ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2013,Vol.29>> Issue(04)>> 837-842     doi: 10.3866/PKU.WHXB201301241         中文摘要
Adsorption and Decomposition of NO2 on Ag/Pt(110) Bimetallic Surface
LI Jin-Bing1, JIANG Zhi-Quan2, HUANG Wei-Xin2
1 Yanshan Branch of SINOPEC Beijing Research Institute of Chemical Industry, SINOPEC, Beijing 102500, China;
2 Hefei National Laboratory for Physical Sciences at the Microscale, Chinese Academy of Sciences, Key Laboratory of Materials for Energy Conversion and Department of Chemical Physics, University of Science and Technology of China, Hefei 230026, Anhui, China
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The adsorption and decomposition of NO2 on Ag/Pt(110) bimetallic surfaces have been investigated by Auger electron spectroscopy (AES) and thermal desorption spectroscopy (TDS). At room temperature, NO2 undergoes dissociative chemisorption on Ag/Pt(110) bimetallic surfaces, forming chemisorbed NO(ads) and O(ads). Upon heating, NO(ads) undergoes both desorption from the surface and further decomposition. At 500 K, NO2 chemisorbs dissociatively on Ag/Pt(110) bimetallic surfaces, forming O(ads). Electron transfer occurs from Pt to Ag, therefore, the presence of Ag on Pt(110) surface weakens the binding energy of O(ads) with the surface and decreases the temperature required for the recombinative desorption of O(ads) from the surface. We observed the formation of a Ag/Pt(110) alloy structure that exhibits catalytic activity towards NO2 decomposition similar to that of Pt(110)-(1×2) but with a binding energy towards O(ads) much lower than that of Pt(110)-(1×2). Such a Ag/Pt(110) alloy structure may be active in catalyzing the direct decomposition of NOx at relatively low temperatures.

Keywords: Ag/Pt(110) bimetallic surface   NO2   Chemisorption   Decomposition   Promotion effect  
Received: 2012-11-28 Accepted: 2013-01-21 Publication Date (Web): 2013-01-24
Corresponding Authors: Email:;

Fund: The project was supported by the National Natural Science Foundation of China (11079033).

Cite this article: LI Jin-Bing, JIANG Zhi-Quan, HUANG Wei-Xin . Adsorption and Decomposition of NO2 on Ag/Pt(110) Bimetallic Surface[J]. Acta Phys. -Chim. Sin., 2013,29 (04): 837-842.    doi: 10.3866/PKU.WHXB201301241

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71. WANG Shao-Xu; ZHAO Zhe; TAN Zhi-Cheng; LI Yan-Sheng; TONG Bo; SHI Quan; LI Ying.Thermal Stability and Kinetics of Thermal Decomposition for Protionamide[J]. Acta Phys. -Chim. Sin., 2007,23(09): 1459-1462
72. ZHANG Yu-Dong; LI Bin-Jie; XU Xiang-Min; LI De-Liang.Thermal Decomposition Kinetics of ZnSn(OH)6[J]. Acta Phys. -Chim. Sin., 2007,23(07): 1095-1098
