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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2014,Vol.30>> Issue(9)>> 1659-1666     doi: 10.3866/PKU.WHXB201406162         中文摘要
ELECTROCHEMISTRY AND NEW ENERGY
Preparation and Electrochemical Properties of Functionalized Graphene/Polyaniline Composite Electrode Materials
WANG Li-Li, XING Rui-Guang, ZHANG Bang-Wen, HOU Yuan
School of Rare Earth, Inner Mongolia University of Science & Technology, Baotou 014010, Inner Mongolia Autonomous Region, P. R. China
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Octadecylamine functionalized graphene (ODA-G) was synthesized by the grafting of graphene oxide (GO) with ODA followed by reduction with hydrazine hydrate. Subsequently, ODA-G/polyaniline (PANI) composites were prepared using a facile solvent-blending procedure. ODA-G and ODA-G/PANI composites were characterized by Fourier transform infrared spectrometry (FTIR), X-ray diffraction (XRD), thermogravimetric analysis (TGA), Raman spectroscopy, and transmission electron microscopy (TEM). The electrochemical properties of the composites were measured based on cyclic voltammetry (CV), galvanostatic charge/discharge, and ac impedance spectroscopy. The results show that ODA-G as a support material provides additional electron transfer paths, as well as active sites, for the electrochemical redox reaction of PANI, which helps to increase its pseudocapacitance. A specific capacitance of 782 F·g-1 is obtained for 2%(w)ODA-G/PANI at a current density of 1.0 A·g-1, compared with 426 F·g-1 for PANI. Furthermore, ODA-G/PANI exhibits better stability than PANI.



Keywords: Functionalized graphene   Polyaniline   Supercapacitor   Electrochemical property   Solvent-blending  
Received: 2014-05-19 Accepted: 2014-06-16 Publication Date (Web): 2014-06-16
Corresponding Authors: ZHANG Bang-Wen Email: bangwenz@126.com

Fund: The project was supported by the National Natural Science Foundation of China (51164026), Inner Mongolia University of Science and Technology Innovation Fund, China (2012NCL007).

Cite this article: WANG Li-Li, XING Rui-Guang, ZHANG Bang-Wen, HOU Yuan. Preparation and Electrochemical Properties of Functionalized Graphene/Polyaniline Composite Electrode Materials[J]. Acta Phys. -Chim. Sin., 2014,30 (9): 1659-1666.    doi: 10.3866/PKU.WHXB201406162

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68. YAN Hui, ZHANG Huan, ZHANG Ding, ZHU Zhi, QI Lu.Hydrothermal Synthesis of Spherical Li4Ti5O12 as Anode Material for High Power Lithium-Ion Secondary Battery[J]. Acta Phys. -Chim. Sin., 2011,27(09): 2118-2122
69. PENG Tian-You, KE Ding-Ning, ZENG Peng, ZHANG Xiao-Hu, FAN Ke.Preparation and Photoelectrochemical Performance of BiVO4 Film Electrode[J]. Acta Phys. -Chim. Sin., 2011,27(09): 2160-2166
