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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 2017,Vol.33>> Issue(5)>> 968-975     doi: 10.3866/PKU.WHXB201702093         中文摘要
Preparation of Biochar from Different Biomasses and Their Application in the Li-S Battery
LI Jun-Tao1, WU Jiao-Hong1, ZHANG Tao1, HUANG Ling2
1 College of Energy, Xiamen University, Xiamen 361005, Fujian Province, P. R. China;
2 College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, Fujian Province, P. R. China
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Biochar derived from reproducible massive biomasses presents the advantages of low cost and renewable resources. In this work aiming to solve the existing problems of the lithium-sulfur battery, sulfur@biochar (S@biochar) composite cathode materials with high capacity and good cycle performance were developed. Specifically, four kinds of biochar prepared from rice husk, miscanthus, fir, and pomelo peel were used as host matrices for the Li-S battery. Among them, the S@biochar derived from rice husk delivered the highest specific capacity and the best cycle stability according to electrochemical tests. To further optimize its performance, we prepared a highly porous rice husk derived biochar (HPRH-biochar) using silica gel as the template. The S@HPRH-biochar composite (60% (w, mass fraction) S) enables the homogeneous dispersion of amorphous sulfur in the carbon matrix and its porous structure could effectively suppress the dissolution of the polysulfide. As a result, its electrochemical performance improved, achieving a high initial charge capacity of 1534.1 mAh·g-1 and maintaining a high capacity of 738.7 mAh·g-1 after 100 cycles at 0.2C (1C corresponds to a current density of 1675 mA·g-1). It also gives a capacity of 485.3 mAh·g-1 at 2.0C in the rate capacity test.



Keywords: Li/S battery   Composite   Rice husk   Miscanthus   Fir   Pomelo peel  
Received: 2016-12-28 Accepted: 2017-02-03 Publication Date (Web): 2017-02-09
Corresponding Authors: LI Jun-Tao Email: jtli@xmu.edu.cn

Fund: The project was supported by the National Natural Science Foundation of China (21373008) and Fundamental Research Funds for the Central Universities, China (20720160124).

Cite this article: LI Jun-Tao, WU Jiao-Hong, ZHANG Tao, HUANG Ling. Preparation of Biochar from Different Biomasses and Their Application in the Li-S Battery[J]. Acta Phys. -Chim. Sin., 2017,33 (5): 968-975.    doi: 10.3866/PKU.WHXB201702093

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