73. LI Hong-Jian; CHEN Gang; LI Zhong-Hua; ZHOU Chao.Synthesis and Photocatalytic Decomposition of Water under Visible Light Irradiation of La2Ti2-xCoxO7 with Pyrochlore Structure[J]. Acta Phys. -Chim. Sin., 2007,23(05): 761-764
74. XUE Li; HE Hong.Catalytic Decomposition of N2O over Co-M(M=La, Ce, Fe, Mn, Cu, Cr) Composite Oxide Catalysts[J]. Acta Phys. -Chim. Sin., 2007,23(05): 664-670
75. TANG Yan-Jun; LI You-Ming; SONG Jing; PAN Zhi-Dong.Structural Characterization and Thermal Decomposition Behavior of Microsized and Nanosized CaCO3[J]. Acta Phys. -Chim. Sin., 2007,23(05): 717-722
76. TANG Wan-Jun; CHEN Dong-Hua.Thermal Decomposition Kinetics of Ferrous Oxalate Dihydrate[J]. Acta Phys. -Chim. Sin., 2007,23(04): 605-608
77. FANG Shu-Mei; OU Yan; LIN Jing-Dong; LIAO Dai-Wei.Preparation of Cu/Sr3Ti2O7 and Its Photocatalytic Activity of Watersplitting for Hydrogen Evolution[J]. Acta Phys. -Chim. Sin., 2007,23(04): 601-604
78. YIN Li-Song;CHEN Min-Tao;LI Ting;ZHOU Ke-Sheng;GAO Song-Hua.Preparation of Rhombic MgO Nanoflakes from Dolomites[J]. Acta Phys. -Chim. Sin., 2007,23(03): 433-437
79. TAO Yan-Xin;YU Jun-Jie;LIU Chang-Chun;HAO Zheng-Ping;ZHANG Ze-Peng .Study on N2O Catalytic Decomposition over Mixed Oxides Derived from Co-Mg/Al Hydrotalcite-like Compounds[J]. Acta Phys. -Chim. Sin., 2007,23(02): 162-168
80. GUO Jin-Yu;ZHANG Jian-Guo;ZHANG Tong-Lai;WU Rui-Feng;YU Wei.Thermal Decomposition Mechanisms of a Three-dimensional Framework Coordination Polymer [Cu(HCOO)2(H2O)2][J]. Acta Phys. -Chim. Sin., 2006,22(10): 1206-1211
81. WU Xin-Min;LIU Jian-Hua;LI Wei;QI Chuan-Song .Thermal Decomposition Kinetics of Complexes of Rare Earths (RE = Nd, Sm) with Amino Acid RE(Val)Cl3•6H2O[J]. Acta Phys. -Chim. Sin., 2006,22(08): 942-946
82. HU Ji-Ming;HOU Yan-Yuan;WANG Xiao-Mei;ZHANG Jian-Qing;CAO Chun-Nan .Effect of Calcination Procedure on the Electrocatalytic Activities of Ti/IrO2 Electrodes in Acidic Aqueous Solution[J]. Acta Phys. -Chim. Sin., 2006,22(08): 1010-1014
83. ZOU Ji-Jun;LIU Chang-Jun.Preparation of NiO/SrTiO3 with Cold Plasma Treatment for PhotocatalyticWater Splitting[J]. Acta Phys. -Chim. Sin., 2006,22(08): 926-931
84. SUN Yuan-Hua;ZHANG Tong-Lai;ZHANG Jian-Guo;YANG Li;QIAO Xiao-Jing.Kinetics of Flash Pyrolysis of [Co(CHZ3](ClO42 and [Ni(CHZ)3](ClO4)2[J]. Acta Phys. -Chim. Sin., 2006,22(06): 649-652
85. ZHANG Xue-Hong;TANG Xing-Hua;CHENG Xin-Sun.Synthesis and Application of Ce-doped Mesoporous TiO2[J]. Acta Phys. -Chim. Sin., 2006,22(05): 532-537
86. YUAN Jun; DENG Ming-jin; AI Jun; XIE Xiao-lin; ZHENG Qi-xin.Non-isothermal Decomposition Kinetics of Poly(3-hydroxybutyrate-co-3-hydroxyvalerate)[J]. Acta Phys. -Chim. Sin., 2005,21(09): 988-992
87. YUE Lin-hai; JIN Da-lai; LU De-yi; XU Zhu-de.The Non-isothermal Kinetic Analysis of Thermal Decomposition of Mg(OH)2[J]. Acta Phys. -Chim. Sin., 2005,21(07): 752-757
