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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2016,Vol.32>> Issue(10)>> 2475-2487     doi: 10.3866/PKU.WHXB201607121         中文摘要
Two-Dimensional Layered Zeolite Precursors: Syntheses, Modifications and Catalytic Applications
ZHAO Zhen-Chao, ZHANG Wei-Ping
State Key Laboratory of Fine Chemicals, School of Chemical Engineering, Dalian University of Technology, Dalian 116024, Liaoning Province, P. R. China
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Two-dimensional layered zeolite precursors (LZPs) with layered structural units of parent threedimensional zeolites possess the properties of the parent materials but with an open framework structure. The structural properties of these materials therefore provide new opportunities to synthesize new zeolites and fabricate sub-zeolites with distinct structures, making them a hot topic in zeolite research. Enormous LZPs were synthesized by the direct crystallization or post-modification of their three-dimensional parent structures. Several layer manipulation strategies, including swelling, delamination, pillaring and layer reassembly have been developed on two-dimensional LZPs. These strategies have provided access to zeolites with new structures as well as materials even violating the theoretical rules, which have greatly enhanced the field of two-dimensional LZPs, and expanded their applications in catalysis and separation. Herein, we have reviewed the structural characteristics of two-dimensional LZPs, as well as summarizing their syntheses, modifications, and catalytic applications. We have also proposed the future perspectives of two-dimensional LZPs.



Keywords: Two-dimensional layer   Lamellar zeolite   Topotactic conversion   Structure modification   Catalytic application  
Received: 2016-05-25 Accepted: 2016-07-12 Publication Date (Web): 2016-07-12
Corresponding Authors: ZHANG Wei-Ping Email: wpzhang@dlut.edu.cn

Fund: The project was supported by the National Natural Science Foundation of China (21173029, 21373035) and Fundamental Research Funds for the Central Universities in China (DUT16RC(3)002).

Cite this article: ZHAO Zhen-Chao, ZHANG Wei-Ping. Two-Dimensional Layered Zeolite Precursors: Syntheses, Modifications and Catalytic Applications[J]. Acta Phys. -Chim. Sin., 2016,32 (10): 2475-2487.    doi: 10.3866/PKU.WHXB201607121

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