Pt-HxWO3 for Methanol Oxidation[J]. Acta Phys. -Chim. Sin., 2009,25(04): 719-723
75. WANG Jian-She, GUO Xun, SONG Cheng-Ying, WANG Liu-Cheng, ZHAO Jian-Hong, QIU Xin-Ping.Promoting Methanol Electro-Oxidation through Fabricating Pore Structure in Pt/CNTs Catalyst Layer by Dissolving Away Premixed La2O3 Particles[J]. Acta Phys. -Chim. Sin., 2009,25(04): 767-772
76. XU Lei; WU Shu-Jie; ZHANG Wen-Xiang; JIA Ming-Jun; LIU Gang.Vapour Phase ortho-Selective Alkylation of Phenol with Methanol over Fe-Zr Oxide Catalysts[J]. Acta Phys. -Chim. Sin., 2009,25(02): 242-246
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79. CHANG Xiao-Tu, WANG Jian-Ming, SHAO Hai-Bo, WANG Jun-Bo, ZENG Xiao-Xu, ZHANG Jian-Qing, CAO Chu-Nan.Corrosion and Anodic Behaviors of Pure Aluminumin a Novel Alkaline Electrolyte[J]. Acta Phys. -Chim. Sin., 2008,24(09): 1620-1624
80. ZHENG Bo; LI He-Xian; WANG Guo-Chang; LIU Kun; YUAN Wei; LI He; LIANG Bo.Supramolecular Complexation in Water-Methanol Mixtures[J]. Acta Phys. -Chim. Sin., 2008,24(08): 1503-1506
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