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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2013,Vol.29>> Issue(02)>> 305-310     doi: 10.3866/PKU.WHXB201211201         中文摘要
ELECTROCHEMISTRY AND NEW ENERGY
Synthesis and Electrochemical Characterization of RuO2·xH2O/Graphite Nanosheet Composite Array Electrodes for Supercapacitors
HU Ying-Ying, HU Zhong-Ai, ZHANG Ya-Jun, LU Ai-Lian, XU Huan, ZHANG Zi-Yu, YANG Yu-Ying, LI Li, WU Hong-Ying
Key Laboratory of Polymer Materials of Gansu Province, Key Laboratory of Eco-Environment-Related Polymer Materials of Ministry of Education, College of Chemistry and Chemical Engineering, Northwest Normal University, Lanzhou 730070, P.R. China
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We used electrochemical exfoliation to construct graphite nanosheet (GNS) arrays, in which the varying number of nanosheet layers were parallel to each other and perpendicular to the carbon substrate. Hydrous ruthenium oxide (RuO2·xH2O) was then loaded directly on the surface of nanosheets using cathodic reduction electrodeposition, resulting in the formation of RuO2·xH2O/GNS composite array electrodes. Electrochemical measurements showed that the composite array electrodes exhibited excellent capacitive behaviors, and achieved specific capacitance values as high as 4226 F·m-2 in the potential window up to 0.9 V, with a scan rate of 5 mV·s-1 in 0.5 mol·L-1 H2SO4 solution. The RuO2·xH2O/GNS composite array electrodes showed good cycling abilities, and maintained 94.18% of their maximum performance after 20000 cycles.



Keywords: Supercapacitor   Graphite nanosheet   RuO2   Electrodeposition   Array electrode  
Received: 2012-09-07 Accepted: 2012-11-19 Publication Date (Web): 2012-11-20
Corresponding Authors: Email: Zhongai@nwnu.edu.cn


Cite this article: HU Ying-Ying, HU Zhong-Ai, ZHANG Ya-Jun, LU Ai-Lian, XU Huan, ZHANG Zi-Yu, YANG Yu-Ying, LI Li, WU Hong-Ying. Synthesis and Electrochemical Characterization of RuO2·xH2O/Graphite Nanosheet Composite Array Electrodes for Supercapacitors[J]. Acta Phys. -Chim. Sin., 2013,29 (02): 305-310.    doi: 10.3866/PKU.WHXB201211201

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77. ZHOU Bao-Ping, YU Gang, OUYANG Yue-Jun, SI Wei-Wei, QIAO Li-Jie.Electrodeposition of Pd-Ag Alloy Nanoparticle Chains on Carbon Fibers and Their Hydrogen Sensing Properties[J]. Acta Phys. -Chim. Sin., 2010,26(01): 237-243
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80. FU Qing-Bin, GAO Bo, SU Ling-Hao, YUAN Chang-Zhou, LU Xiang-Jun, ZHANG Xiao-Gang.Preparation of Polypyrrole/Benzenesulfonic Functionalized Multi-Walled Carbon Nanotubes Induced by Hydrogen Bonding and Their Electrochemical Behavior[J]. Acta Phys. -Chim. Sin., 2009,25(11): 2199-2204
81. SUN Zhe, LIU Kai-Yu, ZHANG Hai-Feng, LI Ao-Sheng, XU Xiao-Cun.Study on Meso-C/MnO2 Asymmetric Supercapacitors[J]. Acta Phys. -Chim. Sin., 2009,25(10): 1991-1997
82. WANG Yan-Kun, ZHANG Jian-Min, LAN Meng.Temperature Effects on ZnO Film Electrodeposition[J]. Acta Phys. -Chim. Sin., 2009,25(10): 1998-2004
83. CAO Yin-Liang, WANG Feng, LIU Jing-Jun, WANG Jian-Jun, ZHANG Liang-Hu, QIN Shi-Yong.Electrochemical Preparation and Electrocatalytic Mechanisms of Ni-S Active Cathode for Hydrogen Evolution[J]. Acta Phys. -Chim. Sin., 2009,25(10): 1979-1984
84. JIANG Dong-Dong, FU Yan-Bao, MA Xiao-Hua.Fabrication and Characterization of Tin Nanorod Electrodes for Lithium Ion Rechargeable Batteries[J]. Acta Phys. -Chim. Sin., 2009,25(08): 1481-1484
85. TIAN Xi-Lin, TAO Jie, TAO Hai-Jun, BAO Zu-Guo, LI Zhuan-Li, ZHANG Yan-Yan, TANG Yu-Xin.Effect of Quenching on Properties of TiO2 Nanotube Arrays[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1111-1116
86. WANG Ming-Yong, WANG Zhi, GUO Zhan-Cheng.Regularity and Mechanism of Pb Electrodeposition Intensified by Super Gravity Field[J]. Acta Phys. -Chim. Sin., 2009,25(05): 883-889
87. YANG Fang-Zu, HUANG Ling, XU Shu-Kai, ZHOU Shao-Min.Preparation, Heat Treatment and Corrosion Behavior of Amorphous Ni-W/ZrO2 Composite Coating[J]. Acta Phys. -Chim. Sin., 2009,25(05): 864-868
88. LI Ning, GAO Cheng-Hui, YANG Su-Zhen.Crystallization Kinetics of Electrodeposited Amorphous/Nanocrystalline Ni81.32Mo18.68 Alloy Coating[J]. Acta Phys. -Chim. Sin., 2009,25(04): 735-740
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90. YANG Hong-Yan, GUO Pan-Pan, LI Wei-Shan.Electrodeposition Preparation and Activity of CO-Resistant Catalyst Pt-HxWO3 for Methanol Oxidation[J]. Acta Phys. -Chim. Sin., 2009,25(04): 719-723
91. DU Bing, JIANG Qi, ZHAO Xiao-Feng, LIN Sun-Zhong, MU Pei-Shan, ZHAO Yong.Preparation of PPy/CNTs Composite Based on the Electrostatic Absorption Effect[J]. Acta Phys. -Chim. Sin., 2009,25(03): 513-518
92. CHEN Li; ZHANG Xiao-Gang; YUAN Chang-Zhou; CHEN Sheng-Yao.Electrochemical Properties of Poly(3,4-ethylenedioxythiophene)/Manganese Oxide Synthesized by Interfacial Polymerization[J]. Acta Phys. -Chim. Sin., 2009,25(02): 304-308
93. YANG Pei-Xia; AN Mao-Zhong; SU Cai-Na; WANG Fu-Ping.Electrodeposition Behaviors of Pure Cobalt in Ionic Liquid[J]. Acta Phys. -Chim. Sin., 2008,24(11): 2032-2036
94. JIANG Qi; ZHANG Qian; DU Bing; ZHAO Xiao-Feng; ZHAO Yong.Preparation and Electrochemical Properties of CNTs-PANI Composite Material via Finite Field Polymerization[J]. Acta Phys. -Chim. Sin., 2008,24(09): 1719-1723
95. SHI Yan-Hua; MENG Hui-Min; SUN Dong-Bai; YU Hong-Ying; FU Hua-Rong.Manganese Oxide Coating Electrodes Prepared by Pulse Anodic Electrodeposition[J]. Acta Phys. -Chim. Sin., 2008,24(07): 1199-1206
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