70. LI Zhao, XU Ju-Liang, LI Xu-Yan, GUO Li-Fang, LI Jin, JIANG Yi-Ming.Preparation of Manganese Dioxide for Electrodes of Supercapacitors Based on Duplex Stainless Steel[J]. Acta Phys. -Chim. Sin., 2011,27(06): 1424-1430
71. ZHOU Jin, LI Wen, XING Wei, ZHUO Shu-Ping.Capacitive Performance of Tunable Ordered Mesoporous Carbons in Organic and H2SO4 Electrolytes[J]. Acta Phys. -Chim. Sin., 2011,27(06): 1431-1438
72. MI Juan, WANG Yu-Ting, GAO Peng-Cheng, LI Wen-Cui.Effects of Thermal Treatment on the Electrochemical Behavior of Manganese Dioxide[J]. Acta Phys. -Chim. Sin., 2011,27(04): 893-899
73. YU Li-Qiu, CHEN Shu-Li, CHANG Sha, LI Yun-Hu, GAO Yin-Yi, WANG Gui-Ling CAO Dian-Xue.Supercapacitance of NiCo2O4 Nanowire Arrays Grown on Nickel Foam[J]. Acta Phys. -Chim. Sin., 2011,27(03): 615-619
74. LI Wen, ZHOU Jin, XING Wei, ZHUO Shu-Ping, Lü Yi-Min.Preparation of Microporous Carbon Using a Zeolite HY Template and Its Capacitive Performance[J]. Acta Phys. -Chim. Sin., 2011,27(03): 620-626
75. TIAN Ying, YAN Jing-Wang, XUE Rong, YI Bao-Lian.Influence of Electrolyte Concentration and Temperature on the Capacitance of Activated Carbon[J]. Acta Phys. -Chim. Sin., 2011,27(02): 479-485
76. ZHANG Hai-Jun, ZHANG Xiao-Gang, YUAN Chang-Zhou, GAO Bo, SUN Kang, FU Qing-Bin, LU Xiang-Jun, JIANG Jian-Chun.Preparation of Water Soluble Chitosan-Based Porous Carbon/NiO Composites and Their Electrochemical Capacitive Behavior[J]. Acta Phys. -Chim. Sin., 2011,27(02): 455-460
77. DENG An-Qiang, FAN Jing-Bo, QIAN Ke-Nong, LUO Yong-Chun.Effect of Heat Treatment on the Structure and Properties of La4MgNi19 Hydrogen Storage Electrode Alloys[J]. Acta Phys. -Chim. Sin., 2011,27(01): 103-107
78. ZHANG Lei-Yong, HE Shui-Jian, CHEN Shui-Liang, GUO Qiao-Hui, HOU Hao-Qing.Preparation and Electrochemical Properties of Polyaniline/Carbon Nanofiber Composite Materials[J]. Acta Phys. -Chim. Sin., 2010,26(12): 3181-3186
79. ZHANG Fang, YUAN Chang-Zhou, ZHANG Xiao-Gang, ZHANG Luo-Jiang, XU Ke.5-Sulfosalicylic Acid-Assisted Hydrothermal Synthesis and Supercapacitive Properties of Co-Ni Layered Double Hydroxides[J]. Acta Phys. -Chim. Sin., 2010,26(12): 3175-3180
80. ZHANG Xiao-Bo, CHEN Ming-Hai, ZHANG Xiao-Gang, LI Qing-Wen.Preparation of Porous Carbon Nanofibers by Electrospinning and Their Electrochemical Capacitive Behavior[J]. Acta Phys. -Chim. Sin., 2010,26(12): 3169-3174
81. ZHANG Qiao-Bao, FENG Zeng-Fang, HAN Nan-Nan, LIN Ling-Ling, ZHOU Jian-Zhang, LIN Zhong-Hua.Preparation and Photoeletrochemical Performance of CdS Quantum Dot Sensitized ZnO Nanorod Array Electrodes[J]. Acta Phys. -Chim. Sin., 2010,26(11): 2927-2934
