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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2017,Vol.33>> Issue(2)>> 399-406     doi: 10.3866/PKU.WHXB201611092         中文摘要
Facet Effect on Surface Thermodynamic Properties and In-situ Photocatalytic Thermokinetics of Ag3PO4
XIAO Ming1, HUANG Zai-Yin1,2,3, TANG Huan-Feng1, LU Sang-Ting1, LIU Chao1
1 College of Chemistry and Chemical Engineering, Guangxi University for Nationalities, Nanning 530006, P. R. China;
2 Key Laboratory of Forest Chemistry and Engineering, Guangxi University for Nationalities, Nanning 530006, P. R. China;
3 Guangxi Colleges and Universities Key Laboratory of Food Safety and Pharmaceutical Analytical Chemistry, Nanning 530006, P. R. China
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Cubic{100}, tetrahedral{111}, and rhombic dodecahedral{110} Ag3PO4 microcrystals were synthesized via a facile wet chemical method. Their components, structure, morphology, and photoelectrical properties were characterized by field emission scanning electron microscopy (FE-SEM), X-ray powder diffraction (XRD), ultraviolet-visible diffuse reflectance spectroscopy (UV-Vis DRS), photocurrent and photoluminescence (PL) analyses. The photocatalytic activity of the Ag3PO4 crystallites with different morphologies were investigated under visible illumination using rhodamine B (RhB) as a target contaminant. Meanwhile, the surface molar Gibbs free energy of the Ag3PO4 crystallites was determined by microcalorimetry via transition state theory and the thermochemical cycle principle. The corresponding values for cubic, tetrahedral, and rhombic dodecahedral microcrystals were 1.2972, 0.9621, and 0.5414 kJ·mol-1, respectively. The heat effect of the in-situ photocatalytic degradation of RhB and heat flow of the stable exothermic stage over the Ag3PO4 crystallites was detected by a LED-photocalorimeter. The results showed that the catalytic activity of Ag3PO4 crystallites and the heat effect and heat flow of the stable exothermic stage were positively correlated with their molar Gibbs free energy.Additionally, the main active species for the photocatalytic degradation of RhB over Ag3PO4 crystallites were determined by trapping experiments and electron paramagnetic resonance (ESR) spectroscopy.



Keywords: Ag3PO4   Surface thermodynamics   In-situ photocalorimeter   Photocatalysis   Facet effect  
Received: 2016-09-08 Accepted: 2016-11-09 Publication Date (Web): 2016-11-09
Corresponding Authors: HUANG Zai-Yin Email: huangzaiyin@163.com

Fund: The project was supported by the National Natural Science Foundation of China (21273050, 21573048).

Cite this article: XIAO Ming, HUANG Zai-Yin, TANG Huan-Feng, LU Sang-Ting, LIU Chao. Facet Effect on Surface Thermodynamic Properties and In-situ Photocatalytic Thermokinetics of Ag3PO4[J]. Acta Phys. -Chim. Sin., 2017,33 (2): 399-406.    doi: 10.3866/PKU.WHXB201611092

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62. SHANG Yang, CHEN Yang, SHI Zhan-Bin, ZHANG Dong-Feng, GUO Lin.Synthesis and Visible Light Photocatalytic Activities of Au/Cu2O Heterogeneous Nanospheres[J]. Acta Phys. -Chim. Sin., 2013,29(08): 1819-1826