88. QIAN Xin-Ming;LIU Li;FENG Chang-Gen.Calculating Apparent Activation Energy of Adiabatic Decomposition Process Using Pressure Data[J]. Acta Phys. -Chim. Sin., 2005,21(02): 134-138
89. LIU Chang-Jian;ZHANG Yi.Thermal Decomposition of NaNH4CrO4•2H2O[J]. Acta Phys. -Chim. Sin., 2005,21(02): 218-220
90. WANG Gui-Yun;WANG Yan-Ji;ZHAO Xin-Qiang;SONG Bao-Jun.Synthesis and Properties of CoO/SrTiO3 for the Photocatalytic Decomposition of Water[J]. Acta Phys. -Chim. Sin., 2005,21(01): 84-88
91. Wu Wang-Ting;Yang Rui;Hu Ting;Peng Ke;He Shui-Yang;Hu Rong-Zu.Thermochemistry of Salicylaldehyde-1H-benzotriazol Acetyl Hydrazone Complexes with RE (III)[J]. Acta Phys. -Chim. Sin., 2004,20(09): 1144-1149
92. Xu Xin;Lü Xin;Wang Nan-Qin;Zhang Qian-Er.Cluster Modeling of Chemisorption and Reactions on Metal Oxide Surfaces[J]. Acta Phys. -Chim. Sin., 2004,20(08S): 1045-1054
93. Yu Xue-Chun;Peng Hai-Lin;Zhang Ran;Zhang Ying-Ying;Liu Zhong-Fan.Influence of Decomposition Temperature on the Threshold Voltage for a Series of Charge Transfer Complexes[J]. Acta Phys. -Chim. Sin., 2004,20(06): 565-568
94. Liu Ji-Xin;Xie You-Chang.Single-wall Carbon Nanotubes Produced by Decomposition of CH4 on W-Fe-MgO Catalysts[J]. Acta Phys. -Chim. Sin., 2003,19(11): 1093-1096
95. Xu Run;Ma Zhong-Yi;Yang Cheng;Wei Wei;Sun Yu-Han.Effect of Manganese Promoter on the CuFeZrO2 Catalyst for Higher Alcohols Synthesis[J]. Acta Phys. -Chim. Sin., 2003,19(05): 423-427
96. Yuan Shi-Bin;Wei Zeng-Quan;Gao Qing-Xiang;Li Hai-Yan.Radiolysis of Amino Acid Derivatives Induced by the Irradiation of 110keV Fe Ion Beams[J]. Acta Phys. -Chim. Sin., 2002,18(11): 1033-1037
97. He Shui-Yang;Cao Wen-Kai;Hu Ting;Zhao Jian-She;Zhang Wei-Ping;Xue Gang-Lin;Hu Rong-Zu.Synthesis, Characterization and Thermochemical Properties of La(III) with Salicylaldehyde-1H- benzotriazol-1-aceylhydrazone[J]. Acta Phys. -Chim. Sin., 2002,18(10): 865-870
98. Liu Bei-Ping;Tan Zhi-Cheng;Nan Zhao-Dong;Liu Ping;Sun Li-Xian;Xu Fen.Calorimetric Study and Thermal Analysis of [Ho2(Ala)4(H2O)8]Cl6 and >;[ErY(Ala)4(H2O)8](ClO4)6[J]. Acta Phys. -Chim. Sin., 2002,18(06): 481-485
99. Gao Gai-Ling;Fang Yu;Wang Ming-Zhen;Hu Dao-Dao.Properties of Y2O3:Eu Nanocrystals Prepared by Thermodecomposition of Benzoic Acid[J]. Acta Phys. -Chim. Sin., 2002,18(05): 399-413
100. Yang Cheng;Dong Qing-Nian;Zhang Jing;Ren Jie;Sun Yu-Han;Xie Ya-Ning;Hu Tian-Dou.The Structural Effect of CeO2 and La2O3 Modified Pd/γ-Al2O3 Catalysts[J]. Acta Phys. -Chim. Sin., 2002,18(02): 170-174
101. Xue Jun;Zhu Jian-Hua;Shen Bin;Ma Li-Li.Investigation on Catalytic Decomposition of N-nitrosamines over Zeolites[J]. Acta Phys. -Chim. Sin., 2001,17(08): 696-701
102. Qian xin-Ming;Wang Yun;Feng Chang-Gen;Zheng Rao.Investigation of Thermal Decomposition of KClO3/CuO/S/Mg-Al/C6Cl6 System by Accelerating Rate Calorimeter[J]. Acta Phys. -Chim. Sin., 2001,17(01): 70-73