82. LUO Yong-Chun, ZHANG Tie-Jun, WANG Duo, KANG Long.Influence of Ball-Milling on Hydrogen Storage and Electrochemical Properties of (Ti Cr)0.497V0.42Fe0.083/30%(w) (LaRMg)(NiCoAl)3.5 Alloy Electrodes[J]. Acta Phys. -Chim. Sin., 2010,26(09): 2397-2404
83. TIAN Ying, YAN Jing-Wang, LIU Xiao-Xue, XUE Rong, YI Bao-Lian.Electrochemical Capacitance of Composites with MnOx Loaded on the Surface of Activated Carbon Electrodes[J]. Acta Phys. -Chim. Sin., 2010,26(08): 2151-2157
84. YANG Su-Xia, LI Yuan, LIU Zhi-Ping, YANG Shu-Qin, HAN Shu-Min.Effect of Partial Substitution of Cu by Fe on the Phase Structure and Electrochemical Property of Low-Co AB5 Type Hydrogen Storage Alloys[J]. Acta Phys. -Chim. Sin., 2010,26(08): 2144-2150
85. LI Li-Min, LIU En-Hui, LI Jian, YANG Yan-Jing, SHEN Hai-Jie, HUANG Zheng-Zheng, XIANG Xiao-Xia.Polyaniline-Based Carbon for a Supercapacitor Electrode[J]. Acta Phys. -Chim. Sin., 2010,26(06): 1521-1526
86. JI Qian-Qian, GUO Pei-Zhi, ZHAO Xiu-Song.Preparation of Chitosan-Based Porous Carbons and Their Application as Electrode Materials for Supercapacitors[J]. Acta Phys. -Chim. Sin., 2010,26(05): 1254-1258
87. JIANG Lei, HUANG Hui, WANG Chun-Tao, ZHANG Wen-Kui, GAN Yong-Ping, TAO Xin-Yong.Photoelectrochromic Properties of TiO2-xNx/NiO Bilayer Thin Films[J]. Acta Phys. -Chim. Sin., 2010,26(02): 299-303
88. ZANG Yang, HAO Xiao-Gang, WANG Zhong-De, ZHANG Zhong-Lin, LIU Shi-Bin.Copolymerization and Capacitive Performance of Composite Carbon Nanotubes/Polyaniline/Nickel Hexacyanoferrate Films[J]. Acta Phys. -Chim. Sin., 2010,26(02): 291-298
89. WANG Wei-Kun, ZHANG Yong-Yong, WANG An-Bang, YU Zhong-Bao, HAN Min-Fang, YANG Yu-Sheng.Electrochemical Performance of 1,4,5,8-Tetrahydroxy-9,10-anthraquinone as Cathode Material in Lithium Batteries[J]. Acta Phys. -Chim. Sin., 2010,26(01): 47-50
90. LU Hua-Quan, WU Feng, SU Yue-Feng, LI Ning, CHEN Shi, BAO Li-Ying.Electrochemical Performance of LiNi0.5Mn0.5O2 as Cathode Material for Lithium-Ion Batteries Prepared by Oxalate Co-Precipitation Method[J]. Acta Phys. -Chim. Sin., 2010,26(01): 51-56
91. PANG Xu, MA Zheng-Qing, ZUO Lie.Sn Doped MnO2 Electrode Material for Supercapacitors[J]. Acta Phys. -Chim. Sin., 2009,25(12): 2433-2437
92. FU Qing-Bin, GAO Bo, SU Ling-Hao, YUAN Chang-Zhou, LU Xiang-Jun, ZHANG Xiao-Gang.Preparation of Polypyrrole/Benzenesulfonic Functionalized Multi-Walled Carbon Nanotubes Induced by Hydrogen Bonding and Their Electrochemical Behavior[J]. Acta Phys. -Chim. Sin., 2009,25(11): 2199-2204
93. SUN Zhe, LIU Kai-Yu, ZHANG Hai-Feng, LI Ao-Sheng, XU Xiao-Cun.Study on Meso-C/MnO2 Asymmetric Supercapacitors[J]. Acta Phys. -Chim. Sin., 2009,25(10): 1991-1997
