ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2011,Vol.27>> Issue(12)>> 2872-2880     doi: 10.3866/PKU.WHXB20112872         中文摘要
Highly Active Au/α-MnO2 Catalysts for the Low-Temperature Oxidation of Carbon Monoxide and Benzene
YE Qing, HUO Fei-Fei, YAN Li-Na, WANG Juan, CHENG Shui-Yuan, KANG Tian-Fang
College of Environmental and Energy Engineering, Beijing University of Technology, Beijing 100124, P. P. China
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α-MnO2-supported gold catalysts (xAu/α-MnO2, x=0-7 (corresponding to the Au loading (mass fraction) of 0-7%) were prepared by a deposition- precipitation method using urea as a precipitation agent and characterized by different techniques such as X-ray diffraction (XRD), N2 adsorption-desorption measurements, transmission electron microscopy (TEM), X-ray photoelectron spectroscopy (XPS), and H2 temperature-programmed reduction (TPR). The catalytic activities of the materials were evaluated for the oxidation of CO and benzene. The Au particle size was found to be related to the Au loading of the xAu/ α-MnO2 samples and increased with Au loading. XPS results showed that the mole ratios of O2-/(O22- or O-), Mn4+/Mn3+ and Au3+/Au0 increased upon the addition of Au. The loading of gold over α-MnO2 significantly modified the catalytic activities. The catalytic performance of xAu/α-MnO2 strongly depended on the Au loading, and 3Au/α-MnO2 gained the best activity at T90=80 °C and T90=20 °C for the catalytic oxidation of CO and benzene, respectively. The excellent performance of 3Au/α-MnO2 is associated with highly dispersed Au, good low-temperature reducibility, and a synergism at the interface between theAu and MnO2 nanodomains.

Keywords: &   alpha   -MnO2 supported gold catalyst   Low-temperature reducibility   Synergistic action   Carbon monoxide oxidation   Benzene combustion  
Received: 2011-06-13 Accepted: 2011-09-13 Publication Date (Web): 2011-09-29
Corresponding Authors: YE Qing Email:

Fund: The project was supported by the National Natural Science Foundation of China (20777005), Natural Science Foundation of Beijing, China (8082008) and Beijing Municipal Foundation for Excellent Person of Ability, China (20071D0501500210).

Cite this article: YE Qing, HUO Fei-Fei, YAN Li-Na, WANG Juan, CHENG Shui-Yuan, KANG Tian-Fang. Highly Active Au/α-MnO2 Catalysts for the Low-Temperature Oxidation of Carbon Monoxide and Benzene[J]. Acta Phys. -Chim. Sin., 2011,27 (12): 2872-2880.    doi: 10.3866/PKU.WHXB20112872
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71. YANG Zhi-Qiang, MAO Dong-Sen, WU Ren-Chun, YU Jun, WANG Qian.Preparation of CuO-Ce0.6Zr0.4O2 by Microwave Heating Decomposition and Its Catalytic Property for CO Oxidation[J]. Acta Phys. -Chim. Sin., 2011,27(05): 1163-1168
72. PENG Xu-Hong, ZHENG Pei-Zhu, MA Yuan-Ming, YIN Tian-Xiang, AN Xue-Qin, SHEN Wei-Guo.The Second Virial Coefficient and Droplet Interaction of AOT/Water/Toluene Microemulsion[J]. Acta Phys. -Chim. Sin., 2011,27(05): 1026-1030
73. SU Shu, HUANG Rong, ZHAO Liu-Bin, WU De-Yin, TIAN Zhong-Qun.Vibrational Spectroscopy Criteria to Determine α-Pyridyl Adsorbed on Transition Metal Surfaces[J]. Acta Phys. -Chim. Sin., 2011,27(04): 781-792
74. ZHANG Xiao-Hong, GUO Hong-Rui, JIAO Zhi, YAN Wei-Wei, RUAN Wen-Juan, ZHU Zhi-Ang.Weak Interactions in Asymmetric Porphyrin Systems[J]. Acta Phys. -Chim. Sin., 2011,27(04): 774-780
75. LIAO Rui-Jin, ZHU Meng-Zhao, ZHOU Xin, YANG Li-Jun, YAN Jia-Ming, SUN Cai-Xin.Molecular Dynamics Simulation of the Diffusion Behavior of Water Molecules in Oil and Cellulose Composite Media[J]. Acta Phys. -Chim. Sin., 2011,27(04): 815-824
76. CAO Yun-Zhu, WEI Dong-Ming, REN Dong-Xue, CHEN Chen, XING Yong-Heng, SHI Zhan.Design, Synthesis and Mimic Catalytic Activity of a Vanadium Haloperoxidase Conformation Model Molecule[J]. Acta Phys. -Chim. Sin., 2011,27(03): 539-546
77. HU Jian-Ping, WANG Jun, TANG Dian-Yong, FU Qin-Chao, ZHANG Yuan-Qin.Reaction Mechanisms of CO Oxidation Catalyzed by Binary Copper Group Cluster Anions[J]. Acta Phys. -Chim. Sin., 2011,27(02): 329-336
78. LIU Yan, WANG Fang-Fang, YU Chun-Yang, LIU Cui, Gong Li-Dong, YANG Zhong-Zhi.Structures and Binding Energies of Sr2+/Ba2+-Water Systems by Ab initio and ABEEM/MM Method[J]. Acta Phys. -Chim. Sin., 2011,27(02): 379-387
