类石墨烯二硫化钼及其在光电子器件上的应用

doi:10.3866/PKU.WHXB201302062

Abstract

Abstract:

Graphene-like molybdenum disulfide (MoS₂), which is composed of a monolayer or few layers of MoS₂, is a new two-dimensional (2D) layered material that has attracted considerable attention recently because of its unique structure and optical and electronic properties. Here we first review the methods used to synthesize graphene-like MoS₂. “Top-down” methods include micromechanical exfoliation, lithium-based intercalation and liquid exfoliation, while the“bottom-up”approaches covered are thermal decomposition and hydrothermal synthesis. We then discuss several methods used to characterize the 2D layered structures of MoS₂, such as atomic force microscopy (AFM), scanning electron microscopy (SEM), transmission electron microscopy (TEM), and Raman spectroscopy. We describe the UV-Vis absorption and photoluminescent properties of graphene-like MoS₂ and their related mechanisms. Finally, we summarize the application of graphene-like MoS₂ in various optoelectronic devices such as secondary batteries, field-effect transistors, sensors, organic light-emitting diodes, and memory. The application principles and research progress are discussed, followed by a summary and outlook for the research of this emerging 2D layered nanomaterial.

Key words: Graphene-like molybdenum disulfide, 2D layered material, Material synthesis, Structure characterization, Photophysical property, Optoelectronic device

MSC2000:

O644

TANG Peng, XIAO Jian-Jian, ZHENG Chao, WANG Shi, CHEN Run-Feng. Graphene-Like Molybdenum Disulfide and Its Application in Optoelectronic Devices[J].Acta Phys. -Chim. Sin., 2013, 29(04): 667-677.

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Graphene-Like Molybdenum Disulfide and Its Application in Optoelectronic Devices

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