94. SU Zhi, XU Mao-Wen, YE Shi-Hai, WANG Yong-Long.Doping of Layered LiMnO2 as Cathode Materials for Lithium-Ion Batteries and Their Electrochemical Properties[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1232-1238
95. GAO Hong-Quan, LAI Yan-Qing, ZHANG Zhi-An, LIU Ye-Xiang.Electrochemical Behaviors of New Lithium Salt LiBC2O4F2 in EC+DMC Solvents[J]. Acta Phys. -Chim. Sin., 2009,25(05): 905-910
96. JIANG Qi, ZHAO Xiao-Feng, HUANG Bin, DU Bing, ZHAO Yong.Effect of the Activated Carbon Reactivation on Its Electrochemical Capacitance[J]. Acta Phys. -Chim. Sin., 2009,25(04): 757-761
97. DU Bing, JIANG Qi, ZHAO Xiao-Feng, LIN Sun-Zhong, MU Pei-Shan, ZHAO Yong.Preparation of PPy/CNTs Composite Based on the Electrostatic Absorption Effect[J]. Acta Phys. -Chim. Sin., 2009,25(03): 513-518
98. CHEN Li; ZHANG Xiao-Gang; YUAN Chang-Zhou; CHEN Sheng-Yao.Electrochemical Properties of Poly(3,4-ethylenedioxythiophene)/Manganese Oxide Synthesized by Interfacial Polymerization[J]. Acta Phys. -Chim. Sin., 2009,25(02): 304-308
99. JIA Yan-Min; LIU Fei-Ye; XIAO Xue-Zhang; HANG Zhou-Ming; LEI Yong-Quan; CHEN Li-Xin.Microstructure and Electrochemical Properties of V2.1TiNi0.4Zr0.06Cu0.03M0.10 (M=Cr, Co, Fe, Nb, Ta) Hydrogen Storage Alloys[J]. Acta Phys. -Chim. Sin., 2009,25(02): 247-252
100. ZHANG Wei; CUI Xiao-Li; JIANG Zhi-Yu.Effect of Composite Modes on Photoelectrochemical Properties of MWCNTs/TiO2 Nanocomposite Films[J]. Acta Phys. -Chim. Sin., 2008,24(11): 1975-1980
101. SU Bi-Tao; ZUO Xian-Wei; HU Chang-Lin; LEI Zi-Qiang.Synthesis and Electromagnetic Properties of Polyaniline/CoFe2O4 Nanocomposite[J]. Acta Phys. -Chim. Sin., 2008,24(10): 1932-1936
102. LIU Fei-Ye; CHEN Li-Xin; LI Lu; JIA Yan-Min; LEI Yong-Quan.Microstructure and Electrochemical Properties of V2.1TiNi0.4Zr0.06Cux (x=0-0.12) Hydrogen Storage Alloys[J]. Acta Phys. -Chim. Sin., 2008,24(09): 1694-1698
103. JIANG Qi; ZHANG Qian; DU Bing; ZHAO Xiao-Feng; ZHAO Yong.Preparation and Electrochemical Properties of CNTs-PANI Composite Material via Finite Field Polymerization[J]. Acta Phys. -Chim. Sin., 2008,24(09): 1719-1723
104. WEN Qing; LIU Zhi-Min; CHEN Ye; LI Kai-Feng; ZHU Ning-Zheng.Electrochemical Performance of Microbial Fuel Cell with Air-Cathode[J]. Acta Phys. -Chim. Sin., 2008,24(06): 1063-1067
105. ZENG Wen-Wen; HUANG Ke-Long; YANG You-Ping; LIU Su-Qin; LIU Ren-Sheng.Solvothermal Synthesis and Capacitance Performance of Co3O4 with Different Morphologies[J]. Acta Phys. -Chim. Sin., 2008,24(02): 263-268
106. YANG Jing; LIU Ya-Fei; CHEN Xiao-Mei; HU Zhong-Hua; ZHAO Guo-Hua.Carbon Electrode Material with High Densities of Energy and Power[J]. Acta Phys. -Chim. Sin., 2008,24(01): 13-19
107. FAN Mao-Song; LEI Xiang-Li; WU Ning-Ning; QI Lu.Electrochemical Performance of LiMn2O4 Power Battery[J]. Acta Phys. -Chim. Sin., 2007,23(Supp): 36-39