79. WANG Wan-Xia, HE Yun-Fei, SHANG Ya-Zhuo, LIU Hong-Lai.Interaction between the Gemini Surfactant (12-6-12) and DNA[J]. Acta Phys. -Chim. Sin., 2011,27(01): 156-162
80. ZHAO Fu-Zhen, ZENG Peng-Hui, JI Sheng-Fu, YANG Xiao, LI Cheng-Yue.Catalytic Combustion of Toluene over CuxCo1?x/Al2O3/FeCrAl Monolithic Catalysts[J]. Acta Phys. -Chim. Sin., 2010,26(12): 3285-3290
81. YANG Zhi-Qiang, MAO Dong-Sen, GUO Qiang-Sheng, GU Lei.Effect of Preparation Method on the Activity of CuO/CeO2-ZrO2 Catalysts for Low Temperature CO Oxidation[J]. Acta Phys. -Chim. Sin., 2010,26(12): 3278-3284
82. ZHAN Yong-Gong, CHEN Qi-Yuan, YIN Zhou-Lan, LI Li-Li, CAI Bing-Xin.Synthesis, Characterization and Surface Functionalization of Novel Spindle-Like α-Fe2O3 Nanocrystals[J]. Acta Phys. -Chim. Sin., 2010,26(11): 3113-3119
83. ZHANG Li-Qun, LI Hao-Ran.Progress of Investigations on Structures and Interactions of Ionic Liquids by Infrared Spectroscopy and Raman Spectroscopy[J]. Acta Phys. -Chim. Sin., 2010,26(11): 2877-2889
84. QIAO Hui, LI Xiao-Qin, XU Hai-Song, KONG Ling-Qiang, PENG Yu.Specificity of Cation-π Interactions in Typical Protein Folds[J]. Acta Phys. -Chim. Sin., 2010,26(10): 2828-2832
85. LIU Yu-Liang, YOU Cui-Rong, LI Yang, HE Tao, ZHANG Xiang-Qin, SUO Zhang-Huai.Preparation of Au@TiO2 Catalyst Using Escherichia Coil as the Template and Its Oxidation Reaction Activity toward CO[J]. Acta Phys. -Chim. Sin., 2010,26(09): 2455-2460
86. ZHU Yan, PANG Xian-Hong, YU Li.Heterotactic Enthalpy of the Interaction between Protein Model Compounds and Diols in Aqueous Solutions at 310.15 K[J]. Acta Phys. -Chim. Sin., 2010,26(08): 2103-2108
87. HUANG Yong-Qi, LIU Zhi-Rong.Intrinsically Disordered Proteins: the New[J]. Acta Phys. -Chim. Sin., 2010,26(08): 2061-2072
88. DANG Zheng, SONG Le-Xin.Powder X-Ray Diffraction Analyses for Molecule-Ion Adducts of β-Cyclodextrin with a Series of Inorganic Salts[J]. Acta Phys. -Chim. Sin., 2010,26(07): 1837-1841
89. CAO Xu-Long, LV Kai, CUI Xiao-Hong, SHI Jing, YUAN Shi-Ling.Interactions between Anionic Surfactants and Cations[J]. Acta Phys. -Chim. Sin., 2010,26(07): 1959-1964
90. CAO Hai, JIANG Jian, ZHU Xue-Feng, DUAN Peng-Fei, LIU Ming-Hua.Interfacial Assembly of Diethyl Ester Glutamic Acid Terminated Bolaamphiphile at the Air/Water Interface: Chiral Interaction and Morphology[J]. Acta Phys. -Chim. Sin., 2010,26(07): 1842-1846
91. AN Shen-Jing, GAN Li-Hua, CHEN Liu-Hua, LIU Ming-Xian, ZHU Da-Zhang, XU Zi-Jie, HAO Zhi-Xian, CHEN Long-Wu.Interaction between [1,1'-Binaphthalene]-2,2'-diols and a Solid Supported Bilayer Lipid Membrane[J]. Acta Phys. -Chim. Sin., 2010,26(07): 1847-1851
92. YANG Xiao-Jing, LIU Xi-Li, LOU Chun-Bo, OUYANG Qi.End Effects during the Binding of Protein to Linear DNA Fragments[J]. Acta Phys. -Chim. Sin., 2010,26(07): 2007-2014
93. BAI Hong-Jun, LAI Lu-Hua.Protein-Protein Interactions: Interface Analysis, Binding Free Energy Calculation and Interaction Design[J]. Acta Phys. -Chim. Sin., 2010,26(07): 1988-1997
94. YAO Wei, GUO Yang-Long, LU Guan-Zhong, GUO Yun, WANG Yan-Qin, ZHANG Zhi-Gang, HE Dan-Nong.Gas Phase Epoxidation of Propylene over a Modified Ag/α-Al2O3 Catalyst[J]. Acta Phys. -Chim. Sin., 2010,26(06): 1579-1584
95. LI Gan, LUO Wen-Hua, CHEN Hu-Chi.CO Adsorption on α-U(001) Surface[J]. Acta Phys. -Chim. Sin., 2010,26(05): 1378-1384
96. YIN Guo-Wei, WEI Wei, XU Jia, LI Zhi-Fen, WANG Bao-Huai, DU Wei-Hong.Interaction of Nickel(II) with Yeast Alcohol Dehydrogenase[J]. Acta Phys. -Chim. Sin., 2010,26(04): 1107-1112
97. CHEN Heng-Jie, TANG Hai-Yan, CHENG Xin-Lu, WANG Quan-Wu.Ground and Low-Lying Excited States of NaC Molecule[J]. Acta Phys. -Chim. Sin., 2010,26(03): 740-744
98. YANG Hui, HU Min, CHEN Hui-Bo, YANG Shi-Wei, WANG Jin-Ben.Molecular Aggregation Behavior in the Mixture of Amphiphilic Poly(amidoamine)-Based Dendrimer and Sodium Dodecyl Sulfate[J]. Acta Phys. -Chim. Sin., 2010,26(03): 626-630
99. WU Xu, QIAO Ying-Jie, HU Chang-Chao, YANG Hui, WANG Jin-Ben.Aggregation Behavior of Amphiphilic Statistical Polymers and Their Interactions with Nonionic Surfactants[J]. Acta Phys. -Chim. Sin., 2010,26(02): 324-330
