ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2016,Vol.32>> Issue(6)>> 1347-1370     doi: 10.3866/PKU.WHXB201603143         中文摘要
Application of Organic Hole-Transporting Materials in Perovskite Solar Cells
LIU Xue-Peng1,2, KONG Fan-Tai1, CHEN Wang-Chao1,2, YU Ting1,2, GUO Fu-Ling1, CHEN Jian1, DAI Song-Yuan3,1
1 Key Laboratory of Novel Thin Film Solar Cells, Institute of Applied Technology, Hefei Institutes of Physical Science, Chinese Academy of Sciences, Hefei 230031, P. R. China;
2 University of Science and Technology of China, Hefei 230026, P. R. China;
3 Beijing Key Laboratory of Novel Thin Film Solar Cells, North China Electric Power University, Beijing 102206, P. R. China
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Organic-inorganic halide perovskite solar cells (PSCs) have attracted increasing attention because of their desirable properties. A key advance has been the replacement of the liquid electrolytes by solid-state hole-transporting materials (HTMs), which not only improves the power conversion efficiency (PCE) but also enhances the cell stability. HTMs are now an integral part of PSCs. Both organic and inorganic HTMs have found application in PSCs. However, inorganic HTMs are hampered by the limited choice of materials and the relatively low PCE of the solar cells based on them. The development of new organic HTMs is therefore necessary to improve the PCE and stability of PSCs. This has become a focus of various research fields, and new HTMs continue to emerge in large numbers. In this paper, we give an overview of the use of organic HTMs in PSCs. According to their molecular weight, organic HTMs are classified as either molecular or polymeric. We discuss in detail the effects of the functional groups and structures of organic HTMs on the PCE, fill factor, open circuit voltage, and stability of the resulting PSCs, as developed in recent years. The paper also covers the highest occupied molecular orbitals, the hole mobility, and the use of additives in HTMs. Finally, forecasts of the future development of organic HTMs are reviewed.

Keywords: Perovskite solar cell   Organic hole transporting material   Triphenylamine   Small-molecule   Polymer  
Received: 2015-12-09 Accepted: 2016-03-09 Publication Date (Web): 2016-03-14
Corresponding Authors: KONG Fan-Tai, DAI Song-Yuan Email:;

Fund: The project was supported by the National High Technology Research and Development Program of China (863)(2015AA050602) and Natural Science Foundation of Anhui Province, China (1508085SMF224).

Cite this article: LIU Xue-Peng, KONG Fan-Tai, CHEN Wang-Chao, YU Ting, GUO Fu-Ling, CHEN Jian, DAI Song-Yuan. Application of Organic Hole-Transporting Materials in Perovskite Solar Cells[J]. Acta Phys. -Chim. Sin., 2016,32 (6): 1347-1370.    doi: 10.3866/PKU.WHXB201603143

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21. ZHANG Jin-Shui, WANG Bo, WANG Xin-Chen.Chemical Synthesis and Applications of Graphitic Carbon Nitride[J]. Acta Phys. -Chim. Sin., 2013,29(09): 1865-1876
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52. LIU Si-Yu, MENG Xiang-Ju, XIAO Feng-Shou.Hydrothermal Synthesis of Ordered Mesoporous Materials with High Stability at High Temperatures[J]. Acta Phys. -Chim. Sin., 2010,26(07): 1852-1859
