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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2016,Vol.32>> Issue(8)>> 2052-2058     doi: 10.3866/PKU.WHXB201604213         中文摘要
Removal of Sr2+ Ions by Ta-Doped Hexagonal WO3: Zeta Potential Measurements and Adsorption Mechanism Determination
JIAN Yuan1,2, MU Wan-Jun2, LIU Ning1, PENG Shu-Ming1,2
1 Key Laboratory of Radiation Physics and Technology, Ministry of Education, Institute of Nuclear Science and Technology, Sichuan University, Chengdu 610064, P. R. China;
2 Institute of Nuclear Physics and Chemistry, China Academy of Engineering Physics, Mianyang 621900, Sichuan Province, P. R. China
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The adsorption of Sr2+ ions onto Ta-doped hex-WO3 nanomaterials was studied by measuring the zeta potentials of the powder nanoparticles and by determining the adsorption isotherm and adsorption mechanism. Five important results were obtained: (1) the zeta potential values of the Ta-doped hex-WO3 suspensions in different electrolyte solutions, within the studied pH ranges, increased with an increase in electrolyte valence; and (2) the zeta potential of the Ta-doped hex-WO3 suspensions increased with an increase in ionic strength. (3) Sr2+ ion adsorption increased with a decrease in temperature and ionic strength. (4) The adsorption enthalpy was calculated as -47 kJ·mol-1, and the interaction between the Ta-doped hex-WO3 surface and Sr2+ ions was concluded to be chemical in nature. (5) The adsorption of Sr2+ ions onto the Ta-doped hex-WO3 was attributed to surface chemical adsorption and ion exchange (in tunnels).



Keywords: Ta   hex-WO3   Zeta potential   Sr2+   Adsorption mechanism  
Received: 2016-02-29 Accepted: 2016-04-20 Publication Date (Web): 2016-04-21
Corresponding Authors: PENG Shu-Ming, JIAN Yuan Email: pengsm01@163.com;inpc207@163.com

Fund: The project was supported by the National Natural Science Foundation of China (21501159).

Cite this article: JIAN Yuan, MU Wan-Jun, LIU Ning, PENG Shu-Ming. Removal of Sr2+ Ions by Ta-Doped Hexagonal WO3: Zeta Potential Measurements and Adsorption Mechanism Determination[J]. Acta Phys. -Chim. Sin., 2016,32 (8): 2052-2058.    doi: 10.3866/PKU.WHXB201604213

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74. Qian Shao-Hua;Qian Jun-Hong;Guo Rong.The Effect of Cephanone on the Structural Characters of CTAB Micelles[J]. Acta Phys. -Chim. Sin., 2003,19(12): 1127-1132
75. Huang Jian-Gou;Xu Man-Cai;Li Hai-Tao;Shi Zuo-Qing;He Bing-Lin.Adsorption Thermodynamics of Macroporous Cross-linked Poly (N-methyl-N-p- vinylbenzylacetamine) Resin for Phenols from Non-aqueous System[J]. Acta Phys. -Chim. Sin., 2003,19(03): 208-211
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77. Guo Rong;Ji Yun;Zhang Qi-Qing;Zhang Xiao-Hong.The Effects of Penicillin Potassium Salt on the Characters of CTAB Micelles[J]. Acta Phys. -Chim. Sin., 2002,18(01): 50-54
78. Guo Rong;Liu Wei-Ya;Fan Guo-Kang.Interaction of Malachite Green with CTAB Micelles[J]. Acta Phys. -Chim. Sin., 2001,17(12): 1062-1066
79. Guo Yuan;Li Yong-Jun;Xia Xi;Zhang Xiao-Gang;He Mao-Xia.Effect of Extrinsic Factors on the CPE Behavior of Film TiO2 Electrode[J]. Acta Phys. -Chim. Sin., 2001,17(04): 372-376
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87. Cao Ya, Li Hui-Lin, Zhang Ai-Min.Studies on Adsorption of Carboxy Methyl Cellulose Based Polymeric Surfactants at Solid/Liquid lnterface[J]. Acta Phys. -Chim. Sin., 1999,15(10): 952-955
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89. Wang Zhen, Zhang Hao-Li, Li Hu-Lin.Self-assembly Behavior of Azobenzene Derivative β-Cyclodextrin Inclusion Complex on Gold[J]. Acta Phys. -Chim. Sin., 1999,15(07): 606-612
90. Sun Ji-Hong, Gong Yan-Jun, Fan Wen-Hao, Wu Dong, Sun Yu-Han.Themal Physical Chemical Characteristics of SiO2-PEG Xerogels[J]. Acta Phys. -Chim. Sin., 1999,15(06): 517-521
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92. Shi Xiang-Yang, Wu Shi-Kang.A Study on the Micellar Polarity of Hydrophobic Poly(N-isopropylacrylmides)[J]. Acta Phys. -Chim. Sin., 1999,15(02): 127-132
93. Pan Yun-Xiang, Guan Xiang-Ying, Feng Zeng-Yuan, Li Xiu-Yu, Yan Zheng.Study on the Kinetic Mechanism of the Dehydration Process of FeC2O4·2H2O Using Double Extrapolation[J]. Acta Phys. -Chim. Sin., 1998,14(12): 1088-1093
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95. Tong Hua, Yao Song-Nian.Effect of Different Types of Electrolyte on Surface Potential of Liposome of PC and PC-Cholesterol[J]. Acta Phys. -Chim. Sin., 1998,14(11): 1043-1047
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