100. WANG Hai-Ying, CHAI Li-Yuan, LV Chun-Xu.Surface Activity of a Mixed Aqueous Solution of Poly(6-dodecyl-2-(acrylamidomethoxy)-1,3,6,2-dioxaza borocane) and Sodium Dodecylbenzene Sulfonate[J]. Acta Phys. -Chim. Sin., 2010,26(01): 73-78
101. WANG Hui-Ping, BAI Fu-Quan, ZHENG Qing-Chuan, ZHAO Zeng-Xia, ZHAO Xiao-Jie, ZHANG Hong-Xing.Electronic Structures and Optical Properties of Indolocarbazole Isomers[J]. Acta Phys. -Chim. Sin., 2010,26(01): 115-119
102. MANG Chao-Yong, ZI Jun-Qing, ZHAO Xia, WU Ke-Chen.The Lowest Triplet Excited States of Ph3PAuXand Ph3AsAuX(X=Cl, Br)[J]. Acta Phys. -Chim. Sin., 2009,25(10): 2113-2117
103. LI Zhen-Quan, ZHANG Lei, YAN Feng, ZHANG Lu, ZHAO Sui, YU Jia-Yong.Surface Dilational Properties of N-Acyltaurate Amphiphiles with Aromatic Side Chains[J]. Acta Phys. -Chim. Sin., 2009,25(09): 1939-1944
104. YU Xian-Yong, PENG Hong-Liang, HUANG Hao-Wen, WANG Zhao-Xu, ZHENG Bai-Shu, LI Xiao-Fang, YI Ping-Gui, CHEN Zhong.NMR Studies on Interactions between Diperoxovanadate and 1-Ethyl-1H-Imidazole[J]. Acta Phys. -Chim. Sin., 2009,25(09): 1779-1784
105. WU Yang, ZHANG Tian-Tian, YU Ning.Interaction between 1-Ethyl-3-Methyl-Imidazolium Cation and Asparagine Anion[J]. Acta Phys. -Chim. Sin., 2009,25(08): 1689-1696
106. SHI Jie-Hua, XIAO Ke-Ke, LV Yuan-Yuan.Host-Guest Interactions of β-Cyclodextrin with Enantiomers of Ethyl α-Chloropropionates[J]. Acta Phys. -Chim. Sin., 2009,25(07): 1273-1278
107. HUANG Xiao-Xuan, XU Xuan.Ir-Hg Interactions and the Nature of Redox Reactions in Ir(CO)Cla(Ph2Ppy)2HgClb(HgCl2)c (a, b=1, 2|c=0, 1)[J]. Acta Phys. -Chim. Sin., 2009,25(07): 1362-1366
108. WANG Fang-Bin, PENG Yong, FAN Mei-Yi, LIU You-Nian, HUANG Ke-Long.Synthesis of Glutathionyl Ferrocene and Its Interaction with Bovine Serum Albumin[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1125-1130
109. DANG Zheng, SONG Le-Xin, PAN Shu-Zhen, WANG Mang.Preparation, Spectral Properties and Decomposition Behavior of a Novel β-Cyclodextrin and Sodium Arsenite Adduct Formed by Stirring[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1059-1064
110. ZHAO Xiao-Fang, HE Yun-Fei, SHANG Ya-Zhuo, HAN Xia, LIU Hong-Lai.Effect of Electrolytes and Ethanol on the Interaction between DNA and the Gemini Surfactant[J]. Acta Phys. -Chim. Sin., 2009,25(05): 853-858
111. XIAO Xiao-Yan, LU Ji-Qing, SU Xiao-Wen, GUO Ming, LUO Meng-Fei.PdO-CeO2 Composite Catalysts for Low Temperature CO Oxidation[J]. Acta Phys. -Chim. Sin., 2009,25(03): 561-566
112. LIU Yi-Liang, YANG Bin-Wei, JIANG Gang.Electronic Effects of Atomic Nitrogen on Carbon on the Ni(111) Surface[J]. Acta Phys. -Chim. Sin., 2009,25(03): 435-440
113. ZHU Yan-Yan; XU Gui-Ying.Investigation of Macromolecule/Surfactant Interaction by Interfacial Dilational Rheology Method[J]. Acta Phys. -Chim. Sin., 2009,25(01): 191-200
114. MA Miao-Rui, YANG Li-Juan, LIU Qian, LIU Hui, WEI Yu.Effect of Ferrihydrite Sub-microstructure on Its Reactivity[J]. Acta Phys. -Chim. Sin., 2008,24(12): 2282-2286
115. SHEN Xin-Chun, WANG Wen-Qing, GONG Yan, ZHANG Yan.Dynamical Spin Chirality and Magnetoelectric Effect of α-Glycine[J]. Acta Phys. -Chim. Sin., 2008,24(12): 2153-2158
116. YUAN Kun; LIU Yan-Zhi; ZHU Yuan-Cheng; ZHANG Ji.Hydrogen-Bonded Complex between Ozone and Thioperoxy Radical in Gas-Phase[J]. Acta Phys. -Chim. Sin., 2008,24(11): 2065-2070
117. LIU Yan-Zhi, HE Li-Hong, YUAN Kun, LV Ling-Ling, WANG Yun-Pu.Structures and Electronic Properties of HOCl…HCOCl Complexes[J]. Acta Phys. -Chim. Sin., 2008,24(09): 1625-1630
118. CHEN Zhi-Ping; GAO Bao-Jiao; YANG Xiao-Feng.Adsorption Mechanism of Bilirubin on Aminated Crosslinking Microspheres of PGMA[J]. Acta Phys. -Chim. Sin., 2008,24(08): 1417-1424
119. LIU Min; ZHU Lan-Ying; LI Bin; ZHAO Qiang; SUN De-Zhi; LIN Rui-Sen.Thermodynamics of Dilution of N,N-Dimethylformamide in Aqueous Sodium Chloride Solutions at Different Concentrations[J]. Acta Phys. -Chim. Sin., 2008,24(07): 1316-1320
120. WEN Li; LIN Zhong-Yu; ZHOU Jian-Zhang; GU Ping-Ying; FU Jin-Kun; LIN Zhong-Hua.Au/γ-Al2O3 Catalyst Prepared from Octanethiolate Monolayer Protected Au Nanoparticles for CO Oxidation[J]. Acta Phys. -Chim. Sin., 2008,24(04): 581-586
121. CAO Tuan-Wu; YANG Ji-Dong.Interaction between Malachite Green and Bovine Serum Albumin[J]. Acta Phys. -Chim. Sin., 2008,24(04): 715-719
