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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2016,Vol.32>> Issue(6)>> 1330-1346     doi: 10.3866/PKU.WHXB201603073         中文摘要
Advances in Cu2ZnSn(S,Se)4 Thin Film Solar Cells
ZHANG Xue1, HAN Yang1, CHAI Shuang-Zhi1, HU Nan-Tao1, YANG Zhi1, GENG Hui-Juan2, WEI Hao1
1 School of Electronic Information and Electrical Engineering, Shanghai Jiao Tong University, Shanghai 200240, P. R. China;
2 College of Physics and Electronic Engineering, Anyang Normal University, Anyang 455000, Henan Province, P. R. China
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CdTe and Cu(In,Ga)(S,Se)2 (CIGSSe) light absorber materials have dominated the research field of compound semiconductor solar cells. Despite the high power conversion efficiencies and technological advances of CdTe and CIGS photovoltaic technologies, certain issues, like rare earth constituent elements or toxic elements, limit their future upscaled applications. In recent years, Cu2ZnSn(S,Se)4 (CZTSSe) thin film solar cells have become research hotspots, drawing increased interest. With earth-abundant and environmentallybenign constituent elements, CZTSSe light absorber materials are widely regarded as the next-generation photovoltaic technology that can replace CdTe and CIGS as a promising candidate for terawatt-level power output. In this review, the synthesis, structure, and properties of CZTSSe materials will be discussed. This review will primarily demonstrate the developments and recent advances of different fabrication techniques and deposition methods, such as vacuum-based and solution-based deposition methods, covering their advantages and disadvantages. Recent developments in CZTSSe fabrication methods and CZTSSe nanocrystal preparation approaches will also be reviewed. Finally, some limitations on CZTSSe photovoltaic technology will be analyzed, and directions for improvement will be suggested, helping scientists to make future developments in this field.



Keywords: Cu2ZnSn(S,Se)4   Thin film   Solar cell   Preparation method   Research progress  
Received: 2016-01-18 Accepted: 2016-03-07 Publication Date (Web): 2016-03-07
Corresponding Authors: YANG Zhi, GENG Hui-Juan, WEI Hao Email: zhiyang@sjtu.edu.cn;ghjhou@126.com;haowei@sjtu.edu.cn


Cite this article: ZHANG Xue, HAN Yang, CHAI Shuang-Zhi, HU Nan-Tao, YANG Zhi, GENG Hui-Juan, WEI Hao. Advances in Cu2ZnSn(S,Se)4 Thin Film Solar Cells[J]. Acta Phys. -Chim. Sin., 2016,32 (6): 1330-1346.    doi: 10.3866/PKU.WHXB201603073

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94. NI Zhe-Ming, XU Qian, PAN Guo-Xiang, MAO Jiang-Hong.Theoretical Processing in Understanding the Structures and Properties of Layered Double Hydroxides[J]. Acta Phys. -Chim. Sin., 2009,25(04): 792-805
95. YUAN Jia-Guo; ZHANG Yu-Zhi; LE Jun; SONG Li-Xin; HU Xing-Fang.Spectrum Investigations of Chloro-Alkoxide Sol-Gel Nanostructured Tungsten Oxide Thin Films[J]. Acta Phys. -Chim. Sin., 2009,25(02): 267-272
96. SHI Cheng-Wu, GE Qian, LI Bing, TAO Li, LIU Qing-An.Influence of Additives on the Performance of Electrolytes in Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2008,24(12): 2327-2330