108. YANG Jian-Jun; HUANG Jun-Jie; JIANG Zhi-Yu.Supercapacitance of MnO2 Thin Film Electrodes Prepared Using Jet Printing Method[J]. Acta Phys. -Chim. Sin., 2007,23(09): 1365-1369
109. WEI Ying-Jin; LI Xu; WANG Chun-Zhong; ZHAN Shi-Ying; CHEN Gang.Preparation and Electrochemical Properties of Cu Doped V2O5[J]. Acta Phys. -Chim. Sin., 2007,23(07): 1090-1094
110. LIU Su-Qin; GONG Ben-Li; HUANG Ke-Long; ZHANG Ge; LI Shi-Cai.Effect of Calcination Temperature on the Compositions and Electrochemical Performance of Products in the Synthesis of LiFePO4[J]. Acta Phys. -Chim. Sin., 2007,23(07): 1117-1122
111. WANG Jie; XU You-Long; SUN Xiao-Fei; XIAO Fang; MAO Sheng-Chun.Capacitance Properties of Porous Polypyrrole Thick Films Prepared Electrochemically by Multi-step Polymerization[J]. Acta Phys. -Chim. Sin., 2007,23(06): 877-882
112. LU Xin-Mei; WU Quan-Fu; MI Hong-Yu; ZHANG Xiao-Gang.Electrochemical Capacitance of Camphorsulfonic Acid Doped Polyaniline Microtubes Prepared at Low Temperature[J]. Acta Phys. -Chim. Sin., 2007,23(06): 820-824
113. GUO Xiao-Li; GUO Min; WANG Xin-Dong.Bienzymatic Glucose Biosensor Based on Graphite Electrode Modified with Nanofibrous Polyaniline[J]. Acta Phys. -Chim. Sin., 2007,23(04): 585-589
114. FENG Zhen-Zhen;NULI Yan-Na;YANG Jun.Conductive Sulfur-Containing Material/Polyaniline Composite for Cathode Material of Rechargeable Magnesium Batteries[J]. Acta Phys. -Chim. Sin., 2007,23(03): 327-331
115. WANG Jie;XU You-Long;CHEN Xi;DU Xian-Feng;LI Xi-Fei.Effect of Doping Ions on Electrochemical Capacitance Properties of Polypyrrole Films[J]. Acta Phys. -Chim. Sin., 2007,23(03): 299-304
116. YANG Zhao-Hui;ZHANG Mao-Feng;CAO Wei-Xiao.Self-assembly Films of Poly(4-diazosulfonate Styrene-co-4-vinylpyridine) with Polyaniline and Their Photoelectric Conversion Properties[J]. Acta Phys. -Chim. Sin., 2007,23(01): 1-5
117. TANG Zhi-Yuan;YU Ming-Yuan;XUE Jian-Jun;GAO Fei;CUI Yan;LI Liang-Dong.Electrochemical Properties and Synthesis of LiNi0.01Co0.01Mn1.98O4 by SAC Route for Lithium Secondary Battery[J]. Acta Phys. -Chim. Sin., 2007,23(01): 134-138
118. HUANG Ling;JIANG Hong-Hong;KE Fu-Sheng;FAN Xiao-Yong;ZHUANG Quan-Chao;YANG Fang-Zu;SUN Shi-Gang.Structure and Properties of Three-dimensional Reticular Sn-Co Alloy Electrodes as Anode Material for Lithium Batteries[J]. Acta Phys. -Chim. Sin., 2006,22(12): 1537-1541
119. XIE Jian;ZHAO Xin-Bing;YU Hong-Ming;QI Hao;CAO Gao-Shao;TU Jiang-Ping .Preparation, Characterization and Electrochemical Li-absorption/extraction Behaviors of Nanosized Co-Sn Intermetallic Compounds[J]. Acta Phys. -Chim. Sin., 2006,22(11): 1409-1412