122. YAN Hua; YANG Jian-Guo; LIANG Hua-Ding; PAN Fu-You; ZHAO Song-Lin; LI Jing-Jing.Interaction between Cinnamic Acid and Bovine Serum Albumin and the Influence of Alcohol[J]. Acta Phys. -Chim. Sin., 2008,24(03): 543-546
123. ZHAN Ying-Ying; CAI Guo-Hui; ZHENG Yong; SHEN Xiao-Nv; ZHENG Ying; WEI Ke-Mei.Synthesis of High Surface Area Silicon Carbide and Its Application in CO Oxidation Reaction[J]. Acta Phys. -Chim. Sin., 2008,24(01): 171-175
124. LI Qin-Yu; XU Xuan.Fe—Hg Interactions and 31P Chemical Shifts in [Fe(CO)3(PPh2R)2(HgCl2)] (R=pym, fur, py, thi)[J]. Acta Phys. -Chim. Sin., 2007,23(12): 1875-1880
125. ZHOU Ming; WANG Zheng-Wu; XU Zu-Min.Study on the Interaction between Two Identical Parallel Plates with Iteration Method in Functional Theory[J]. Acta Phys. -Chim. Sin., 2007,23(11): 1776-1780
126. YU Xian-Yong; LI Guo-Bin; ZHENG Bai-Shu; HUANG Hao-Wen; YI Ping-Gui; ZENG Yun-Long; CHEN Zhong.NMR Studies on Interactions between Diperoxovanadate and Imidazole-like Ligands[J]. Acta Phys. -Chim. Sin., 2007,23(11): 1765-1770
127. WANG Rui; YU Zhi-Wu.Validity and Reliability of Benesi-Hildebrand Method[J]. Acta Phys. -Chim. Sin., 2007,23(09): 1353-1359
128. ZHOU Tian-Hua; ZHAO Jian-Xi.Adsorption Kinetics of Asymmetric Gemini Surfactants at Air/Water Interface[J]. Acta Phys. -Chim. Sin., 2007,23(07): 1047-1052
129. YUAN Wei; LI He-Xian; WANG Ying; YANG Hai-Long; WANG Guo-Chang.Computer Simulation on Intermolecular Interaction of N-(1-naphthyl)-succinimide[J]. Acta Phys. -Chim. Sin., 2007,23(05): 630-634
130. ZHANG Zhong; XU Xuan; ZUO Xiao-Xi; LI Wei-Shan.Stabilizing Effect of Amine on SmallMolecules in Electrolyte of LithiumBatteries[J]. Acta Phys. -Chim. Sin., 2007,23(04): 526-530
131. JIANG Li-Ding;GAO Bao-Jiao;LI Gang.Interaction between Cationic Gemini Surfactant with Hydrophobically Associatied Polyacrylamide of a New Family[J]. Acta Phys. -Chim. Sin., 2007,23(03): 337-342
132. WANG Hai-Ying;LI Bin-Dong;HU An-Jun;LU Chun-Xu .Surface Activity of a Novel Borate Ester Surfmer and Its Interaction with LAS in Aqueous Solutions[J]. Acta Phys. -Chim. Sin., 2007,23(02): 253-257
133. YU Dan-Mei;CHEN Chang-Guo;SI Yu-Jun;ZHOU Shang-Qi;WANG Li.Study on the Electronic Structure of Doped Nickel Hydroxide Using the DV-Xα Method of Quantum Chemistry[J]. Acta Phys. -Chim. Sin., 2007,23(01): 27-31
134. ZHENG Wen-Qing;SUN De-Zhi;QU Xiu-Kui.Thermodynamic Properties of Dilution of Myo-inositol in Pure Water and Aqueous Sodium Halide Solutions[J]. Acta Phys. -Chim. Sin., 2006,22(10): 1277-1280
135. LI Yong-Qing;LI Jian;SONG Peng;MA Feng-Cai.The Differential Interference Angle of Λ-Related Quantum Interference of 1Π-state Diatom[J]. Acta Phys. -Chim. Sin., 2006,22(05): 602-607
136. LI Hui-Juan;JIANG Xiao-Yuan;ZHENG Xiao-Ming.Synthesis of TiO2/[[gamma]]r-Al2O3 and Effect of CuO Loading on NO Reduction[J]. Acta Phys. -Chim. Sin., 2006,22(05): 584-589
137. ZHAI Cui-Ping;WANG Jian-Ji;XUAN Xiao-Peng;WANG Han-Qing.NMR Study on the Interactions of Ionic Liquid with Acetone[J]. Acta Phys. -Chim. Sin., 2006,22(04): 456-459
138. WU Dan; XU Gui-ying.Study on Protein-Surfactant Interaction by Spectroscopic Methods[J]. Acta Phys. -Chim. Sin., 2006,22(02): 254-260
139. LI Ling; QIU Xiao-mei; SUN De-zhi; LIU Feng; DI You-ying; YIN Bao-lin.Dilution Enthalpies of D-mannitol and D-sorbitol in Aqueous Sodium Chloride Solution[J]. Acta Phys. -Chim. Sin., 2006,22(02): 215-220
140. GAO Bao-jiao; ZHANG Xin; LIU Qi-fa.Effect of Organic Electrolyte on Chloromethylation of Polystyrene in Micellar Catalytic System[J]. Acta Phys. -Chim. Sin., 2006,22(01): 86-91
141. WANG Wen-feng; ZHANG Yong-fan; LI Jun-qian.DFT Study on the Mechanism of Cheletropic Addition of SO2[J]. Acta Phys. -Chim. Sin., 2006,22(01): 82-85
142. MENG Xiang-jun.Theoretical Study on Structures and Properties of Dihydrated Zwitterionic Glycine Complexes[J]. Acta Phys. -Chim. Sin., 2006,22(01): 98-101
143. XU Li; WANG Xu; LIN Rui-sen.Volumetric Properties of L-Serine in n-propanol-Water Mixed Solvents at 298.15 K[J]. Acta Phys. -Chim. Sin., 2005,21(11): 1315-1318
144. GE Min; ZHAO Hong-wei; ZHANG Zeng-yan; WANG Wen-feng; YU Xiao-han; LI Wen-xin.Far-infrared Spectra of 2,2′-biphenol and 4,4′-biphenol Measured by Terahertz Time-Domain Spectroscopy[J]. Acta Phys. -Chim. Sin., 2005,21(09): 1063-1066