63. LI Bo, LÜ Gong Xuan.Highly Active and Stable Catalyst for Visible Light Hydrogen Production Based on Oxidative Quenching of Eosin Y[J]. Acta Phys. -Chim. Sin., 2013,29(08): 1778-1784
64. LV Yong-Gang, LI Zhi-Jun, WU Li-Zhu, WANG Peng, FU Li-Min, ZHANG Jian-Ping.Application of Time-Resolved Coherent Anti-Stokes Raman Scattering Technique on the Study of Photocatalytic Hydrogen Production Kinetics[J]. Acta Phys. -Chim. Sin., 2013,29(08): 1632-1638
65. WANG Xiang, LI Ren-Gui, XU Qian, HAN Hong-Xian, LI Can.Roles of (001) and (101) Facets of Anatase TiO2 in Photocatalytic Reactions[J]. Acta Phys. -Chim. Sin., 2013,29(07): 1566-1571
66. GUO Li-Mei KUANG Yuan-Jiang YANG Xiao-Dan YU Yan-Long YAO Jiang-Hong CAO Ya-An.Investigation on Photocatalytic Reduction of CO2into CH4 Using SrB2O4/SrCO3Composite Catalyst[J]. Acta Phys. -Chim. Sin., 2013,29(07): 1558-1565
67. WANG Yang, SHAO Xiang, WANG Bing.Preparation, Characterization and Photocatalytic Activity of Cr-Doped Rutile TiO2(110) Single Crystal Thin Films[J]. Acta Phys. -Chim. Sin., 2013,29(07): 1363-1369
68. LIN Pei-Bin, YANG Yu, CHEN Wei, GAO Han-Yang, CHEN Xiao-Ping, YUAN Jian, SHANGGUAN Wen-Feng.Hydrothermal Synthesis and Activity of NiS-PdS/CdS Catalysts for Photocatalytic Hydrogen Evolution under Visible Light Irradiation[J]. Acta Phys. -Chim. Sin., 2013,29(06): 1313-1318
69. YANG Han-Pei, ZHANG Ying-Chao, FU Xiao-Fei, SONG Shuang-Shuang, WU Jun-Ming.Surface Modification of CNTs and Improved Photocatalytic Activity of TiO2-CNTs Heterojunction[J]. Acta Phys. -Chim. Sin., 2013,29(06): 1327-1335
70. LONG Mei, CONG Ye, LI Xuan-Ke, CUI Zheng-Wei, DONG Zhi-Jun, YUAN Guan-Ming.Hydrothermal Synthesis and Photocatalytic Activity of Partially Reduced Graphene Oxide/TiO2 Composite[J]. Acta Phys. -Chim. Sin., 2013,29(06): 1344-1350
71. HUANG Hai-Feng, JIA Jian-Ming, LU Han-Feng, ZHANG Hong-Hua, PAN Lie-Qun.Effect of Designed Zr/Ti Molar Ratio on the Photocatalytic Activity of Sr-Zr-Ti Mixed Oxide Catalysts under Visible Light[J]. Acta Phys. -Chim. Sin., 2013,29(06): 1319-1326
72. LIU Su-Qin, DAI Gao-Peng, LIANG Ying, LIU Hua-Jun, LIANG Gui-Jie.Fabrication and Visible-Light Photocatalytic Activity of In situ Carbon and Nitrogen Co-Doped TiO2 Hollow Sphere[J]. Acta Phys. -Chim. Sin., 2013,29(03): 585-589
73. ZHU Yan-Yan, LIU Yan-Fang, LÜ Yan-Hui, WANG Hua, LING Qiang, ZHU Yong-Fa.Reflux Preparation and Photocatalytic Performance of Bismuth Phosphate Nanorods[J]. Acta Phys. -Chim. Sin., 2013,29(03): 576-584
74. GAN Yong-Ping, QIN Huai-Peng, HUANG Hui, TAO Xin-Yong, FANG Jun-Wu, ZHANG Wen-Kui.Preparation and Photocatalytic Activity of Rutile TiO2-Graphene Composites[J]. Acta Phys. -Chim. Sin., 2013,29(02): 403-410
75. GUO Li-Mei, KUANG Yuan-Jiang, YANG Xiao-Dan, YU Yan-Long, YAO Jiang-Hong, CAO Ya-An.Photocatalytic Reduction of CO2 into CH4 Using SrB2O4 Catalyst[J]. Acta Phys. -Chim. Sin., 2013,29(02): 397-402
76. LIN Xue, GUAN Qing-Feng, LIU Ting-Ting, ZHANG Yao, ZOU Chun-Jie.Controllable Synthesis and Photocatalytic Activity of Bi4Ti3O12 Particles with Different Morphologies[J]. Acta Phys. -Chim. Sin., 2013,29(02): 411-417