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54. SUN Zhe, YUE Xin-Rong, LIU Chuan, ZHANG Ai.Self Consistent Field Analysis on the Adsorption of Equilibrium Polymers between Two Parallel Plates[J]. Acta Phys. -Chim. Sin., 2010,26(06): 1629-1636
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65. WANG Chun-Guang, XING Yong-Heng, XIE Yan, LI Zhang-Peng, LI Jing, ZENG Xiao-Qing, GE Mao-Fa.Syntheses, Structures and Luminescent Properties of the Heterometallic Complexes [Ln2Zn2(2,5-pydc)5(H2O)2]·4H2O[J]. Acta Phys. -Chim. Sin., 2009,25(08): 1545-1549
66. TAO Chang-Gui, FENG Hai-Jun, ZHOU Jian, LV Ling-Hong, LU Xiao-Hua.Molecular Simulation of Oxygen Adsorption and Diffusion in Polypropylene[J]. Acta Phys. -Chim. Sin., 2009,25(07): 1373-1378
67. DENG Yi-Bin, HU Bing-Wen, ZHOU Ping.Solid-State NMR Studies of Structures and Molecular Motions for the Spidroin-Like Polymers[J]. Acta Phys. -Chim. Sin., 2009,25(07): 1427-1433
68. YANG Ji-Sheng, CHEN Sheng-Bi, FANG Yun.Effect of Surfactants on the Shear Viscosity of Dilute Aqueous Solutions of Sodium Alginate[J]. Acta Phys. -Chim. Sin., 2009,25(04): 752-756
69. ZHANG Guo-Qiang, MA Li, WU Zhong-Jie, ZHANG Hai-Yan, NI Pei.Electrochemical Behaviour of the Composite Polymer Electrolyte P(VDF-HFP)-PMMA/CaCO3(SiO2)[J]. Acta Phys. -Chim. Sin., 2009,25(03): 555-560
70. DOU Wen-Ling; XIN Xia; XU Gui-Ying.Dispersion of Carbon Nanotubes by Amphiphilic Molecules[J]. Acta Phys. -Chim. Sin., 2009,25(02): 382-388
71. WANG Fei-Yu; GAO Bao-Jiao; WANG Rui-Xin.Simultaneous Synthesis and Linkage of Porphyrin onto Side Chain of Copolymer P(GMA-co-MMA)[J]. Acta Phys. -Chim. Sin., 2009,25(02): 341-346
72. XU Jian-Hua; YANG Ya-Jie; JIANG Ya-Dong; YU Jun-Sheng.Synthesis of Ordered Conducting Polymer Ultrathin Film and Its Application as Hole Injection Layer for Organic Light-Emitting Diode[J]. Acta Phys. -Chim. Sin., 2009,25(01): 19-24
73. JIANG Jin-Qiang; FENG Yan; WANG Hong-Mei; LIU Xiao-Ya; ZHANG Sheng-Wen; CHEN Ming-Qing.Synthesis and Micellization of Photosensitive Amphiphilic Comblike SMA Polymer[J]. Acta Phys. -Chim. Sin., 2008,24(11): 2089-2095
74. PEI Juan, LIANG Mao, CHEN Jun, TAO Zhan-Liang, XU Wei.Application of Triphenylamine-Based Sensitizers with Two Carboxylic Acid Groups to Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2008,24(11): 1950-1956
75. ZHENG Shao-Jun; YUAN Zhao; ZENG Yi; LI Ying-Ying; LI Yi.Microenvironment of Dendrimers Probing by Pyrene and Anthracene as Fluorescence Probes[J]. Acta Phys. -Chim. Sin., 2008,24(10): 1785-1789
76. QIAN Bao-Hua; MA Wei-Xing; XU Xing-You; LU Lu-De; YANG Xu-Jie; WANG Xin.Synthesis, Characterization and Quantum Chemistry Study of a One-dimensional Chain Coordination Polymer [Zn(acac)2(4,4’-bipy)]n[J]. Acta Phys. -Chim. Sin., 2008,24(09): 1650-1654
77. SUN Zhe; SONG Hai-Hua.Stratification in Bimodal Polymer Brushes[J]. Acta Phys. -Chim. Sin., 2008,24(08): 1487-1492
78. XIAO Ping-Ping.Real-Time Investigation on Refractive-Index and Thickness of Polymer Films during Photobleaching Process[J]. Acta Phys. -Chim. Sin., 2008,24(07): 1321-1325
79. TANG Xiao-Qing; YU Jun-Sheng; LI Lu; WANG Jun; JIANG Ya-Dong.Polymer Doped High Brightness Phosphorescent Organic Light-Emitting Diodes[J]. Acta Phys. -Chim. Sin., 2008,24(06): 1012-1016