145. CAO Chen-zhong; GAO Shuo.A Novel Approach for Estimating the Enthalpies of Formation of Monosubstituted Alkanes RX in Liquid-phase[J]. Acta Phys. -Chim. Sin., 2005,21(09): 1028-1035
146. LIU Jing; XU Gui-ying; LIU Jun; YU Li; ZHANG Hong-lin; YU Xiu-fang.Interaction between Tween-20 and BSA[J]. Acta Phys. -Chim. Sin., 2005,21(08): 862-866
147. MA Yan-hua; JIANG Rong; ZHAO Jian-xi.Surface Adsorption and Micelle Formation of C9pPHCNa and C10TABr Mixed Aqueous Solutions[J]. Acta Phys. -Chim. Sin., 2005,21(08): 939-943
148. XU Gui-Ying; LUAN Yu-Xia; LIU Jing; YU Li.Study on Surfactant/Macromolecule Interaction by Static Fluorescence Technology[J]. Acta Phys. -Chim. Sin., 2005,21(05): 577-582
149. TIAN Na;CHEN Wei;SUN Shi-Gang.Spectroscopic Characterization and Electrocatalytic Properties of Core-Shell Au-Pt Nanoparticles[J]. Acta Phys. -Chim. Sin., 2005,21(01): 74-78
150. Dai Zhi-Hui;Ju Huang-Xian.Direct Electron Transfer of Protein Immobilized on Mesoporous Molecular Sieves Matrix[J]. Acta Phys. -Chim. Sin., 2004,20(10): 1262-1266
151. Han Ke-Li.Nonadiabatic Dynamics with Split-Operator Scheme on Multiple Potential Energy Surfaces[J]. Acta Phys. -Chim. Sin., 2004,20(08S): 1032-1036
152. Gao Ying;Lai Lu-Hua.Analysis of Protein-Protein Interface[J]. Acta Phys. -Chim. Sin., 2004,20(07): 676-679
153. Wang Shu-Rong;Wu Shi-Hua;Shi Juan;Zheng Xiu-Cheng;Huang Wei-Ping.Preparation and Catalytic Activity of Au/SnO2 for Low-temperature CO Oxidation[J]. Acta Phys. -Chim. Sin., 2004,20(04): 428-431
154. Zhou Bao-Xue;Cai Wei-Min;Zou Li-Zhuang.Thermodynamic Functions of Transfer of Naphthalene from Water to Water-t-butyl Alcohol Solutions[J]. Acta Phys. -Chim. Sin., 2003,19(09): 867-870
155. Li Wei;Qu Jun-Yan;Zhao Xin-Sheng.Ab initio Investigation on the Potential Energy Surface of [He3H][J]. Acta Phys. -Chim. Sin., 2003,19(08): 751-756
156. Zhang Min;Jin Zhen-Sheng;Wang Shou-Bin;Zhang Shun-Li;Zhang Zhi-Jun.The Photocatalytic Enhancement Effect of CO on Pd/TiO2[J]. Acta Phys. -Chim. Sin., 2003,19(02): 100-104
157. Luan Yu-Xia;Xu Gui-Ying;Chen Ai-Min.Applications of Surfactant-selective Membrane Electrode in the Study of the Interactions between Surfactants and Polymers[J]. Acta Phys. -Chim. Sin., 2003,19(02): 185-192
158. Li Shu-Qin;Sang Wen-Qiang;Lin Rui-Sen.Volumetric Properties of Serine in Glucose-water and Sucrose-water Mixed Solvents at 298.15 K[J]. Acta Phys. -Chim. Sin., 2002,18(12): 1110-1115
159. Yan Yun;Han Feng;Huang Jian-Bin;Li Zi-Chen;Ma Ji-Ming.The Study of Bolaamphiphile/SDS Mixed Systems by Applying the Regular Solution Theory[J]. Acta Phys. -Chim. Sin., 2002,18(09): 830-834
160. Li Shu-Qin;Lin Rui-Sen.The Dilution Enthalpies of Serine in Aqueous Sucrose Solutions at 298.15 K[J]. Acta Phys. -Chim. Sin., 2002,18(09): 825-829
161. Gao Ying;Wang Ren-Xiao;Lai Lu-Hua.New Method to Analyze Protein-protein Interaction Interface[J]. Acta Phys. -Chim. Sin., 2002,18(08): 676-679
162. Mei Ming-Hua;Yan Jing-Jing;Wu Shi-Kang.The pH Effect on the Fluorescence of Linear Poly-amino-compounds and the Recognition of Nucleoside Phosphates[J]. Acta Phys. -Chim. Sin., 2002,18(08): 686-691
163. Tan Jin-Zhi;Xiao He-Ming;Gong Xue-Dong;Li Jin-Shan.Comparison of DFT with Ab initio Method on the Study of Intermolecular Interaction of (CH3ONO2)2[J]. Acta Phys. -Chim. Sin., 2002,18(04): 307-314
164. Yang E;Zhou Li-Xin;Zhang Yong-Fan.Theoretical Study on the Interaction between β-D-ribose(RI) and Bivalent and Monovalent Cations[J]. Acta Phys. -Chim. Sin., 2002,18(03): 253-259
165. Yang Yong-Lai;Xu Heng-Yong;Li Wen-Zhao.Study on Carbon Deposition of CH4,C2H6 and C2H4 Cracking over Ni-based Catalysts[J]. Acta Phys. -Chim. Sin., 2001,17(09): 773-775
166. Shao Shuang;Lin Rui-Sen;Hu Xin-Gen;Fang Wen-Jun;Ying Xiao-Hong.Enthalpic Interactions of Some Amino Acids with Monomethylurea in Aqueous Solutions at 298.15 K[J]. Acta Phys. -Chim. Sin., 2001,17(07): 645-650
167. Li Shu-Qin;Hu Xin-Gen;Lin Rui-Sen;Fang Wen-Jun;Sang Wen-Qiang;Liu Qing-Wang.Volumetric Properties of Glycine in Ethylene Glycolwater and Glycerolwater Mixtures at 298.15 K[J]. Acta Phys. -Chim. Sin., 2001,17(05): 400-405
168. Chen Chong-Jun;Luo Gen-Xiang;Jin Jun;Wang Hao-Ping.Approximate Expressions for Strong Interaction of Colloidal Particles with High Surface Potential[J]. Acta Phys. -Chim. Sin., 2001,17(04): 377-380