77. YUAN Wen-Hui, LIU Xiao-Chen, LI Li.Improving Photocatalytic Performance for Hydrogen Generation over Co-Doped ZnIn2S4 under Visible Light[J]. Acta Phys. -Chim. Sin., 2013,29(01): 151-156
78. DING Zhi-Zhong, DONG Yong-Chun, LI Bing, LI Miao.Preparation of Grafted PTFE Fiber Metallic Complexes and Their Photocatalytic Degradation Abilities[J]. Acta Phys. -Chim. Sin., 2013,29(01): 157-166
79. CHEN Fu-Xiao, FAN Wei-Qiang, ZHOU Teng-Yun, HUANG Wei-Hong.Core-Shell Nanospheres (HP-Fe2O3@TiO2) with Hierarchical Porous Structures and Photocatalytic Properties[J]. Acta Phys. -Chim. Sin., 2013,29(01): 167-175
80. CHEN Wei, GAO Han-Yang, YANG Yu, LIN Pei-Bin, YUAN Jian, SHANGGUAN Wen-Feng, SU Jia-Chun, SUN Yang-Zhou.Polymerizable Complex Synthesis of Protonated Form of Layered Perovskite K0.5La0.5Bi2Ta2O9 for Water Splitting into Hydrogen[J]. Acta Phys. -Chim. Sin., 2012,28(12): 2911-2916
81. LONG Ming-Ce, WAN Lei, ZENG Ceng, LIU Yi-Yi, CHEN Yuan-Yuan.Enhanced Visible Light Activity of BiVO4 by Treating in HCl Aqueous Solution and Its Mechanism[J]. Acta Phys. -Chim. Sin., 2012,28(12): 2917-2923
82. YANG Xiao-Hong, TONG Qin, LIU Chang, LIU Jin-Ku, HE Wen-Zhi, LI Guang-Ming.Photocatalytic Properties of Aluminum Doped Zinc Oxide Nanocrystals Controlled Prepared via a Synergistic Ultrasonic/Hydrothermal Technique[J]. Acta Phys. -Chim. Sin., 2012,28(11): 2713-2720
83. ZHENG Hua-Rong, ZHANG Jin-Shui, WANG Xin-Chen, FU Xian-Zhi.Modification of Carbon Nitride Photocatalysts by Copolymerization with Diaminomaleonitrile[J]. Acta Phys. -Chim. Sin., 2012,28(10): 2336-2342
84. FAN Hai-Bin, ZHANG Dong-Feng, GUO Lin.Fabrication, Formation Mechanism and the Photocatalytic Properties of Hierarchical Porous Hematite Networks[J]. Acta Phys. -Chim. Sin., 2012,28(09): 2214-2220
85. WEN Wen, GAO Xiao-Ya, SONG Zhi-Ying, HAN Dong, WANG Juan, ZHU Mei-Xia, ZHANG Ai-Ping.Preparation of Magnetic Targeted Fe3O4-TiO2Nanoparticles and Their Photocatalytic Killing Effect on Hepatoma Carcinoma Cells[J]. Acta Phys. -Chim. Sin., 2012,28(09): 2221-2230
86. JI Ping-Li, WANG Jin-Gang, ZHU Xiao-Li, KONG Xiang-Zheng.Preparation of Silver Doped TiO2 Hollow Nanoparticles and Characterization of Their Structures and Photocatalytic Properties[J]. Acta Phys. -Chim. Sin., 2012,28(09): 2155-2161
87. DAI Gao-Peng, LIU Su-Qin, PENG Rong, LUO Tian-Xiong.Fabrication of Bi2O3/Bi2O3 Nanotube Arrays with High Visible-Light Photocatalytic Activity by Impregnation-Decomposition Method[J]. Acta Phys. -Chim. Sin., 2012,28(09): 2169-2174
88. LI Hui-Quan, CUI Yu-Min, WU Xing-Cai, HUA Lin, HONG Wen-Shan.Structure and Properties of BiOI/TiO2 (A) Photocatalysts with Different Bi/Ti Molar Ratios[J]. Acta Phys. -Chim. Sin., 2012,28(08): 1985-1991
89. LIN Xue, Lü Peng, GUAN Qing-Feng, LI Hai-Bo, LI Hong-Ji, CAI Jie, ZOU Yang.Visible Light Photocatalytic Properties of Bi3.25La0.75Ti3O12 Nanowires[J]. Acta Phys. -Chim. Sin., 2012,28(08): 1978-1984
90. ZHAO Peng-Jun, WU Rong, HOU Juan, CHANG Ai-min, GUAN Fang, ZHANG Bo.One-Step Hydrothermal Synthesis and Visible-Light Photocatalytic Activity of Ultrafine Cu-Nanodot-Modified TiO2 Nanotubes[J]. Acta Phys. -Chim. Sin., 2012,28(08): 1971-1977