120. LI Chang-Yu;LÜ Zhe;LIU Li-Li;LIU Zhi-Ming;SU Wen-Hui.Preparation and Performance Test of Ni-Fe/SDC Cell Anode[J]. Acta Phys. -Chim. Sin., 2006,22(10): 1181-1184
121. ZHUANG Da-Gao;ZHAO Xin-Bing;XIE Jian;TU Jian;ZHU Tie-Jun;CAO Gao-Shao.One-step Solid-state Synthesis and Electrochemical Performance of Nb-doped LiFePO4/C[J]. Acta Phys. -Chim. Sin., 2006,22(07): 840-844
122. TANG Ding-Guo;CI Yun-Xiang;QI Lu.Influence of Thermal Initiators on the Electrochemical Performances of Gel Polymer Electrolytes[J]. Acta Phys. -Chim. Sin., 2006,22(07): 826-830
123. CHEN Li-Xin;LI Lu;WANG Xin-Hua;DAI Fa-Bang;ZHENG Fang-Ping;LEI Yong-Quan.Phase Structures and Electrochemical Properties of V2.1TiNi0.4Zrx(x= 0~0.06) Hydrogen Storage Electrode Alloys*[J]. Acta Phys. -Chim. Sin., 2006,22(05): 523-527
124. YI Shuang-Ping;ZHANG Hai-Yan;PEI Lei;HU Shou-Le;ZENG Guo-Xun;CHEN Jin.Effect of CNTs Treated at Different Temperatures in Nitrogen Ambient on the Electrochemical Properties of CNTs-LaNi5 Electrodes[J]. Acta Phys. -Chim. Sin., 2006,22(04): 436-440
125. WEN Jing-bang; ZHOU Hai-hui; LI Song-lin; LUO Sheng-lian; CHEN Jin-hua; KUANG Ya-fei.Growth Process of Nano-fibrous Polyaniline Film on Stainless Steel[J]. Acta Phys. -Chim. Sin., 2006,22(01): 106-109
126. TANG Zhi-yuan; LU Xing-he; ZHANG Na.The Anion-cation Multiple Doping Effect of Spinel Cathode Materials on Electrochemical Speciality[J]. Acta Phys. -Chim. Sin., 2005,21(08): 934-938
127. LIU Chun-ling; WEN Yue-hua; CHENG Jie; GUO Quan-gui; CAO Gao-ping; LIU Lang; YANG Yu-sheng.Influence of Pore Structure of Phenolic Resin Based Activated Carbon Fibers on the Electrochemical Performance of Electrical Double-layer Capacitors[J]. Acta Phys. -Chim. Sin., 2005,21(07): 786-791
128. MA Hui-ru; GUAN Jian-guo; LU Guo-jun; YUAN Run-zhang.The Preparation and Characterization of PAn-PEG-PAn Rod-coil Triblock Copolymers[J]. Acta Phys. -Chim. Sin., 2005,21(06): 627-631
129. WU Mei-Yin; WANG Jian-Ming; ZHANG Jian-Qing; CAO Chu-Nan.Structure and Electrochemical Performance of Mn-substituted Nickel Hydroxide[J]. Acta Phys. -Chim. Sin., 2005,21(05): 523-527
130. XIAO Xue-Zhang; CHEN Chang-Pin; WANG Xin-Hua; CHEN Li-Xin; WANG Li; GAO Lin-Hui.Microstructure and Electrochemical Properties of Amorphous Mg-Fe-Ni Hydrogen Storage Electrode Material[J]. Acta Phys. -Chim. Sin., 2005,21(05): 565-568
131. CAI Cheng-Dong; ZHOU Jian-Zhang; QI Li; XI Yan-Yan; LAN Bi-Bo; WU Ling-Ling; LIN Zhong-Hua.Conductance of a Single Conducting Polyaniline Nanowire[J]. Acta Phys. -Chim. Sin., 2005,21(04): 343-346
132. YANG Hong-Sheng; ZHOU Xiao; ZHANG Qing-Wu.Electrochemical Performances of Supercapacitor with Polyaniline Particles with Hierarchy as Active Electrode Material[J]. Acta Phys. -Chim. Sin., 2005,21(04): 414-418