103. Zhang Jian-Guo, Zhang Tong-Lai.Synthesis,Structural Characterization and Thermal Decomposition Mechanism of {[Ag(ATO)2]ClO4}n[J]. Acta Phys. -Chim. Sin., 2000,16(12): 1110-1114
104. Liu Shi-Jun, Chen Qi-Yuan, Zhang Ping-Min.Thermal Decomposition of Monoclinic Ammonium Paratungstate[J]. Acta Phys. -Chim. Sin., 2000,16(11): 1048-1052
105. Lv Chun-Hua, Zhang Tong-Lai, Qiao Xiao-Jing, Cai Rui-Jiao, Yu Kai-Bei.Structure and Thermal Decomposition Mecharism of [Pb2(TNR)2(CHZ)2(H2O)2]4H2O[J]. Acta Phys. -Chim. Sin., 2000,16(05): 441-446
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107. Chen Jie-Hao, Wang Yan, Feng Wen-Lin.Mechanism of Pyrolysis of Pyruvic Acid and Benzoylformic Acid and Calculations of Thermal Rate Constants[J]. Acta Phys. -Chim. Sin., 1999,15(05): 431-435
108. Hong San-Guo, Peng Yi-Yuan, Zhu Shi-Lai, Wang Shen.Theoretical Study on the Thermolyses of ο-acetylcyclopentanone and ο-acetylcyclohexanone[J]. Acta Phys. -Chim. Sin., 1999,15(02): 186-189
109. Cai Yong, Zhu Xi-Wen, Yan Min, Chen Yong-Tai, Gao Ke-Lin.Chemical Reactions of Transition-metals with CO[J]. Acta Phys. -Chim. Sin., 1999,15(02): 162-166
110. Liu Shi-Jun, Chen Qi-Yuan, Zhang Ping-Min, Liu Min-Na.Study on Thermal Decomposition of Sodium Paratungstate Na10H2W12O42·27H2O[J]. Acta Phys. -Chim. Sin., 1998,14(09): 821-825
111. Xu Wen-Yuan, Liu Gou-Sheng, Peng Yi-Yuan, Hong San-Guo.AM1 Method Study of Thermolyses of Formacyl and Benzoyl Azides[J]. Acta Phys. -Chim. Sin., 1998,14(07): 669-672
112. Zhao Bang-Rong, Lu Chong-Xian, Ye Xue-Qi.Study on Unimolecular lon Decomposition Reaction Machanism of Acetanilide and p-aminoacetophenone[J]. Acta Phys. -Chim. Sin., 1998,14(05): 419-423
113. Luo Jin, Su Lian-Yong, Xie Lei, Zhou Jing, Zu Yan-Bing, Lin Zhong-Hua.Studies on Photoelectrochemical Behaviors of Nanocrystalline TiO2 Films[J]. Acta Phys. -Chim. Sin., 1998,14(04): 315-319
114. Zhang Ying, Xu Hai-Bo.CO Chemisorption on Disordered Binary Alloy[J]. Acta Phys. -Chim. Sin., 1998,14(01): 68-72
115. Lv Xin,Xu Xin,Wang Nan-Qin,Liao Meng-Sheng,Zhang Qian-Er.Cluster Modelling of CO Chemisorption on Cu/ZnO[J]. Acta Phys. -Chim. Sin., 1997,13(11): 1005-1009
116. Tian Sheng-Jun,Cheng Qing-Tang,Xi Guo-Xi,Lou Xiang-Dong,Li Jing-Hua.Preparation of Inclusion Complex of Benzyl Acetate with β-Cyclodextrin and Studies on its Thermal Dissociation[J]. Acta Phys. -Chim. Sin., 1997,13(05): 459-465
117. Zheng Wen-Xia,Wang Ze-Xin.Effect of the Ni(115) Step Surface for the Chemical Kinetics of Hydrogen Atom and Molecule on the Surface[J]. Acta Phys. -Chim. Sin., 1996,12(10): 910-915