169. Hai Ming-Tan;Han Bu-Xing;Yan Hai-Ke.Investigation on the Interaction of Sodium Dodecyl Sulfate with Poly(Ethylene Oxide) by Electron Spin Resonance and UV Spectrum[J]. Acta Phys. -Chim. Sin., 2001,17(04): 338-342
170. Chen Yuan-Mei;Huang Yuan-He;Liu Ruo-Zhuang.Intermolecular Electron-phonon Coupling in One-dimensional C36 Polymers[J]. Acta Phys. -Chim. Sin., 2001,17(03): 196-200
171. Zhao Jian-Xi, Chen Xiao-Dong, Jiang Lin-Qin.Interaction of Binary Pluronic Block Molecules[J]. Acta Phys. -Chim. Sin., 2000,16(12): 1093-1102
172. Li Ming, Yang Hua-Quan.Lithiation Behavior of α-Fe2O3 in LiOH Electrolyte Solution[J]. Acta Phys. -Chim. Sin., 2000,16(08): 735-740
173. Jiang Hui-Jun, Yang Chun, Meng Zhong-Yue.Study on Ni-supported Bifunctional Basic Zeolite Catalyst[J]. Acta Phys. -Chim. Sin., 2000,16(04): 331-337
174. Jiang Ji-Sen, Gao Lian, Yang Xie-Long, Guo Jing-Kun.Preparation and Mössbauer Studies of α-Fe2O3 Nanoparticle[J]. Acta Phys. -Chim. Sin., 2000,16(04): 312-316
175. Li Gang, Lin Rui-Sen, Zong Han-Xing.Thermodynamics of Carboxyl Group's Protonation of α-amino Acids in Water-Ethanol Mixtures at 298.15K[J]. Acta Phys. -Chim. Sin., 2000,16(02): 188-192
176. Li Jin-Shan, Xiao He-Ming.lntermolecular lnteraction of (HN3)2[J]. Acta Phys. -Chim. Sin., 2000,16(01): 36-40
177. Shi Lei, Zhang Xiao-Gang, Zhang Xi-Feng, Yang Guan-Ying, Han Bu-Xing, Yan Hai-Ke.Study of Molecular lnteraction in Mixed Supercritical Fluids by Molecular Simulation and Partial Molar Volume Measurement[J]. Acta Phys. -Chim. Sin., 2000,16(01): 31-35
178. Shen Yu-Hua, Yang Zhan-Lan, Wu Jin-Guang.FT-IR for the Soluble Complexes of Bovine Serum Albumin Reacted with Calcium Hydroxyapatites[J]. Acta Phys. -Chim. Sin., 1999,15(12): 1064-1069
179. Gao Zuo-Ning, Li Hu-Lin.Spectroscopic and Electrochemical Studies of Phenylhydrazine-α-cyclodextrin lnclusion Complex and Its Adsorption Behaviors[J]. Acta Phys. -Chim. Sin., 1999,15(11): 1005-1010
180. Zhang Yu-Hong, Xiong Guo-Xing, Sheng Shi-Shan, Liu Sheng-Lin, Yang Wei-Shen.Interaction of NiO with γ-Al2O3 Supporter of NiO/γ-Al2O3 Catalysts[J]. Acta Phys. -Chim. Sin., 1999,15(08): 735-741
181. Yan Zhen-Ning, Cheng Qing-Tang, Wang Jian-Ji, Liu Da-Zhuang.The Volumetric Properties of Some α-Amino Acids in Aqueous Sodium Butyrate Solutions at 308.15K[J]. Acta Phys. -Chim. Sin., 1999,15(07): 662-667
182. Chen Tong, Li Wen-Zhao, Yu Chun-Ying.Investigation of the Interaction between NiO and Support,γ-Al2O3,for Oxidative Dehydrogenation of Ethane[J]. Acta Phys. -Chim. Sin., 1999,15(07): 613-618
183. Zeng Jian-Qing, Zhang Jing-Cheng, Zhong Bing.Monte Carlo Simulation of CO Oxidation Reaction on Fractal Surface[J]. Acta Phys. -Chim. Sin., 1999,15(06): 555-559
184. Zhou Ping, OU Yang-Zhi-Xun, Meng Qing-An.The Second Sphere Interaction in the Supramolecular Complexes Studiey by 59Co Solid Static NMR[J]. Acta Phys. -Chim. Sin., 1999,15(06): 533-540
185. Chen Hong-Shan, Ji Sheng-Fu, Niu Jian-Zhong, Xie Bao-Han, Li Shu-Ben.Vibration Spectroscopy on Transformation of Amorphous Silica to α-cristobalite[J]. Acta Phys. -Chim. Sin., 1999,15(05): 454-457
186. Liu Ying-Jun, Zhang Ji-Jun, Li Neng, Lin Bing-Xiong.The Effect of CO2 on Catalytic Activity of Cu-Ce-O Complex Oxides for CO Oxidation[J]. Acta Phys. -Chim. Sin., 1999,15(02): 97-100
187. Zhang Ji-Jun, Liu Ying-Jun, Li Neng, Lin Bing-Xiong.Synergistic Effect between CuO and CeO2 for CO Oxidation[J]. Acta Phys. -Chim. Sin., 1999,15(01): 15-21
188. Jiang Yong-Cai, Wu Shi-Kang.A Study on the Interaction between Pyrazoline Derivatives and Solvents[J]. Acta Phys. -Chim. Sin., 1998,14(12): 1068-1072
189. Fu Jin-Kun, Liu Yue-Ying, Hu Rong-Zong, Zeng Jin-Long, Xu Pian-Pian, Lin Zhong-Yu, Yao Bing-Xin, Weng Cheng-Zhou.Preparation of Highly Dispersive Supported Gold Catalyst by Microbial Reduction Method[J]. Acta Phys. -Chim. Sin., 1998,14(09): 769-771
190. Bi Zhi-Chu, Neuman A W.Interaction between BSA and SDBS at Water-air Interface by ADSA Method[J]. Acta Phys. -Chim. Sin., 1998,14(07): 649-653
191. Ma Zhi, Qin Yong-Ning, Qi Xiao-Zhou, Liang Zhen-Cheng, He Fei.Studies on Prepartion and CO Oxidation Activity of LaSrBO4 Compound[J]. Acta Phys. -Chim. Sin., 1998,14(05): 453-457