91. BI Dong-Qin, XU Yi-Ming.Influence of Iron Oxide Doping on the Photocatalytic Degradation of Organic Dye X3B over Tungsten Oxide[J]. Acta Phys. -Chim. Sin., 2012,28(07): 1777-1782
92. LIN Xue, GUAN Qing-Feng, LI Hai-Bo, LI Hong-Ji, BA Chun-Hua, DENG Hai-De.Bi3.25Nd0.75Ti3O12 Nanostructures: Controllable Synthesis and Visible-Light Photocatalytic Activities[J]. Acta Phys. -Chim. Sin., 2012,28(06): 1481-1488
93. LIU Yan-Fang, MA Xin-Guo, YI Xin, ZHU Yong-Fa.Controllable Synthesis and Photocatalytic Performance of Bismuth Phosphate Nanorods[J]. Acta Phys. -Chim. Sin., 2012,28(03): 654-660
94. YU Chang-Lin, CAO Fang-Fang, SHU Qing, BAO Yu-Long, XIE Zhi-Peng, YU Jimmy C, YANG Kai.Preparation, Characterization and Photocatalytic Performance of Ag/BiOX (X=Cl, Br, I) Composite Photocatalysts[J]. Acta Phys. -Chim. Sin., 2012,28(03): 647-653
95. GAO Yue-Jun, XU Yi-Ming.Effect of Fluoride Doping and Adsorption on the Photocatalytic Activity of TiO2[J]. Acta Phys. -Chim. Sin., 2012,28(03): 641-646
96. LI Ai-Chang, LI Gui-Hua, ZHENG Yan, FENG Ling-Ling, ZHENG Yan-Jun.Photocatalytic Property and Reaction Mechanism of (Ni-Mo)/TiO2 Nano Thin Film Evaluated with Congo Red[J]. Acta Phys. -Chim. Sin., 2012,28(02): 457-464
97. LI Cao-Long, CHEN Wei, YUAN Jian, SHANGGUAN Wen-Feng.Hydrogen Evolution by Photocatalytic Steam Reforming of Methane over Pt/TiO2[J]. Acta Phys. -Chim. Sin., 2012,28(02): 450-456
98. CHEN Xiao-Yun, LU Dong-Fang, HUANG Jin-Feng, LU Yan-Feng, ZHENG Jian-Qiang.Preparation and Properties of N-F Co-Doped TiO2 Photocatalyst with Wide Range Light Response and Multipore Structure from Ionic Liquid-Water Mixture Solvent[J]. Acta Phys. -Chim. Sin., 2012,28(01): 161-169
99. YANG Xiao-Hong, LIU Chang, LIU Jin-Ku, ZHU Zi-Chun.Facile Synthesis of Assembly HAP Nanoribbon Spheres and the Synergized Action of Its Photocatalytic Properties[J]. Acta Phys. -Chim. Sin., 2011,27(12): 2939-2945
100. LI Ben-Xia, WANG Yan-Fen, LIU Tong-Xuan.Adjustable Synthesis and Visible-Light Responsive Photocatalytic Performance of V2O5·xH2O-BiVO4 Nanocomposites[J]. Acta Phys. -Chim. Sin., 2011,27(12): 2946-2952
101. CHEN Shu-Hai, XU Yao, LÜ Bao-Liang, WU Dong.Microwave-Assisted Hydrothermal Synthesis of Ag-Loaded Titania Nanotubes and Their Photocatalytic Performance[J]. Acta Phys. -Chim. Sin., 2011,27(12): 2933-2938
102. YAN Shi, HUANG Qin-Dong, LIN Jing-Dong, YUAN You-Zhu, LIAO Dai-Wei.Photocatalytic Activity of Cobalt Doped Titania for H2 Evolution[J]. Acta Phys. -Chim. Sin., 2011,27(10): 2406-2410
103. CUI Bai, LIN Hong, ZHAO Xiao-Chong, LI Jian-Bao, LI Wen-Di.Visible Light Induced Photocatalytic Activity of ZnCo2O4 Nanoparticles[J]. Acta Phys. -Chim. Sin., 2011,27(10): 2411-2415
104. XIA Hui-Yun, ZHANG Ying, GAO Li-Ning, YAN Lu-Ke.Ag-P(AM-co-MAA) Composite Microspheres Based on Morphology Transcription Method[J]. Acta Phys. -Chim. Sin., 2011,27(10): 2485-2492
105. LU Sheng-Yong, HUANG Yi-Long, WANG Qiu-Lin, LI Xiao-Dong, YAN Jian-Hua.Photocatalytic Degradation of Gaseous 1,2-Dichlorobenzene over TiO2/AC Photocatalysts[J]. Acta Phys. -Chim. Sin., 2011,27(09): 2191-2199
