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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2012,Vol.28>> Issue(10)>> 2456-2464     doi: 10.3866/PKU.WHXB201209062         中文摘要
PHYSICAL CHEMISTRY OF MATERIALS
Controlled Growth of Graphene on Metal Substrates and STM Characterizations for Microscopic Morphologies
ZHANG Yan-Feng1,2, GAO Teng1, ZHANG-Yu2, LIU Zhong-Fan1
1 Center for Nanochemistry (CNC), College of Chemistry and Molecular Engineering, Peking University;
2 Department of Materials Science and Engineering, College of Engineering, Peking University, Beijing 100871
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Recently, chemical vapor deposition (CVD) has been widely applied to the large-scale synthesis of graphene on various metal substrates. As a powerful and direct imaging method, scanning tunneling microscopy (STM) has been used to study the microscopic morphologies of graphene on metal substrates, for the purpose of further optimizing the growth parameters. This review presents the recent progress in the controlled growth of graphene on Cu foils, Pt foils, and Ni substrates, as well as the research of the microscopic morphologies, defect states, and stacking orders of graphene. Monolayer growth of graphene on Cu and Pt foils follows a surface catalyzed growth mechanism, while bilayer graphene growth follows an epitaxial growth mechanism. After the formation of a bilayer, the corrugated substrate breaks the planar conjugated π bonds of graphene, inducing a binding configuration change from sp2 to sp3. Then, pristine wrinkles are introduced by the thermal expansion mismatch between graphene and the metal substrates. Finally, the roughness of graphene on the Pt foils is considerably less than that of graphene on Cu foils, and the multifaceted interweaving Pt substrate has almost no effect on the in-plane continuity of graphene.



Keywords: Chemical vapor deposition   Metal substrate   Graphene   Scanning tunneling microscope  
Received: 2012-07-19 Accepted: 2012-09-06 Publication Date (Web): 2012-09-06
Corresponding Authors: Email: yanfengzhang@pku.edu.cn; zfliu@pku.edu.cn

Fund: The project was supported by the National Natural Science Foundation of China (21073003) and The Ministry of Science and Technology of China (2011CB921903, 2011CB933003, 2012CB921404).

Cite this article: ZHANG Yan-Feng, GAO Teng, ZHANG-Yu, LIU Zhong-Fan. Controlled Growth of Graphene on Metal Substrates and STM Characterizations for Microscopic Morphologies[J]. Acta Phys. -Chim. Sin., 2012,28 (10): 2456-2464.    doi: 10.3866/PKU.WHXB201209062

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74. WU Hai-Fei, WU Ke, ZHANG Han-Jie, LIAO Qing, HE Pi-Mo.Oxidation and Oxygen Thermal Desorption Mechanism on Narrow-Gap IV-VI Semiconductor PbTe(111) Surface[J]. Acta Phys. -Chim. Sin., 2012,28(05): 1252-1256
75. LIU Bo, SUN Hong-Juan, PENG Tong-Jiang.Factor Group Analysis of Molecular Vibrational Modes of Graphene and Density Functional Calculations[J]. Acta Phys. -Chim. Sin., 2012,28(04): 799-804
76. JIN Yu, CHEN Hong-Yuan, CHEN Ming-Hai, LIU Ning, LI Qing-Wen.Carbon Nanotube/Polyaniline/Graphene Composite Paper and Its Electrochemical Capacitance Behaviors[J]. Acta Phys. -Chim. Sin., 2012,28(03): 609-614
77. XIE Peng-Yang, ZHUANG Gui-Lin, LÜ Yong-An, WANG Jian-Guo, LI Xiao-Nian.Enhanced Bonding between Noble Metal Adatoms and Graphene with Point Defects[J]. Acta Phys. -Chim. Sin., 2012,28(02): 331-337
78. XU Ke, SHEN Lai-Fa, MI Chang-Huan, ZHANG Xiao-Gang.Synthesis and Electrochemical Performance of Graphene Modified LiFePO4 Cathode Materials[J]. Acta Phys. -Chim. Sin., 2012,28(01): 105-110
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81. WANG Xi-Wen, JIANG Fang-Ting, SUO Quan-Ling, FANG Yu-Zhu, LU Yong.Self-supporting Macroscopic Carbon/Ni-Fiber Hybrid Electrodes Prepared by Catalytic Chemical Vapor Deposition Using Various Carbonaceous Compounds and Their Capacitive Deionization Performance[J]. Acta Phys. -Chim. Sin., 2011,27(11): 2605-2612
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83. DU Xiao-Qing, LI Hui-Qin, ZHU Qi-Rong, ZOU Zhi-Qiang, LIANG Qi.Growth and Nanotribological Properties of C60 Multilayer Films on Si(111)-7×7 Surface[J]. Acta Phys. -Chim. Sin., 2011,27(10): 2457-2461
84. LU Xiang-Jun, DOU Hui, YANG Su-Dong, HAO Liang, ZHANG Fang, ZHANG Xiao-Gang.Fabrication and Electrochemical Capacitive Behavior of Freestanding Graphene/Polyaniline Nanofibre Film[J]. Acta Phys. -Chim. Sin., 2011,27(10): 2333-2339
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