80. YU Huang-Zhong; PENG Jun-Biao.Annealing Treatment Effect on Photoelectric Properties of P3HT:PCBMBlend System[J]. Acta Phys. -Chim. Sin., 2008,24(05): 905-908
81. WANG Miao; YU Hai-Yan; OUYANG Jian-Ming.Modulation of Eucheuma Striatum Sulfated Polysaccharide before and after Degradation on Crystal Growth of Calcium Oxalates[J]. Acta Phys. -Chim. Sin., 2008,24(01): 109-114
82. TANG Ding-Guo.Application of Polymer LithiumIon Batteries Based on IPN[J]. Acta Phys. -Chim. Sin., 2007,23(Supp): 18-20
83. DENG Zheng-Hua; LI Ren-Gui; WANG Lu; DENG Jia-Min; GAO Jian-Dong; MA Zhi-Gang; DU Hong-Chang; SUO Ji-Shuan.Research and Development of Separators for Lithium-ion Battery[J]. Acta Phys. -Chim. Sin., 2007,23(Supp): 90-93
84. FENG Hua-Jun; CHEN Yuan;DAI Ke-Hua; SONG Zhao-Shuang; MA Jian-Wei; QI Lu.Preparation and Characterization of a Novel Kind of Polymer Electrolyte Composite Membrane for Lithium-Ion Battery[J]. Acta Phys. -Chim. Sin., 2007,23(12): 1922-1926
85. SONG Zhao-Shuang; QI Lu; QIU Jing-Yi; MA Jian-Wei.Preparation and Characterization of γ-Ray Irradiated Gel Polymer Electrolyte for Lithium-Ion Polymer Batteries[J]. Acta Phys. -Chim. Sin., 2007,23(12): 1932-1936
86. CHEN Jie; ZHAO Xin; CHEN Jin-Ping; LI Yi.Fluorescence Quenching of Poly(aryl ether) Dendrimers by Metal Ions[J]. Acta Phys. -Chim. Sin., 2007,23(11): 1696-1700
87. YU Huang-Zhong; PENG Jun-Biao.The Influence of the Solvent and the Device Structure on Performance of the MEH-PPV:PCBM Solar Cell[J]. Acta Phys. -Chim. Sin., 2007,23(10): 1637-1641
88. ZHANG Ji-Fu; SANG Shang-Bin; WU Qiu-Mei; LIAO Yu-Gen.Preparation and Characterization of the Composite Alkaline Polymer Electrolyte Based on PVA-Bentonite-KOH-H2O[J]. Acta Phys. -Chim. Sin., 2007,23(07): 1136-1140
89. PENG Shun-Jin; ZHAO Lei; WU Li-Min.Surface Properties of Fluorinated Acrylate Polymers Latex Films[J]. Acta Phys. -Chim. Sin., 2007,23(04): 531-536
90. YANG Ya-Jie; JIANG Ya-Dong; XU Jian-Hua.Preparation and Properties of Conducting Polymeric Ultrathin Films[J]. Acta Phys. -Chim. Sin., 2007,23(04): 484-488
91. TONG Shao-Ping;MA Chun-An;FEI Hui.Deactivation of Two Different Kinds of Anodes during the Degradation of Organics and Their Oxidative Mechanisms[J]. Acta Phys. -Chim. Sin., 2007,23(03): 424-428
92. CHEN Hong-Xiang;ZHOU Jian-Zhang;XI Yan-Yan;LAN Bi-Bo;FENG Zeng-Fang;YAO Guang-Hua;LIN Zhong-Hua.Charge Transport Performance of Nafion-based Redox Polymer in Atmosphere[J]. Acta Phys. -Chim. Sin., 2007,23(03): 404-408
93. DENG Hui-Ning;WANG Yu-Xin .Sulfonated Poly(phthalazinones) Membranes For Direct Methanol Fuel Cell[J]. Acta Phys. -Chim. Sin., 2007,23(02): 187-191
94. GUO Jin-Yu;ZHANG Jian-Guo;ZHANG Tong-Lai;WU Rui-Feng;YU Wei.Thermal Decomposition Mechanisms of a Three-dimensional Framework Coordination Polymer [Cu(HCOO)2(H2O)2][J]. Acta Phys. -Chim. Sin., 2006,22(10): 1206-1211
95. LEI Zhong-Li;FAN You-Hua .Preparation and Characterization of Silver Nanocomposites Based on Copolymers[J]. Acta Phys. -Chim. Sin., 2006,22(08): 1021-1024
96. TANG Ding-Guo;CI Yun-Xiang;QI Lu.Influence of Thermal Initiators on the Electrochemical Performances of Gel Polymer Electrolytes[J]. Acta Phys. -Chim. Sin., 2006,22(07): 826-830
97. LU Xiang-Guo;WANG Wei.The Molecular Configuration and Its Influential Factors of Al3+ Cross-linked Polyacrylamide Gel[J]. Acta Phys. -Chim. Sin., 2006,22(05): 631-634