106. TONG Xin, CHEN Rui, CHEN Tie-Hong.Photocatalytic Activity of TiO2 with Micrometer-Sized Macropores[J]. Acta Phys. -Chim. Sin., 2011,27(08): 1941-1946
107. LI You-Ji, CHEN Wei, LI Lei-Yong.Effects of Surface Areas and Adsorption Strength on the Photoactivity and Decomposition Kinetics of Acid Red 27 over TiO2-Coated/Activated Carbon Composites[J]. Acta Phys. -Chim. Sin., 2011,27(07): 1751-1756
108. QIU Wei, REN Cheng-Jun, GONG Mao-Chu, HOU Yun-Ze, CHEN Yao-Qiang.Structure, Surface Properties and Photocatalytic Activity of TiO2 and TiO2/SiO2 Catalysts Prepared at Different pH Values[J]. Acta Phys. -Chim. Sin., 2011,27(06): 1487-1492
109. CONG Ye, QIN Yun, LI Xuan-Ke, DONG Zhi-Jun, YUAN Guan-Ming, CUI Zheng-Wei.Preparation and Visible Light Photocatalytic Activity of Titanium Dioxide Coated Multiwalled Carbon Nanotubes[J]. Acta Phys. -Chim. Sin., 2011,27(06): 1509-1515
110. YING Hong, WANG Zhi-Yong, GUO Zheng-Duo, SHI Zu-Jin, YANG Shang-Feng.Reduced Graphene Oxide-Modified Bi2WO6 as an Improved Photocatalyst under Visible Light[J]. Acta Phys. -Chim. Sin., 2011,27(06): 1482-1486
111. CHEN Jin-Yi, LI Nian, LI Jing, ZHU Liang, PENG Chang-Jun.Synthesis and Visible Light Photocatalytic Activity of Cross-Linked Sodium Rectorite/Cu2O Nanocomposites[J]. Acta Phys. -Chim. Sin., 2011,27(04): 932-938
112. YU Chang-Lin, YANG Kai, YU Jimmy C, PENG Peng, CAO Fang-Fang, LI Xin, ZHOU Xiao-Chun.Effects of Rare Earth Ce Doping on the Structure and Photocatalytic Performance of ZnO[J]. Acta Phys. -Chim. Sin., 2011,27(02): 505-512
113. XIE Juan, WANG Hu, DUAN Ming.Controlled Growth of Self-Assembled ZnO Thin Films and Characterization of Their Photocatalytic Properties[J]. Acta Phys. -Chim. Sin., 2011,27(01): 193-198
114. WU Da-Wang, LI Shuo, CHEN Yao-Qiang, GONG Mao-Chu, ZHANG Qiu-Lin, LIU Kang-Lian, WANG Yu-Lin.Photocatalytic Degradation of Gas Phase Benzene over WO3/Bi12SiO20[J]. Acta Phys. -Chim. Sin., 2010,26(12): 3299-3304
115. ZHANG Xiao-Ru, LIN Yan-Hong, ZHANG Jian-Fu, HE Dong-Qing, WANG De-Jun.Photoinduced Charge Carrier Properties and Photocatalytic Activity of N-Doped TiO2 Nanocatalysts[J]. Acta Phys. -Chim. Sin., 2010,26(10): 2733-2738
116. DU Huan, WANG Sheng, LIU Lian-Lian, LIU Zhong-Xiang, LI Zhen, LU Nan, LIU Fu-Sheng.Preparation, Characterization and Photocatalytic Property of p-CoO/n-CdS Compound Semiconductor Photocatalyst[J]. Acta Phys. -Chim. Sin., 2010,26(10): 2726-2732
117. GAO Guan-Dao, LI Jing, ZHANG Ai-Yong, AN Xiao-Hong, ZHOU Lei.Optimizational Preparation and Mesoporous Material Characteristics of a Novel Biomimetic Photocatalyst and Its Application to the Photocatalytic Degradation of Phenol[J]. Acta Phys. -Chim. Sin., 2010,26(09): 2437-2442
118. XU Ping-Chang, LIU Yang, WEI Jian-Hong, XIONG Rui, PAN Chun-Xu, SHI Jing.Solvothermal Preparation of Ag/TiO2 Nanoparticles and Their Photocatalytic Activity[J]. Acta Phys. -Chim. Sin., 2010,26(08): 2261-2266
119. LI Li, LU Dan, JI Yuan, ZHAO Yue-Hong.Preparation of Nanocomposite Ag/TiO2-ZrO2 and the Microwave Enhanced Photocatalytic Degradation of Methyl Orange[J]. Acta Phys. -Chim. Sin., 2010,26(05): 1323-1329
