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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2016,Vol.32>> Issue(12)>> 2826-2840     doi: 10.3866/PKU.WHXB201609141         中文摘要
Soft-Templated Ordered Mesoporous Carbon Materials: Synthesis, Structural Modification and Functionalization
LIU Dan, HU Yan-Yan, ZENG Chao, QU De-Yu
Department of Chemistry, School of Chemistry, Chemical Engineering and Life Sciences, Wuhan University of Technology, Wuhan 430070, P. R. China
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Ordered mesoporous carbon materials (OMCs) have potentially broad applications in many fields, such as adsorption, separation, catalysis, and energy storage/conversion. Compared with the elaborate hardtemplate strategy, the soft-template approach, which is based on the self-assembly between amphiphilic block copolymers and polymerizable precursors (e.g., phenolic resins), is a more effective and efficient method for the synthesis of OMCs. In this review, the mechanism and characteristics for three main soft-template methods, i.e., solvent evaporation-induced self-assembly synthesis, aqueous cooperative self-assembly synthesis and solvent-free synthesis, are discussed and compared. In addition, a few highlights of recent progress, including application of novel carbon precursors, structural modification and functionalization of OMCs, are outlined. Finally, we summarize the crucial issues to be addressed in developing the synthesis methodology of OMCs.



Keywords: Ordered mesoporous material   Porous carbon   Block copolymer   Soft template   Self-assembly  
Received: 2016-06-24 Accepted: 2016-09-14 Publication Date (Web): 2016-09-14
Corresponding Authors: QU De-Yu Email: deyuquwuhan@163.com

Fund: The project was supported by the National Natural Science Foundation of China (21401145, 11474226).

Cite this article: LIU Dan, HU Yan-Yan, ZENG Chao, QU De-Yu. Soft-Templated Ordered Mesoporous Carbon Materials: Synthesis, Structural Modification and Functionalization[J]. Acta Phys. -Chim. Sin., 2016,32 (12): 2826-2840.    doi: 10.3866/PKU.WHXB201609141
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97. ZHOU Xiao-shun; XU Xiaomi; ZHONG Hui-ping; LONG La-sheng; HUANG Rong-bin; XIE Zhao-xiong; ZHENG Lan-sun; MAO Bing-wei.Adsorption of Metal-Organic Complex Molecule on Au(111) Surface[J]. Acta Phys. -Chim. Sin., 2005,21(09): 949-951
98. AN Shi-yan; XU Shan-dong; ZENG Qing-dao; TAN Zhong-yin; WANG Chen; WAN Li-jun; BAI Chun-li.The Self-assembly Structure of Pyrazine Derivative on Highly Oriented Pyrolytic Graphite[J]. Acta Phys. -Chim. Sin., 2005,21(08): 925-928
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155. CHENG Fang, WANG Han-Qi, XU Kuang, HE Wei.Preparation and Characterization of Dithiocarbamate Based Carbohydrate Chips[J]. Acta Phys. -Chim. Sin., 0,(): 0-0
156. YUAN Hong, ZHANG Jing, WEI Xue-Hong, FANG Hui-Min, YUAN Shi-Fang, WU Li-Xin.A Chiral Luminescent Liquid Crystal Material Based on Europium-Substituted Polyoxometalate[J]. Acta Phys. -Chim. Sin., 0,(): 0-0
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159. YANG Hai-Kuan.A Solution-Based Self-Assembly Approach to Preparing Functional Supramolecular Hybrid Materials[J]. Acta Phys. -Chim. Sin., 0,(): 0-0
160. GUO Rui, ZHANG Jialin, ZHAO Songtao, YU Xiaojiang, ZHONG Shu, SUN Shuo, LI Zhenyu, CHEN Wei.LT-STM Investigation of the Self-Assembled F16CuPc-Corannulene Binary System on Ag(111) and Graphite[J]. Acta Phys. -Chim. Sin., 0,(): 0-0
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