192. Zhou Zhi-Fen, Lin Hua-Kuan, Li Su-Qi, Zhu Shou-Rong, Chen Rong-Ti.Study of Thermochemical Properties of Cu(II)-α,α'-bipyridyl-macrocyclic Dioxotetraamine Ternary Systems[J]. Acta Phys. -Chim. Sin., 1998,14(04): 343-348
193. Chen Shun-Qing, Yang Ya-Hong.The Fluorescence Studi E dified Polyelectrolytes[J]. Acta Phys. -Chim. Sin., 1998,14(04): 380-384
194. Zhou Ren-Xian, Chen Fang, Jiang Xiao-Yuan, Zheng Xiao-Ming.The Dispersed States of Manganese Species on Mn-O/ZrO2 Catalysts and its Influents on the Catalytic Performance[J]. Acta Phys. -Chim. Sin., 1998,14(02): 178-180
195. Qi Xue-Yong,Wang Ya-Juan,Yang Kong-Zhang.XRD Studies on the Interaction between CrO3 and NaY、NaM Zeolites[J]. Acta Phys. -Chim. Sin., 1997,13(10): 938-941
196. Wang Kai-Xuan,Yang Xia-Wan,Zhao Bi-Ying,Xie You-Chang,Sun Ping-Chuan,Men Ai-Ju.7Li MAS NMR Studies on LiCl/γ-Al2O3[J]. Acta Phys. -Chim. Sin., 1997,13(03): 196-199
197. Zhou Ren-Xian,Jiang Xiao-Yuan,Lv Guang-Lie,Zheng Xiao-Ming.Desorption of Surface Oxygen on Cu/ZrO2-γ-Al2O3 and its Influence on the Catalytic Performance[J]. Acta Phys. -Chim. Sin., 1997,13(02): 128-133
198. Zeng Jian-Qing,Zhang Jing-Cheng,Guo Xiang-Yun,Zhong Bing.The Influence of Diffusion on the First Order Phase Transition Point of CO Oxidation:Monte Carlo Simulation[J]. Acta Phys. -Chim. Sin., 1997,13(02): 183-187
199. Chu Gao-Sheng,Zhang Zhi-Cheng,Zhang Man-Wei,Yao Si-De,Wang Wen-Feng,Lin Nian-Yun.Pulse Radiolysis of Phosphoryl and Non-phosphoryl Methionine in Aqueous Solution[J]. Acta Phys. -Chim. Sin., 1996,12(12): 1114-1118
200. Ye Gang,Li Guang-Hui,Zhang Ming-Hai.The Hydrothermal Behavior of Alumina IV. Rehydration of α-Al2O3[J]. Acta Phys. -Chim. Sin., 1996,12(12): 1098-1102
201. He Shao-Guang,Zhao Guo-Xi.Effect of Organic Ammonium Salts on the Surface Activity and Solubility of Fluorocarbon Surfactant[J]. Acta Phys. -Chim. Sin., 1996,12(11): 976-980
202. Zhu Chuan-Bao,Yan Ji-Min.Investigation on Characteristics of Interaction and Bonding Nature in C60 Cage of Endohedral Complexes X@C60[J]. Acta Phys. -Chim. Sin., 1996,12(09): 796-803
203. Zhang Ji-Shu,Zhang Wen-Xia,Wang Ze-Xin.Adsorption and Diffusion of Hydrogen Atom on Pd Loe Index Surfaces[J]. Acta Phys. -Chim. Sin., 1996,12(09): 773-779
204. Miao Ming-Ming,Sun Xian-Ru,Shi Jing-Min,Cheng Peng,Laio Dai-Zheng,Jiang Zong-Hui.Study on Tetraiodoterephthalato-bidged Cobalt(II) Binuclear Complexes[J]. Acta Phys. -Chim. Sin., 1996,12(07): 577-580
205. Xiong Ya,Huang Su-Qiu,Wu Ding-Quan,Qu Song-Sheng.Studies on the Interactions of Two Kinds of Water-Soluble Porphyrins with DNA[J]. Acta Phys. -Chim. Sin., 1996,12(06): 543-546
206. Li Xu-Yuan,Zhang Zi-Ping,Ma Jian-Tai,Zhu Zong-Zhen,Meng Yi-Min.The Catalytic Activity for CO Oxidation and Characterization of Perovskite-type Oxides Catalysts La1+X/2Sr1-x/2Co1-xCuxO3[J]. Acta Phys. -Chim. Sin., 1996,12(06): 502-507
207. Xu Zong-Rong,Gao Yan-Ling.Calculation of Vibrational Spectroscopy for Tri-atomic Molecules Using Interaction Model[J]. Acta Phys. -Chim. Sin., 1996,12(06): 555-559
208. Wei Yu,Liu Xiao-Lin,Zheng Xue-Zhong.Preparation of Ultrafine Monodispersed α-Fe2O3 Hydrosol[J]. Acta Phys. -Chim. Sin., 1996,12(06): 551-554
209. Zhou Ren-Xian,Chen Ping,Zheng Xiao-Ming,Chen Lin-Shen.The Lnteraction between Active Phase and Support and the TPR Characteristics on CuO/ZrO2 Catalyst[J]. Acta Phys. -Chim. Sin., 1996,12(05): 464-467
210. Zhu Xiao-Lei,Zhou Zhi-Hua,Xu Yong-Jin,Zhou Yao-Ming.Investigation on Dipole-dipole Interaction(II)[J]. Acta Phys. -Chim. Sin., 1996,12(04): 365-367
211. ZHOU Ren-Xian, WEI Jian-Gen, ZHENG Xiao-Ming, WU Hong-Li, LV Guang-Lie.Study on Phase Structure, Pore Structure and catalytic Property of Out-layer ZrO2 on Alumina Base[J]. Acta Phys. -Chim. Sin., 1995,11(12): 1097-1100
212. Ying Bai-Ning,Wu Guo-Xiang.Charge Transfer Complexation of N-substituted Phenothiazines with DDQ[J]. Acta Phys. -Chim. Sin., 1995,11(10): 937-940
213. Liu Han-Xing.Molecular Orbital Interactions in Cyclophanes[J]. Acta Phys. -Chim. Sin., 1995,11(10): 896-901
214. Liu Wen-Bin,Wu Yan-Ping,Wang Jian-Ji,Lu Jin-Suo.Viscosity of NaCl and KCl in Aqueous Sucrose Solutions[J]. Acta Phys. -Chim. Sin., 1995,11(07): 590-595
215. Li Xue-Gang,Zhao Guo-Xi.Molecular Interaction and Phase-separation in the Aqueous Solution of Anioniccationic Sufractant Mixture[J]. Acta Phys. -Chim. Sin., 1995,11(05): 450-453