133. TAO Bin-Wu;LIU Jian-Hua;LI Song-Mei;ZHAO Liang.Electrochemical Properties of a V2O5/C Composite in Aqueous Solution Used for Zinc Secondary Battery[J]. Acta Phys. -Chim. Sin., 2005,21(03): 338-342
134. WANG Xiao-Feng; RUAN Dian-Bo; WANG Da-Zhi; LIANG Ji.Hybrid Electrochemical Supercapacitors Based on Polyaniline and Activated Carbon Electrodes[J]. Acta Phys. -Chim. Sin., 2005,21(03): 261-266
135. Wang Wei-Kun; Wang An-Bang; Cao Gao-Ping; Yang Yu-Sheng.Electrochemical Performance of a Novel Cathode Material Phenyl Polysulfide for Lithium Batteries[J]. Acta Phys. -Chim. Sin., 2004,20(12): 1440-1444
136. Chang Xiao-Yan;Wang Zhi-Xing;Li Xin-Hai;Kuang Qiong;Peng Wen-Jie;Guo Hua-Jun;Zhang Yun-He.Synthesis and Performance of LiMnPO4 Used as Cathode Material for Lithium Ion Batteries[J]. Acta Phys. -Chim. Sin., 2004,20(10): 1249-1252
137. Chen Hong;Chen Jin-Song;Zhou Hai-Hui;Jiao Shu-Qiang;Chen Jin-Hua;Kuang Ya-Fei.The Application of Nano-fibrous Polyaniline in Electrochemical Capacitor[J]. Acta Phys. -Chim. Sin., 2004,20(06): 593-597
138. Dong Ping;Zhou Jian-Zhang;Xi Yan-Yan;Cai Cheng-Dong;Zhang Yan;Zou Xu-Dong;Huang Huai-Guo;Wu Ling-Ling;Lin Zhong-Hua.The Growth Mechanism of Eletrosynthesized Polyaniline Nanotubules in Alumina Template[J]. Acta Phys. -Chim. Sin., 2004,20(05): 454-458
139. Jiang Qi;Lu Xiao-Ying;Zhao Yong;Yu Zuo-Long.Effect of Microstructure’s Change on Electrochemical Capacitance of Carbon Nanotubes[J]. Acta Phys. -Chim. Sin., 2004,20(05): 546-549
140. Liu Xian-Ming;Zhang Yi-He;Zhang Xiao-Gang;Fu Shao-Yun.The Supercapacitive Properties of Ni-Ru Oxide Composites[J]. Acta Phys. -Chim. Sin., 2004,20(04): 417-420
141. Deng Mei-Gen;Zhang Zhi-An;Hu Yong-Da;Wang Bin-Hua;Yang Bang-Chao.Effect of Activation and Surface Modification on the Properties of Carbon Nanotubes Supercapacitors[J]. Acta Phys. -Chim. Sin., 2004,20(04): 432-435
142. Zhou Hai-Hui;Jiao Shu-Qiang;Chen Jin-Hua;Wei Wan-Zhi;Kuang Ya-Fei.Electrocatalytic Oxidation of Methanol on Nano-fibular Polyaniline Electrode Modified with Pt Microparticles[J]. Acta Phys. -Chim. Sin., 2004,20(01): 9-14
143. Fang Kun;Li Shou-Ping;Tao Xue-Yu;Wang Qing-Lu;Mao Wei-Min;Wu Qi-Ye.Preparation by Dispersion Polymerization and Characterization of Soluble and Stable Colloidal Polyaniline Microparticles[J]. Acta Phys. -Chim. Sin., 2004,20(01): 103-106
144. Li Jian-Gang;Wan Chun-Rong;Yang Dong-Ping;Yang Zhang-Ping.Effect of Cell Temperature on the Electrochemical Reaction of LiNi3/8Co2/8Mn3/8O2[J]. Acta Phys. -Chim. Sin., 2003,19(11): 1030-1034
145. Feng Wei;Yi Wen-Hui;Wang Xiao-Gong;Wu Hong-Cai.Electrical and Optical Properties of PANI-C60 Composite Films[J]. Acta Phys. -Chim. Sin., 2003,19(09): 795-799