120. ZHANG Shu-Cui, JIANG Dong, TANG Tao, LI Jun-Hua, XU Yao.Synthesis and Photocatalytic Activity of Highly Dispersed TiO2/SBA-15[J]. Acta Phys. -Chim. Sin., 2010,26(05): 1330-1336
121. ZHANG Ai-Ping, ZHANG Jin-Zhi.Syntheses and Activities of Visible-Light-Driven Cu/BiVO4 Composite Photocatalysts[J]. Acta Phys. -Chim. Sin., 2010,26(05): 1337-1342
122. LI Zhao-Hui, LIU Ping, FU Xian-Zhi.Wide Bandgap p-Block Metal Oxides/Hydroxides for Photocatalytic Benzene Degradation[J]. Acta Phys. -Chim. Sin., 2010,26(04): 877-884
123. DEDG Pei-Chang, HU Jie-Zhen, WANG Hai-Zeng, SUN Bao-Wei.Hydrothermal Preparation and Photocatalytic Activity of Chlorine Doped Titanium Dioxide Supported on SiO2[J]. Acta Phys. -Chim. Sin., 2010,26(04): 915-920
124. ZHAI Xiao-Hui, LONG Hui-Jin, DONG Jiang-Zhou, CAO Ya-An.Doping Mechanism of N-TiO2/ZnO Composite Nanotube Arrays and Their Photocatalytic Activity[J]. Acta Phys. -Chim. Sin., 2010,26(03): 663-668
125. ZHANG Qiong, HE Yun-Qiu, CHEN Xiao-Gang, HU Dong-Hu, LI Lin-Jiang, YIN Ting, JI Ling-Li.Intercalated Structure and Photocatalytic Properties of TiO2-Graphite Oxide Composite[J]. Acta Phys. -Chim. Sin., 2010,26(03): 654-662
126. XU Xin, WANG Xiao-Jing, HU Zhong-Hua, LIU Ya-Fei, WANG Chen-Chen, ZHAO Guo-Hua.Influence of Sol-Gel and Dip-Hydrothermal Preparation Methods on Structure and Performance of TiO2/AC Photocatalysts[J]. Acta Phys. -Chim. Sin., 2010,26(01): 79-86
127. WANG Meng-Ye, WANG Cheng-Lin, XIE Kun-Peng, SUN Lan, LIN Chang-Jian.Fabrication of a Spongelike Nanostructured TiO2 Filmand Its Photocatalytic Activity[J]. Acta Phys. -Chim. Sin., 2009,25(12): 2475-2480
128. LI Ben-Xia, WANG Yuan-Yuan, WANG Yan-Fen.Facile Synthesis and Photocatalytic Property of CuO Nanostructure Arrays[J]. Acta Phys. -Chim. Sin., 2009,25(11): 2366-2372
129. ZHOU Bo, LIU Zhi-Guo, WANG Hong-Xia, HUANG Xi-Qiang, SUI Yu, WANG Xian-Jie, LV Zhe, SU Wen-Hui.Hydrothermal Preparation and Visible Photocatalytic Activity of Flower-Like Cu2O/Cu Nanocomposites[J]. Acta Phys. -Chim. Sin., 2009,25(09): 1841-1846
130. ZHANG Xiao-Yan, CUI Xiao-Li.Preparation and Photocatalytic Hydrogen Evolution Performance of C-N Co-doped Nano TiO2 Photocatalysts[J]. Acta Phys. -Chim. Sin., 2009,25(09): 1829-1834
131. DU Wei-Ping, LI Zhen, LENG Wen-Hua, XU Yi-Ming.Photocatalytic Reduction of Silver Ions on Ferric Oxides and Ferric Hydroxides[J]. Acta Phys. -Chim. Sin., 2009,25(08): 1530-1534
132. LI Chang-Yu, LIU Shou-Xin, MA Yue.Preparation of Visible-Light Response Cu-Cu2+1O Composites by a One-Step Hydrothermal Method[J]. Acta Phys. -Chim. Sin., 2009,25(08): 1555-1560
133. SU Bi-Tao, SUN Jia-Xing, HU Chang-Lin, ZHANG Xiao-Hong, FEI Peng, LEI Zi-Qiang.Preparation and Characterization of Fe3+-Doped TiO2 Photocatalytic Fiber Materials[J]. Acta Phys. -Chim. Sin., 2009,25(08): 1561-1566
134. WANG Qi-Zhao, JIANG Li, LIU Hui, YUAN Jian, CHEN Ming-Xia, SHI Jian-Wei, SHANGGUAN Wen-Feng.Preparation and Characterization of Bi1-xGdxVO4 Photocatalyst and Its Application toWater Splitting[J]. Acta Phys. -Chim. Sin., 2009,25(08): 1703-1707