97. ZHANG Hong-Wei, ZHANG Zheng-Fu, LI Yang, YANG Xi-Hun, LIU Shuo.Structural Effects and Electrooxidation Activity of a Two-Dimensional Multilayer PtRu/PtNd Alloy Nanostructure Thin Film[J]. Acta Phys. -Chim. Sin., 2008,24(12): 2268-2274
98. GAO Cheng-Yao; CHANG Ming.Ta/BDD Film Electrode for Electrochemical Oxidation Nitrophenol[J]. Acta Phys. -Chim. Sin., 2008,24(11): 1988-1994
99. PEI Juan, LIANG Mao, CHEN Jun, TAO Zhan-Liang, XU Wei.Application of Triphenylamine-Based Sensitizers with Two Carboxylic Acid Groups to Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2008,24(11): 1950-1956
100. ZHAO Feng-Ming; SHEN Hai-Ping; CHEN Zhao-Yang; MA Chun-An.Electrocatalytic Reduction of Maleic Acid at Bundles of TiO2 Anodization Film[J]. Acta Phys. -Chim. Sin., 2008,24(11): 2139-2142
101. HUO Wei-Liang; LIU Qing-Feng; LIU Qian; ZHU Li-Hui; WANG Li.Application of Combinatorial Material Chip Method in Screening of Anticorrosion Zn-Al Alloy[J]. Acta Phys. -Chim. Sin., 2008,24(09): 1703-1708
102. WANG Shuo; LUO Chong; ZHAO Ying; XIONG Shao-Zhen.Al-Induced Crystallization of Polycrystalline Silicon Thin Films Based on Solution Method[J]. Acta Phys. -Chim. Sin., 2008,24(09): 1689-1693
103. HUANG Jun-Jie; JIANG Zhi-Yu.Electrochemical Performance of LiMn2O4 Thin Film Electrode Fabricated by Ink-Jet Printing Technique[J]. Acta Phys. -Chim. Sin., 2008,24(09): 1563-1567
104. ZHANG Hua; ZHOU Yong-Ning; WU Xiao-Jing; FU Zheng-Wen.Electrochemical Properties of CuF2 Films Fabricated by Pulsed Laser Deposition[J]. Acta Phys. -Chim. Sin., 2008,24(07): 1287-1291
105. AO Jian-Ping; SUN Guo-Zhong; YAN Li; KANG Feng; YANG Liang; HE Qing; ZHOU Zhi-Qiang; LI Feng-Yan; SUN Yun.Properties of One-Step Electrodeposited Cu(In1-x, Gax)Se2 Thin Films[J]. Acta Phys. -Chim. Sin., 2008,24(06): 1073-1079
106. TANG Yu-Xin; TAO Jie; TAO Hai-Jun; WU Tao; WANG Ling; ZHANG Yan-Yan; LI Zhuan-Li; TIAN Xi-Lin.Fabrication and Characterization for Transparent Electrodes of TiO2 Nanotube Arrays on Fluorine-Doped Tin Oxide-Coated Glass[J]. Acta Phys. -Chim. Sin., 2008,24(06): 1120-1126
107. DENG Zheng-Hua; LI Ren-Gui; WANG Lu; DENG Jia-Min; GAO Jian-Dong; MA Zhi-Gang; DU Hong-Chang; SUO Ji-Shuan.Research and Development of Separators for Lithium-ion Battery[J]. Acta Phys. -Chim. Sin., 2007,23(Supp): 90-93
108. HU Jing; YANG Mei-Ni; LU Feng-Ting; DING Li-Ping; ZHANG Shu-Juan; FANG Yu.Monolayer Assembly of Pyrene on Glass Plate Surface and Its Selective Sensing Performances to Organic Copper (II) Salts[J]. Acta Phys. -Chim. Sin., 2007,23(12): 1839-1845
109. CHU Yan-Qiu; WU Bo; WU Liang; SHUI Qing; FU Zheng-Wen.Electrochromic Properties of Bismuth Oxide Thin Films Prepared by Reactive Pulsed Laser Deposition[J]. Acta Phys. -Chim. Sin., 2007,23(11): 1787-1791
110. MAN Yi; ZONG Rui-Long; ZHU Yong-Fa.Preparation and Photoelectrochemical Properties of Bi2MoO6 Films[J]. Acta Phys. -Chim. Sin., 2007,23(11): 1671-1676
111. ZHU Lei; CUI Xiao-Li; SHEN Jie; YANG Xi-Liang; ZHANG Zhuang-Jian.Visible Light Photoelectrochemical Response of Carbon-doped TiO2 Thin Films Prepared by DC Reactive Magnetron Sputtering[J]. Acta Phys. -Chim. Sin., 2007,23(11): 1662-1666