146. Liu Chen;Chen Feng-En;Zhang Jia-Xin;Shi Gao-Quan.Raman Spectroscopic Studies on Electrosynthesized Polyaniline Film[J]. Acta Phys. -Chim. Sin., 2003,19(09): 810-814
147. Zhuang Xin-Guo;Yang Yu-Sheng;Ji You-Ju;Yang Dong-Ping;Tang Zhi-Yuan.The Influence of Porous Structure of Activated Carbons Used as Supercapacitor Electrode Materials on Its Properties[J]. Acta Phys. -Chim. Sin., 2003,19(08): 689-694
148. Zhao Kai-Yuan;Wang Yu-Qing.Surface Complex Adsorption Wave of Cadmium Ion at Ultra-micro Disc-electrode Modified by Polyaniline[J]. Acta Phys. -Chim. Sin., 2003,19(08): 727-732
149. Mu Shao-Lin;Yang Yi-Fei;Tan Zhi-An.The Electrocatalytic Oxidation of Hydrogen Peroxide on Polyaniline Doped with Ferrocenesulfonic Acid[J]. Acta Phys. -Chim. Sin., 2003,19(07): 588-592
150. Wei Jian-Hong;Shi Jing;Guan Jian-Guo;Yuan Run-Zhang.Surface Modification of PAn Particles[J]. Acta Phys. -Chim. Sin., 2003,19(07): 657-660
151. Liao Chuan-Ping;Gu Ming-Yuan.Mechanism for the Reduction of Dichromate in the Polymerization of Aniline[J]. Acta Phys. -Chim. Sin., 2003,19(07): 580-583
152. Wang Xiao-Feng;Wang Da-Zhi;Liang Ji.Carbon Nanotube Capacitor Materials Loaded with Different Amounts of Ruthenium Oxide[J]. Acta Phys. -Chim. Sin., 2003,19(06): 509-513
153. Zhang Bao-Hong;Zhang Na.Research on Nanophase MnO2 for Electrochemical Supercapacitor[J]. Acta Phys. -Chim. Sin., 2003,19(03): 286-288
154. Chen Di-Zhao;Liang Yi-Zeng;Xu Cheng-Jian.Rank Analysis on Two-dimensional Kinetic Data and Its Related Application[J]. Acta Phys. -Chim. Sin., 2002,18(10): 924-929
155. Wei Jian-Hong;Guan Jian-Guo;Chen Wen-Yi;Yuan Run-Zhang.Preparation and Characteristics of Polyaniline - Barium Titanate Nanocomposite Particles[J]. Acta Phys. -Chim. Sin., 2002,18(07): 653-656
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158. Liao Chuan-Ping;Gu Ming-Yuan.Mixied-Potential for Autocatalytic Polymerization of Aniline[J]. Acta Phys. -Chim. Sin., 2001,17(10): 904-907
159. Kan Jin-Qing;Hou Jun-Hua;Mu Shao-Lin.Bioelectrochemical Characters of Doping-coating Polyanilineuricase Electrode[J]. Acta Phys. -Chim. Sin., 2001,17(01): 32-36
160. Mu Shao-Lin, Yang Yi-Fei.Polyaniline Used as An Electron Transfer Mediator for the Catalyzed Dehydrogenating Renction of Alcohol[J]. Acta Phys. -Chim. Sin., 2000,16(09): 830-834
161. Huo Li-Hua, Wang Dong-Mei, Zeng Guang-Fu, Xi Shi-Quan.Preparation and Properties of Conducting Polymer of Doped Polyaniline LB Film[J]. Acta Phys. -Chim. Sin., 2000,16(07): 632-635
162. Li Jian-Chang, Xue Zeng-Quan, Zhang Hao, Zeng Yan, Liu Wei-Min, Wu Quan-De.Chiral Fractal Patterns of TCNQ Thin Films Grown by Vacuum Evaporation[J]. Acta Phys. -Chim. Sin., 2000,16(07): 579-582
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