135. LI Li, MA Yu, CAO Yan-Zhen, JI Yuan, GUO Yi-Hang.Preparation of Periodic Mesoporous H6P2W18O62/TiO2(Brij-76) Composite and Microwave Enhanced Photocatalytic Degradation of Monochlorobenzene[J]. Acta Phys. -Chim. Sin., 2009,25(07): 1461-1466
136. FENG Li-Li, ZHAO Wei, LIU Yang, JIAO Liang, LI Xing-Guo.Photocatalytic Degradation of Rhodamine B by Nanocrystalline TiO2 Loaded into MCM-41 Molecular Sieves[J]. Acta Phys. -Chim. Sin., 2009,25(07): 1347-1351
137. MIN Shi-Xiong, WANG Fang, ZHANG Zhen-Min, HAN Yu-Qi, FENG Lei.Preparation and Photocatalytic Activity of PANI/AMTES-TiO2 Nanocomposite Materials[J]. Acta Phys. -Chim. Sin., 2009,25(07): 1303-1310
138. LEI Jian-Fei, LI Wei-Shan.Photoelectrocatalytic Performance of Arrayed Porous TiO2/Ti[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1173-1178
139. CAO Yong-Qiang, LONG Hui-Jin, CHEN Yong-Mei, CAO Ya-An.Photocatalytic Activity of TiO2 Films with Rutile/Anatase Mixed Crystal Structures[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1088-1092
140. CHEN Wei, DONG Xin-Fa, CHEN Zhi-Shan, CHEN Sheng-Zhou, LIN Wei-Ming.Effect of Fe3+ Doping on Photocatalytic Activity of K2La2Ti3O10 for Water Decomposition to Hydrogen under Visible Light[J]. Acta Phys. -Chim. Sin., 2009,25(06): 1107-1110
141. SHEN Jing-Jing, LIU Chang, ZHU Yu-Dan, LI Wei, FENG Xin, LU Xiao-Hua.Photocatalytic Properties of Mesoporous TiO2 Prepared by Hydrothermal Method[J]. Acta Phys. -Chim. Sin., 2009,25(05): 1013-1018
142. CHEN Qi-Feng, JIANG Dong, XU Yao, WU Dong, SUN Yu-Han.Visible Region Photocatalysis of Ce-Si/TiO2 Synthesized Using Sol-Gel-Hydrothermal Method[J]. Acta Phys. -Chim. Sin., 2009,25(04): 617-623
143. HU Yuan-Fang; LI Yue-Xiang; PENG Shao-Qin; LV Gong-Xuan; LI Shu-Ben.Photocatalytic Properties of Composite of SiO2 and Pt-Cd0.53Zn0.47S Solid Solutions[J]. Acta Phys. -Chim. Sin., 2008,24(11): 2071-2076
144. LI Xiao-Hui, LIU Shou-Xin.Characterization of Visible Light Response N-F Codoped TiO2 Photocatalyst Prepared by Acid Catalyzed Hydrolysis[J]. Acta Phys. -Chim. Sin., 2008,24(11): 2019-2024
145. WANG Wei-Cheng, LI Shuo, WEN Yi-Yun, GONG Mao-Chu, ZHANG Lei, YAO Yan-Ling, CHEN Yao-Qiang.Synthesis and Characterization of TiO2/YFeO3 and Its Photocatalytic Oxidation of Gaseous Benzene[J]. Acta Phys. -Chim. Sin., 2008,24(10): 1761-1766
146. CHEN Yu-Juan; HU Zhong-Hua; WANG Xiao-Jing; ZHAO Guo-Hua; LIU Ya-Fei; LIU Wei.Influence of Pore Size and Surface Area of Activated Carbon on the Performance of TiO2/AC Photocatalyst[J]. Acta Phys. -Chim. Sin., 2008,24(09): 1589-1596
147. LIU Ding, XU Yi-Ming.Reaction Mechanism on the Synergistic Photodegradation of Dye X3B and Photoreduction of Dichromate in the Presence of Polyoxometalate[J]. Acta Phys. -Chim. Sin., 2008,24(09): 1584-1588
148. SUN Yi; XU Juan; CAI Wen-Bin; JIANG Zhi-Yu.Mechanism of Photokilling LoVo Cells by Nano TiO2 Photocatalytic Oxidation Combined with Immunity and Electroporation Method[J]. Acta Phys. -Chim. Sin., 2008,24(08): 1359-1365
149. LI Hai-Long; LUO Wu-Lin; CHEN Tao; TIAN Wen-Yu; SUN Mao; LI Chun; ZHU Di; LIU Ran-Ran; ZHAO Yu-Liang; LIU Chun-Li.Preparation and Photocatalytic Performance of Titania Nanotubes Loaded with Ag Nanoparticles[J]. Acta Phys. -Chim. Sin., 2008,24(08): 1383-1386