216. Zhu Xiao-Lei, Zhou Zhi-Hua.Investigation on Dipole-dipole Interaction(I)[J]. Acta Phys. -Chim. Sin., 1995,11(05): 438-441
217. Yang Sheng-Yong, Xiao Shen-Xiu, Chen Tian-Lang.Studies on the Electronic Structure and Catalytic Properties of Heteropoly Anion (NiV13O38)7-[J]. Acta Phys. -Chim. Sin., 1994,10(12): 1071-1074
218. Chen Xue-Jun, Wang Yan, Li Yi-Gui.He-Ne Interatomic Potential from Inversion Scattering Theory[J]. Acta Phys. -Chim. Sin., 1994,10(12): 1099-1104
219. Liu Han-Xing, Li Bo-Fu, Sun Jia-Zhong.Study on Electronic Structure and d-d Excited Energies of Cr3+ Complexes[J]. Acta Phys. -Chim. Sin., 1994,10(11): 978-985
220. Lin Meng-Hai, Zhang Qian-Er.Exploration on Bonding Regularity for Mixed-metal Four-nuclear Clusters Pt2M2[J]. Acta Phys. -Chim. Sin., 1994,10(10): 887-891
221. Wang Ze-Xin, Zhang Ji-Shu, Yu Xiao-An, Hao Ce, Chen Zong-Qi.Effect of the Ni(510) Step Surface for the Dissociative Adsorption of Hydrogen Molecule[J]. Acta Phys. -Chim. Sin., 1994,10(10): 915-920
222. Xu Gui-Ying, Su Hong-Mei, Li Gan-Zuo, Liu Mu-Xin, Li Fang, Mao Hong-Zhi.The Interaction between Polyacrylamide and Mixed Surfactants[J]. Acta Phys. -Chim. Sin., 1994,10(10): 909-914
223. Chen Long-Wu, Gan Li-Hua, Yue Tian-Yi, Jiang Ji-Sen, Yang Xie-Long.Studies on the Pareparation of α-Fe2O3 Ultrafine Particles by Microemulsion Reaction Method[J]. Acta Phys. -Chim. Sin., 1994,10(08): 750-754
224. Zheng Shou-Rong, Qi Hai-Hua, Yan Qi-Jie, Fu Xian-Cai.A Study of the Interaction Between 12-Molybdophosphoric Acid and γ-Alumina[J]. Acta Phys. -Chim. Sin., 1994,10(06): 521-525
225. Yang Li-Ting, Chang Qing, Wang Feng-Li, Wang An-Zhou.Kinetics and Mechanism of Oxidation of α-alanine by Dihydroxydiperiodatonickelate (IV) Complex Ion[J]. Acta Phys. -Chim. Sin., 1994,10(04): 297-302
226. Xiao He-Ming, Li Yong-Fu, Qian Jian-Jun.A Study on Sensitivity and Conductivity of Alkali and Heavy Metal Azides[J]. Acta Phys. -Chim. Sin., 1994,10(03): 235-240
227. Lu Yan, Zhen Shao-Qiang, Lu Jin-Suo.The Enthalpic Interaction Parameters of Glycine with Some Alkali-Metal Chlorides[J]. Acta Phys. -Chim. Sin., 1994,10(03): 281-284
228. Ye Dai-Qi; Liang Hong; Huang Zhong-Tao.Study on the Interaction Between the Active Phase and Support on V2O5/TiO2 Catalyst[J]. Acta Phys. -Chim. Sin., 1993,9(04): 501-508
229. Zhao Dong-Yuan; Yang Ya-Shu; Guo Xie-Xian; Chen Heng-Rong; Xin Qin; Wang Guo-Jia.Preparation,Characterization and Surface Acidity of Hydroxy-Fe-Al Pillared Clays Containing Mixed-matal Complexes(II)[J]. Acta Phys. -Chim. Sin., 1993,9(03): 336-344
230. Huang Yuan-He; Liu Ruo-Zhuang.Temperature Dependence of Conductivity for Quasi-one Dimensional Organic Charge Transfer Crystal[J]. Acta Phys. -Chim. Sin., 1992,8(06): 728-731
231. Wang Dian-Xun; Wang Dong; Zhao Heng-Qi; Tang Qing; Xu Guang-Zhi.An Example of Lone Pair Orbital and Their Interaction——Gas Phase Ultravlolet Photoelctron Spectroscople Study of some Nitrogen Heterocyclle Compounds[J]. Acta Phys. -Chim. Sin., 1992,8(06): 809-813
232. Sun Xiang-Yu; Zhao Yao-Xing; Liang Xiao-Tian.Solvent Effect on Conformations of α,ω-Bis(4-Nitrophenoxy)-Alkanes[J]. Acta Phys. -Chim. Sin., 1992,8(05): 659-663
233. Zhu Yuan-Liang; Zhou Xi-Shun; Yang Fa-Wang; Lu Jin-Suo.Study on the Thermodynamic Properties of Hydrochloric Acid in Aqueous Solutions Containing Amino Acid I. Glycine+Hydrochloric acid+Water[J]. Acta Phys. -Chim. Sin., 1992,8(01): 132-135
234. Liang Wei-Gen; Yan Ji-Min; Hu Ri-Heng.On Intramolecular NON-Bonded Interaction of 1,1-Difluoroethane and 1,2-Difluoroethane[J]. Acta Phys. -Chim. Sin., 1992,8(01): 33-38
235. Ding Hui-Jun; Tian Bin; Zhao Guo-Xi.Interaction Between Cationic-Antonic and Zwitterionic Surfactant in Mixed Aqueous Solutions[J]. Acta Phys. -Chim. Sin., 1991,7(04): 413-419
236. Li Xue-Gang; Zhao Guo-Xi.Interactions of Surfactants with Metallic Cations[J]. Acta Phys. -Chim. Sin., 1991,7(03): 345-348
237. HOU Jing-Fei, YANG Yan-Lian, WANG Chen.Molecular Mechanisms of Interface Interactions between Nanomaterials and Proteins[J]. Acta Phys. -Chim. Sin., 0,(): 0-0
238. DENG Yu-Ling, YU Lu, HUANG Qiang.A Multi-Target Docking System of Human Kinome[J]. Acta Phys. -Chim. Sin., 0,(): 0-0
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