112. YU Huang-Zhong; PENG Jun-Biao.The Influence of the Solvent and the Device Structure on Performance of the MEH-PPV:PCBM Solar Cell[J]. Acta Phys. -Chim. Sin., 2007,23(10): 1637-1641
113. SHI Cheng-Wu; GE Qian; QIU Zhi-Guo; LI Bing; HAN Shi-Kui.Synthesis of 3-hexyl-1-methylimidazolium Iodide and Its Application in Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2007,23(09): 1473-1477
114. ZHANG Wei; WANG Shu-Liang; MA Yun-Qing; WANG Cui-Ping; LIU Xing-Jun.Influence of Interface Diffusion between Al Substrate and TiO2 Filmon Photocatalytic Activity[J]. Acta Phys. -Chim. Sin., 2007,23(09): 1347-1352
115. YUAN Hao; LI Qing-Hua; SHA Fei; XIE Li-Li; TIAN Zhen; WANG Li-Jun.Application of Ultraviolet Treatment in the Synthesis of Pure-silica Zeolite Thin Films with Low Dielectric Constant[J]. Acta Phys. -Chim. Sin., 2007,23(08): 1219-1223
116. LI Shi-Bin; WU Zhi-Ming; ZHU Kui-Peng; JIANG Ya-Dong; LI Wei; LIAO Nai-Man.Effect of Substrate Temperature on the Optical Properties of a-Si:H Films by RF-PECVD[J]. Acta Phys. -Chim. Sin., 2007,23(08): 1252-1256
117. YANG Hui; SHEN Qian-Hong; GAO Ji-Wei.Morphology Control of Anatase TiO2 Films Prepared at Low Temperature Using 4,4’-isopropylidenediphenol[J]. Acta Phys. -Chim. Sin., 2007,23(08): 1269-1274
118. ZHANG Hong-Fang; FU Ping-Ping; SONG Ying-Jie; DU Chen-Shu; YANG Hua-Bin; ZHOU Zuo-Xiang; WU Meng-Tao; HUANG Lai-He.Preparation and Properties of Sandwich-type Si/Fe/Si Film Anode for Lithium-ion Battery[J]. Acta Phys. -Chim. Sin., 2007,23(07): 1065-1070
119. TAI Hui-Ling; JIANG Ya-Dong; XIE Guang-Zhong; DU Xiao-Song; CHEN Xuan.Preparation and Gas Sensitive Properties of Polyaniline/Titanium Oxide Composite Thin Films[J]. Acta Phys. -Chim. Sin., 2007,23(06): 883-888
120. WU Lun-Peng; ZHAO Lian-Hua; ZHANG Hai-Ming; ZHAO Qing-Nan.Effects of the Adsorption of Oxygen on the Photocatalytic Activity of TiO2 Films Using PhotocurrentMethod[J]. Acta Phys. -Chim. Sin., 2007,23(05): 765-768
121. WU Yan; YAO Wen-Qing; ZHU Yong-Fa.Interfacial Structure of Ta2O5/Si Filmand Photoactivity[J]. Acta Phys. -Chim. Sin., 2007,23(05): 625-629
122. YANG Ya-Jie; JIANG Ya-Dong; XU Jian-Hua.Preparation and Properties of Conducting Polymeric Ultrathin Films[J]. Acta Phys. -Chim. Sin., 2007,23(04): 484-488
123. MA Liang; MA Jie; LIU Hui.Composite Electrodeposition of CoNiP-BaFe12O19Magnetic Thin Film[J]. Acta Phys. -Chim. Sin., 2007,23(04): 590-594
124. YAN Shan-Shan;WU Lian-Di;CHEN Feng;ZHANG Jin-Long.Low-temperature Preparation and Characterization of TiO2 Thin Films with a Bicrystalline Framework[J]. Acta Phys. -Chim. Sin., 2007,23(03): 414-418
125. YANG Xi-Kun;LI Yang;HENG Gen-Hua.Structure and Catalytic Properties of PtRu Alloy Thin-film[J]. Acta Phys. -Chim. Sin., 2007,23(03): 389-393
126. GAO Li-Ning;LU Feng-Ting;HU Jing; FANG; Yu.Progress in the Studies of Fluorescent Film Sensors[J]. Acta Phys. -Chim. Sin., 2007,23(02): 274-284
127. ZHANG Shi-Cheng;YAO Wen-Qing;ZHU Yong-Fa;SHI Li-Yi.Preparation and Photoelectrochemical Properties of Bi2WO6 Films with Visible Light Response[J]. Acta Phys. -Chim. Sin., 2007,23(01): 111-115
128. LIU Wen-Yuan;LI Chi-Lin;FU Zheng-Wen .Stability of Lithium Phosphorous Oxynitride Thin Films in Humid Air[J]. Acta Phys. -Chim. Sin., 2006,22(11): 1413-1418