150. SHI Jian; LI Jun; CAI Yun-Fa.Fabrication of C, N-Codoped TiO2 Nanotube Photocatalysts with Visible Light Response[J]. Acta Phys. -Chim. Sin., 2008,24(07): 1283-1286
151. XU Di; GAO Ai-Mei; DENG Wen-Li.Self-Assembly and Photocatalytic Properties of Clustered and Flowerlike CdS Nanostructures[J]. Acta Phys. -Chim. Sin., 2008,24(07): 1219-1224
152. PAN Hai-Bo; WANG Fang; HUANG Jin-Ling; CHEN Nai-Sheng.Binding Characteristics of CoPc/SnO2 by In-situ Process and Photocatalytic Activity under Visible Light Irradiation[J]. Acta Phys. -Chim. Sin., 2008,24(06): 992-996
153. LI Jin-Huan; KANG Wan-Li; YAN Wen-Hua; GUO Yi-Hang; GAO Hong-Feng; LIU Zhong-He.Preparation of Eu3+ Doped Titania Nanocrystals and Photocatalytic Degradation Partially Hydrolyzed Polyacrylamide[J]. Acta Phys. -Chim. Sin., 2008,24(06): 1030-1034
154. LUO Da-Chao; ZHANG Lan-Lan; LONG Hui-Jin; CHEN Yong-Mei; CAO Ya-An.Effect of Surface Modification by Ni2+ on Photocatalysis Activity of TiO2[J]. Acta Phys. -Chim. Sin., 2008,24(06): 1095-1099
155. FENG Cai-Xia; WANG Yan; JIN Zhen-Sheng; ZHANG Shun-Li.Kinetic Behavior of Visible Light Photocatalytic Oxidation of Propylene for N-Doped Nano-TiO2[J]. Acta Phys. -Chim. Sin., 2008,24(04): 633-638
156. LU Han-Feng; ZHOU Ying; XU Bo-Qing; CHEN Yin-Fei; LIU Hua-Zhang.Effect of Gold Doping on the Photocatalytic Activity of the Anatase TiO2[J]. Acta Phys. -Chim. Sin., 2008,24(03): 459-464
157. LIU Shou-Xin; CHEN Xiao-Yun.Effect of Pore Structure of Activated Carbon on the Photocatalytic Activity of TiO2/AC Composite Photocatalyst[J]. Acta Phys. -Chim. Sin., 2008,24(03): 533-538
158. WU Yu-Cheng; LIU Xiao-Lu; YE Min; XIE Ting; HUANG Xin-Min.Preparation and Properties of Carbon Nanotube-TiO2 Nanocomposites[J]. Acta Phys. -Chim. Sin., 2008,24(01): 97-102
159. LIU Fu-Sheng; JI Ren; WU Min; SUN Yue-Ming.Hydrogen Production from Water Splitting Using Perylene Dye-Sensitized Pt/TiO2 Photocatalyst[J]. Acta Phys. -Chim. Sin., 2007,23(12): 1899-1904
160. CHEN Qi-Yuan; TONG Hai-Xia; YIN Zhou-Lan; HU Hui-Ping; LI Jie; LIU Liang-Liang.Preparation, Characterization and Photo-catalytic Behavior of TiO2 Catalysts with Oxygen Vacancies[J]. Acta Phys. -Chim. Sin., 2007,23(12): 1917-1921
161. ZHANG Tian-Yong; FAN Qiao-Fang; ZENG Miao; WANG Zheng; XIA Wen-Juan; CHI Li-Feng.Photocatalytic Degradation of Light Fast Scarlet BBN and Surfactant Bicomponents[J]. Acta Phys. -Chim. Sin., 2007,23(11): 1803-1807
162. ZHANG Wei; WANG Shu-Liang; MA Yun-Qing; WANG Cui-Ping; LIU Xing-Jun.Influence of Interface Diffusion between Al Substrate and TiO2 Filmon Photocatalytic Activity[J]. Acta Phys. -Chim. Sin., 2007,23(09): 1347-1352
163. ZHOU Xue-Feng; LI Wei; ZHANG Yan; YANG Zhu-Hong; FENG Xin; LU Xiao-Hua.Hole Oxidation on TiO2 Films in Aqueous Solutions Studied by Using OTS SAMs as a Probe[J]. Acta Phys. -Chim. Sin., 2007,23(07): 1113-1116
164. TIAN Bao-Zhu; TONG Tian-Zhong; CHEN Feng; ZHANG Jin-Long.Effect of Water Washing Treatment on the Photocatalytic Activity of Au/TiO2 Catalysts[J]. Acta Phys. -Chim. Sin., 2007,23(07): 978-982
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