98. ZHANG Lu; YOU Chang-Jiang; CHEN Jin-Ping; YANG Guo-Qiang; LI Yi.Dendritic Bis-(8-hydroxyquinoline) Derivatives: Studies on the Fluorescence Quenching and Decay[J]. Acta Phys. -Chim. Sin., 2006,22(03): 326-329
99. TANG Ding-guo; LIU Jian-hong; CI Yun-xiang; QI Lu.Preparation and Performances of a Novel Gel Polymer Electrolyte[J]. Acta Phys. -Chim. Sin., 2005,21(11): 1263-1268
100. ZHANG Shu-guang; SHI Wen-yan; LEI Wu; XIA Ming-zhu; WANG Feng-yun.Molecular Dynamics Simulation of Interaction between Calcite Crystal and Water-soluble Polymers[J]. Acta Phys. -Chim. Sin., 2005,21(11): 1198-1204
101. WANG Dong-xian; LUO Lan; ZHANG Lu; WANG Yi-yang; ZHAO Sui; YU Jia-yong.Study on Interfacial Interaction between Hydrophobically Modified Polyacrylamide and Surfactants[J]. Acta Phys. -Chim. Sin., 2005,21(11): 1205-1210
102. LI Xue-Li; GUO Juan; WU Qiang; CHENG Yan; LONG Ying-Cai; JIANG Zhi-Yu.Research on the Enhanced Conductivity of Poly(ethylene oxide) Electrolyte by Adding Zeolite Li-FER[J]. Acta Phys. -Chim. Sin., 2005,21(04): 397-401
103. Zhou Jian-Zhang; Dong Ping; Cai Cheng-Dong; Lin Zhong-Hua.Chemically Modified AAO Template and Application to PANI Nanowires Synthesis[J]. Acta Phys. -Chim. Sin., 2004,20(11): 1287-1291
104. Zhang Ming;Lu Ping;Tian Lei-Lei;Zhang Wu;Yang Bing;Ma Yu-Guang.Study of the Fluorescent Conjugated Polymers on Metal Ion Sensing[J]. Acta Phys. -Chim. Sin., 2004,20(08S): 924-929
105. Lin Mei-Qin;Sun Ai-Jun;Dong Zhao-Xia;Tang Ya-Lin;Li Ming-Yuan;Wu Zhao-Liang.Study on Properties of the Linked Polymer Solution with Low Polymer Concentration[J]. Acta Phys. -Chim. Sin., 2004,20(03): 285-289
106. Wang Zhan-Liang;Tang Zhi-Yuan.Research on the Interfacial Properties of Polymer Electrolyte by A.C.Impedance[J]. Acta Phys. -Chim. Sin., 2003,19(12): 1097-1101
107. Xu Yi-Ting;Dai Li-Zong;He Yun-You;Tahina Rakotoartsoa;JeanYves Gal;Wu HuiHuang.Electrochemical and Electrocatalytic Properties of Polyaniline Derivatives Membrane Modified Electrode[J]. Acta Phys. -Chim. Sin., 2003,19(06): 564-568
108. Hou Ji-Rui;Liu Zhong-Chun;Zhang Shu-Fen;Yue Xiang-An;Yang Jin-Zong.Effect of Alkali on Molecular Configuration of Polymer and Its Rheologic Behavior[J]. Acta Phys. -Chim. Sin., 2003,19(03): 256-259
109. Wang Zhan-Liang;Tang Zhi-Yuan;Geng Xin;Xue Jian-Jun.Research on Novel PMMAbased Gel Electrolyte for Lithium Ion Battery[J]. Acta Phys. -Chim. Sin., 2002,18(03): 272-275
110. Huang Wei-Ping;Zheng Xiu-Cheng;Zhang Shou-Min;Qiu Xiao-Hang;Li Bao-Qing;Wu Shi-Hua.Structure and Activity of Polymer Immobilized Co-Pd Catalysts[J]. Acta Phys. -Chim. Sin., 2002,18(03): 243-247
111. Kong Yong;Mu Shao-Lin.Electrochemical Polymerization of Thionine and Properties of Polythionine[J]. Acta Phys. -Chim. Sin., 2001,17(04): 295-299
112. Chen Yuan-Mei;Huang Yuan-He;Liu Ruo-Zhuang.Intermolecular Electron-phonon Coupling in One-dimensional C36 Polymers[J]. Acta Phys. -Chim. Sin., 2001,17(03): 196-200
113. Shao Ke, Ma Ying, Cao Ya-An, Chen Chao-Hui, Ji Xue-Hai, Yao Jian-Nian.Inclusion of Poly(TMPD) into MoO3 via a Cooperative Formation Route[J]. Acta Phys. -Chim. Sin., 2000,16(10): 865-868
114. Yang Qiu-Xia, Gao Gui-Lian, Wang Xue-Lin.Electropolymerized Hemin Film Electrode and its Catalytic Reuction of Oxygen[J]. Acta Phys. -Chim. Sin., 2000,16(08): 741-745