129. ZHOU Yong-Ning;WU Chang-Liang;ZHANG Hua;WU Xiao-Jing;FU Zheng-Wen.The Electrochemical Properties of LiF-Ni Nanocomposite Thin Film[J]. Acta Phys. -Chim. Sin., 2006,22(09): 1111-1115
130. CHEN Ming-An;XIE Xuan;QI Hai-Ying;ZHANG Xin-Ming;LI Hui-Zhong;YANG Xi .Characterization of Self-assembled Bis-[triethoxysilylpropyl]tetrasulfide Silane Films on Surface of 2A12-T6 Aluminum Alloy[J]. Acta Phys. -Chim. Sin., 2006,22(08): 1025-1029
131. GAO Chen;BAO Jun;LUO Zhen-Lin;LIU Wen-Han.Recent Progresses in the Combinatorial Materials Science[J]. Acta Phys. -Chim. Sin., 2006,22(07): 899-912
132. ZHAO Feng-Ming;MA Chun-An;CHU You-Qun;XU Ying-Hua.Oxygen Reduction on Ni-MnO2 Electrode in Alkaline Solution[J]. Acta Phys. -Chim. Sin., 2006,22(06): 716-720
133. ZHONG Cheng;JIANG Yi-Ming;LUO Yu-Feng;LIAO Jia-Xing;WU Wei-Wei;LI Jin.Two New Methods for Characterizing the Kinetics of the Complexation of Metal/Organic Thin Films and Oxidation of Metal Thin Films[J]. Acta Phys. -Chim. Sin., 2006,22(06): 696-700
134. ZHOU Li-Jun;YAN Shan-Shan;TIAN Bao-Zhu;CHEN Feng;ZHANG Jin-Long;HUANG Jia-Zhen.Preparation and Characterization of Anatase-Brookite TiO2 Film on the PET Surface[J]. Acta Phys. -Chim. Sin., 2006,22(05): 569-573
135. XUE Ming-Zhe; CHENG Sun-Chao; YAO Jia; FU Zheng-Wen.Electrochemical Properties of SnSe Thin Film Electrode Fabricated by Pulsed Laser Deposition[J]. Acta Phys. -Chim. Sin., 2006,22(03): 383-387
136. LI Hai-Ling; WANG Wen-Jing; KANG Guo-Hu; HUANG Jin-Zhao; XU Zheng.The Effect of Reactive Pressure to Fe:NiOx Film as Anode Catalytic Film in Hydrogen Producing System by Solar Cell[J]. Acta Phys. -Chim. Sin., 2006,22(03): 330-334
137. SHI Jian-zhen; FANG Jing-huai; MU Ren-wang; LI Ya-li.Preparation of Au Core-Ag Shell Nanoparticles Film and Its SERS Activity Study[J]. Acta Phys. -Chim. Sin., 2006,22(02): 135-140
138. WANG Ying; LIU Wen-yuan; FU Zheng-wen.Electrochemistry of Mn4N with Lithium[J]. Acta Phys. -Chim. Sin., 2006,22(01): 65-70
139. DAI Wen-xin; WANG Xu-xu; FU Xian-zhi; LIU Ping; LIN Hua-xiang.Effect of Halides on Photo-induced Hydrophilicity over TiO2 Films[J]. Acta Phys. -Chim. Sin., 2005,21(11): 1274-1279
140. LIU Ping; JIANG Yi-ming; GUO Feng; XIE Heng-bo; LI Jin.Studies on the Transport Behavior in Ag/TCNQ Thin Films[J]. Acta Phys. -Chim. Sin., 2005,21(10): 1073-1075
141. PENG Feng; CHEN Shui-hui; ZHANG Lei; WANG Hong-juan; XIE Zhi-yong.Preparation of Visible-light Response Nano-sized ZnO Film and Its Photocatalytic Degradation to Methyl Orange[J]. Acta Phys. -Chim. Sin., 2005,21(08): 944-948
142. XUE Ming-zhe; FU Zheng-wen.Electrochemical Properties of LiFePO4 Cathode Thin Film Fabricated by Pulsed Laser Deposition[J]. Acta Phys. -Chim. Sin., 2005,21(07): 707-710
143. XIONG Yu-hua; LI Feng-yi.Degradation of Polyethylene Film by Fe3+/TiO2 Photocatalyst[J]. Acta Phys. -Chim. Sin., 2005,21(06): 607-611
144. CHEN Zhi-gang; TANG Yi-wen; ZHANG Li-sha; CHEN Zheng-hua; JIA Zhi-jie.Electrochemical Deposition and Characterization of Zinc Oxide Thin Films[J]. Acta Phys. -Chim. Sin., 2005,21(06): 612-615
145. PAN Xu; DAI Song-yuan; WANG Kong-jia; SHI Cheng-wu; GUO Li.Development and Application of Electrolyte based on Ionic Liquid in Dye-sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2005,21(06): 697-702