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119. Yin Zhou-Lan.Study on the Kinetics of the Thermal Decomposition of Ammonium Molybdates[J]. Acta Phys. -Chim. Sin., 1996,12(02): 181-184
120. Cao Rong,Hou Zhen-Shan,Zhao Hong,He Di-Jing,Chen Wen-Hai.Propane Aromatization over Pt-Ga/HZSM-5 Catalyst[J]. Acta Phys. -Chim. Sin., 1996,12(02): 114-118
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124. Li Jun, Li Xin-Sheng, Zhou Jian-Lue, Xin Qin, Zhang Hui, Chen Yao-Qiang, Chen Yu.Co or/and NO Adsorption on Reduced Rh2/SiO2 and Rh2-V/SiO2 Catalysts Characterized by Infrared Spectroscopy[J]. Acta Phys. -Chim. Sin., 1995,11(05): 401-406
125. Hong San-Guo.Quantum Chemical Study of the Thermolysis of Chroman[J]. Acta Phys. -Chim. Sin., 1995,11(04): 297-301
126. Pang Xian-Jie, Zhong Bang-Ke.Studies on XRD and Thermal Decomposition of Tris [Tetrammine-μ-dihydroxo-cobaltium(III)] Cobaltium(III) Sulfate Ennea-Hydrate[J]. Acta Phys. -Chim. Sin., 1995,11(03): 262-265
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129. Hong San-Guo, Wang Shen.Study of the Thermolysis of RC(X)OC(O)CH3 Using MIVDO/3[J]. Acta Phys. -Chim. Sin., 1994,10(09): 779-784
130. Guo Xiang-Yun, Zhong Bing.Monte Carlo Simulation of N2O Decomposition[J]. Acta Phys. -Chim. Sin., 1994,10(08): 733-736
131. Hong San-Guo, Wang Shen.The Theoretical Study of the Thermolysis of Acetylacetone[J]. Acta Phys. -Chim. Sin., 1994,10(05): 424-427
132. Ruan Wen-Juan, Zhu Zhi-Ang, Huang Xiao-Qun, Chen Rong-Ti, Jiang Dong-Qing.Kinetic Study on Porphinatoiron(III) Catalyzing Decomposition of β-Carotene[J]. Acta Phys. -Chim. Sin., 1994,10(04): 312-318
133. Deng Jun-Zhuo; Wang Hong-Li.Adsoption History Dependence of the State of Chemisorbed CO on Fe(110)[J]. Acta Phys. -Chim. Sin., 1993,9(05): 589-593
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135. Wang Han-Zhang; Zhang De-Cheng; Guo Song-Shan; Bao Han-Bing; Yang Li; Lu Zhen-Rong.The Kinetics on Thermal Decomposition Reaction of Palladium Complexes with Thioether p-CH3C6H4SR[J]. Acta Phys. -Chim. Sin., 1993,9(01): 103-106
136. Shao Shu-Min; Xi Guang-Kang; Wang Jun-Rong; Li Sheng-Lin; Yang Xue-Zhu; Wang Jin-He; Zhou Zhi-Qiang; He Tian-Xi; Yu Bao-Xia.Activated Chemisorption of CH4 On Ni Surface and La Film[J]. Acta Phys. -Chim. Sin., 1992,8(06): 767-771
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138. JIN Cheng-Wei, WANG Ye, XU Su-Ling, ZHANG Jian-Jun.Synthesis, Crystal Structures and Thermochemical Properties of Ternary Rare Earth Complexes Based on 3,4-Diethoxybenzoic Acid and 2,2'-Bipyridine[J]. Acta Phys. -Chim. Sin., 0,(): 0-0
139. QIU Wei-Tao, HUANG Yong-Chao, WANG Zi-Long, XIAO Shuang, JI Hong-Bing, TONG Ye-Xiang.Effective Strategies towards High-Performance Photoanode for Photoelectrochemical Water Splitting[J]. Acta Phys. -Chim. Sin., 0,(): 0-0
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