115. Liu Shou-Xin, Fang Yu, Hu Dao-Dao, Lv Hong-Wang.Complexation between Poly(methacrylic acid) and Cationically Modified Polyacrylamide[J]. Acta Phys. -Chim. Sin., 2000,16(03): 214-220
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117. Yan Li-Jing, He Yu-Fan, Lin Hai-Chao, Wu Wei-Tao.Study on the Inhibition Effect of Polymer Film of Propargyl Alcohol in Fe/H2SO4 and Fe/H2SO4+H2S Systems[J]. Acta Phys. -Chim. Sin., 1999,15(08): 726-734
118. Chen Wen, Xu Qing, Yuan Run-Zhang, Ren Hai-Lan, Yue Yong, Ye Chao-Hui.Study on the lonic Transport of Polymer-Lithium Exchanged Montmorlillonite Composites[J]. Acta Phys. -Chim. Sin., 1999,15(08): 704-708
119. Tan Ye-Bang, Zhang Li Ming, Li Zhuo-Mei.Adsorption of Amphoteric Cellulose Graft Copolymer on Bentonite[J]. Acta Phys. -Chim. Sin., 1998,14(12): 1112-1115
120. Jiang Jun-Hua, Chen Lan, Wu Bing-Liang, Zhai Run-Sheng.Electrochemical Reduction of Nitrobenzene on the Cu/C-Nafion Composite Electrode[J]. Acta Phys. -Chim. Sin., 1998,14(08): 704-708
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122. Tan Hai-Shu,Chen Li-Chun,Yang Xiao-Hui,Wang Xiang-Jun,Xie Hong-Quan,Gao Guang-Hu.Thin Film Light-emitting Diodes with Organic/Inorganic Heterostructure[J]. Acta Phys. -Chim. Sin., 1997,13(10): 942-945
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124. Zhou Xu-Zhang,Chen Jing-Wei,Shan Fu.Determination of Terminal OH Groups in Polymers by Differential Direct Injection Enthalpimetry[J]. Acta Phys. -Chim. Sin., 1997,13(01): 64-67
125. Chen Li-Chun,Deng Zhen-Bo,Wang Xiang-Jun,Xu Xu-Rong,Yao Jian-Quan.AC Electroluminescent Device Based on Polymers[J]. Acta Phys. -Chim. Sin., 1996,12(08): 755-757
126. Chen Zhen.Application of Solid Polymer Electrolyte in Electrooxidation of Cinnamyl Alcohol(II)——Influence of Follow-up Reaction on Electro-catalytic Reaction[J]. Acta Phys. -Chim. Sin., 1993,9(03): 319-324
127. Chen Zhen.Application of SPE(Solid Polymer Electrolyte) in Electrooxidation of Cinnamyl Alcohol(I)[J]. Acta Phys. -Chim. Sin., 1993,9(02): 181-186
128. Chen Yan-Zhen; Gu Zhi-Jun; Tian Zhong-Qun.Photoelectrochemical Polymerization of Conducting Polymer Monomers[J]. Acta Phys. -Chim. Sin., 1993,9(02): 277-280
129. Zeng Guang-Fu; Guo Xin; Wang Cui-Ying; Lin Yong-Hua; Li Han.Infrared Spectra and Crystal Structure of BIS-(Dimethoxylphosphato) Copper[J]. Acta Phys. -Chim. Sin., 1992,8(06): 778-782
130. PENG Xue-Feng, LEI Yong, LIU Zhen, FAN Chang-Jun, JI Xia-Xia, YANG Xiao-Hui.Thermally Activated Delayed Fluorescence and Sensitization Devices using Polymer Host Material[J]. Acta Phys. -Chim. Sin., 0,(): 0-0
131. HAO Wei-Ju, ZHANG Jun-Qi, SHANG Ya-Zhuo, XU Shou-Hong, LIU Hong-Lai.Preparation of Fluoresence Labeling pH-Sensitive Micelles for Controlled Drug Release[J]. Acta Phys. -Chim. Sin., 0,(): 0-0
132. LIANG Jia-Xu, XIAO Zhi-Chang, ZHI Lin-Jie.Graphenal Polymers: 3D Carbon-rich Polymers as Energy Materials with both Electronic and Ionic Transport Path[J]. Acta Phys. -Chim. Sin., 0,(): 0-0
133. WANG Yan-Qing, LI Long, NIE Lin-Hui, LI Nan-Nan, SHI Cheng-Wu.Organic-Inorganic Hybrid Perovskite Solar Cells Processed with Br or Cl Doping Via the Two Steps Deposition[J]. Acta Phys. -Chim. Sin., 0,(): 0-0
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