146. LI Jian-Kang; YAO Xi.

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147. SHI Cheng-Wu; DAI Song-Yuan; WANG Kong-Jia; GUO Li; PAN Xu; KONG Fan-Tai; HU Lin-Hua.Optimization of 1,2-dimethyl-3-propylimidazolium Iodide Concentration in Dye-sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2005,21(05): 534-538
148. BAO Xing-Wang;ZHANG Jin-Long;LIANG Xue-Hai;HUANG Jia-Zhen;ZHANG Li-Zhong.Preparation of TiO2 Thin Films at Low Temperature and Characterization of Their Properties[J]. Acta Phys. -Chim. Sin., 2005,21(01): 69-73
149. Wang Juan; Zhang Chang-Rui; Feng Jian.Modification of Nanoporous Silica Film by Trimethylchlorosilane[J]. Acta Phys. -Chim. Sin., 2004,20(12): 1399-1403
150. Yu Chun-Ling;Zhai Jin;Ge Hong-Li;Wan Mei-Xiang;Jiang Lei;Li Ze-Sheng;Li Tie-Jin.Ordered Self-assembly of Polymer Nano-structure[J]. Acta Phys. -Chim. Sin., 2004,20(10): 1258-1261
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152. Shen Jie;Wo Song-Tao;Cui Xiao-Li;Cai Zhen-Wei;Yang Xi-Liang;Zhang Zhuang-Jian.Photoelectrochemical Characteristics of Nano-Titanium Dioxide Thin Films Prepared by RF Magnetron Sputtering[J]. Acta Phys. -Chim. Sin., 2004,20(10): 1191-1195
153. Cao Jiang-Lin;Leng Wen-Hua;Zhang Jian-Qing;Cao Chu-Nan.Adsorption Behavior and Photooxidation Kinetics of OH- at TiO2 Thin Film Electrodes[J]. Acta Phys. -Chim. Sin., 2004,20(07): 735-739
154. Ren Da-Sen;Bei Zong-Min;Huang Li;Shen Jie;Cui Xiao-Li;Yang Xi-Liang;Zhang Zhuang-Jian.The Effect of Dopant Sb on the Superhydrophilicity and the Microstructure of the Nanoscale TiO2 Thin Film[J]. Acta Phys. -Chim. Sin., 2004,20(04): 414-416
155. Liao Wei;Wei Fang;Cao Wei-Xiao;Zhao Xin-Sheng.Monitoring Layer-by-layer Assembling of Films Containing Diazo-resines by Attenuated Total Reflection Fourier Transform Infrared Spectroscopy[J]. Acta Phys. -Chim. Sin., 2004,20(04): 405-408
156. Chen You-Jiang;Sun Shi-Gang;Gong Hui;Chen Sheng-Pei;Zhou Zhi-You;Li Jun-Tao.Nanostructured Films Prepared on Pt Microelectrode through Square Wave Oxidation-reduction Cycles and Their Particular IR Properties[J]. Acta Phys. -Chim. Sin., 2004,20(02): 129-133
157. Ren Da-Sen;Cui Xiao-Li;Zhang Qun;Wo Song-Tao;Yang Xi-Liang;Zhang Zhuang-Jian;Lu Ming.Characteristics of SiO2-TiO2 Complex Thin Films Prepared by Sol Method[J]. Acta Phys. -Chim. Sin., 2003,19(09): 829-833
158. Wang Shan;Fang Yu;Zhang Ying;Wang MingZhen;Hu DaoDao;Liao YiKun.Preparation of Chitosan/CdS Composite Films and Their Sensing Properties to Pyridine[J]. Acta Phys. -Chim. Sin., 2003,19(06): 514-518
159. Zhang Wen-Kui;Yang Xiao-Guang;Wang Yun-Gang;Yu Li-Yang;Ma Chun-An.Electrochemical Behaviors of Pd/Mm Rare Earth Film Electrodes in KOH Solution[J]. Acta Phys. -Chim. Sin., 2003,19(06): 569-572
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161. Cui Xiao-Li;Jiang Zhi-Yu.Electrochemical Behavior of ITO/TiO2 Electrode under UV Illumination[J]. Acta Phys. -Chim. Sin., 2002,18(11): 1014-1017
162. Zhao Zhuan-Qing;Yao Su-Wei;Zhang Wei-Guo;Gong Zheng-Lie.Preparation and Photoelectrochemical Performance of Photoelectrode of TiO2 Film on Nickel[J]. Acta Phys. -Chim. Sin., 2002,18(05): 473-476
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164. Zhao Wen-Kuan;Fang You-Ling.Synthesis of Photocatalytic Activity TiO2 Thin Films at LowTemperature[J]. Acta Phys. -Chim. Sin., 2002,18(04): 368-371
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