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ISSN 1000-6818CN 11-1892/O6CODEN WHXUEU
Acta Phys Chim Sin >> 0,Vol.>> Issue()>> 0-0     doi: 10.3866/PKU.WHXB201709131         中文摘要
Accepted manuscript
Morphology Control of Non-fullerene Blend Systems Based on Perylene Diimide Acceptors
HAN Jie1, LIANG Qiuju2,3, QU Yi1,4, LIU Jiangang2, HAN Yanchun2
1 State Key Laboratory of High Power Semiconductor Laser;Changchun University of Science and Technology, Changchun 130022, P. R. China;
2 State Key Laboratory of Polymer Physics and Chemistry;Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, P. R. China;
3 University of the Chinese Academy of Sciences, Beijing 100049, P. R. China;
4 College of Physics & Electronic Engineering;Hainan Normal University, Haikou 571158, P. R. China
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In recent years, the development of perylene diimide derivative (PDI)-based non-fullerene organic solar cells has been extensively studied. These solar cells exhibit unique advantages such as complementary light absorption, tunable energy levels, excellent electron transport properties, and relatively low cost. However, the strong π-π stacking between the PDI molecules tends to induce an uncontrolled phase separation structure, large domain size, and an unmanageable mixed phase, leading to severe geminate and non-geminate recombination and restriction of the final power conversion efficiency of the non-fullerene-based systems. In this work, it was found that one of the most important parameters that helps regulate phase structure is the molecular diffusion rate. By tuning the thermal annealing and liquid-solid phase separation and blend ratio, the phase-separated structure could be adjusted. Further, the domain size of blend systems with different compatibilities was regulated by balancing the π-π and charge transfer interactions. In addition, the amount of the intermixed phase was controlled by tuning the solubility parameter difference (△δ) between the solvent and the solute.



Keywords: Solar cells   Nonfullerene   Morphology control   Phase separation   Domain size   Intermixed phase  
Received: 2017-08-11 Accepted: 2017-09-07 Publication Date (Web): 2017-09-13
Corresponding Authors: QU Yi, LIU Jiangang, HAN Yanchun Email: 2686566673@qq.com;niitawh@ciac.ac.cn;ychan@ciac.ac.cn

Fund: The project was supported by the National Natural Science Foundation of China (51573185, 21334006, 21474113) and the Strategic Priority Research Program of the Chinese Academy of Sciences (XDB12020300).

Cite this article: HAN Jie, LIANG Qiuju, QU Yi, LIU Jiangang, HAN Yanchun. Morphology Control of Non-fullerene Blend Systems Based on Perylene Diimide Acceptors[J]. Acta Phys. -Chim. Sin., 0, (): 0-0.    doi: 10.3866/PKU.WHXB201709131

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9. LIU Yan-Ping, WU Yi-Shi, FU Hong-Bing.Recent Progress in Singlet Exciton Fission[J]. Acta Phys. -Chim. Sin., 2016,32(8): 1880-1893
10. HUANG Chang-Shui, LI Yu-Liang.Structure of 2D Graphdiyne and Its Application in Energy Fields[J]. Acta Phys. -Chim. Sin., 2016,32(6): 1314-1329
11. XU Guo-Cheng, DENG Xian-Yun, LI Jun-Li, ZHANG Rui, XIE Yun-Peng, TU Guo-Li, XIA Jiang-Bin, LU Xing.Lead Iodide as a New Type of Hole Transport Layer for the High Performance of P3HT:PC61BM-Based Solar Cells[J]. Acta Phys. -Chim. Sin., 2016,32(6): 1307-1313
12. SHI Ji-Fu, HUANG Qi-Zhang, WAN Qing-Cui, XU Xue-Qing, LI Chun-Sheng, XU Gang.Sulfide-Based Ionic Liquid Electrolyte Widening the Application Temperature Range of Quantum-Dot-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2016,32(4): 822-827
13. WANG Li-Juan, LI Qi, HAO Yan-Zhong, SHEN Shi-Gang, XU Dong-Sheng.Improvement of Quantum Dot Coverage of CdS/CdSe/TiO2 Hierarchical Hollow Sphere Photoanodes[J]. Acta Phys. -Chim. Sin., 2016,32(4): 983-989
14. HE Rong-An, CAO Shao-Wen, YU Jia-Guo.Recent Advances in Morphology Control and Surface Modification of Bi-Based Photocatalysts[J]. Acta Phys. -Chim. Sin., 2016,32(12): 2841-2870
15. WEI Hui-Yun, WANG Guo-Shuai, WU Hui-Jue, LUO Yan-Hong, LI Dong-Mei, MENG Qing-Bo.Progress in Quantum Dot-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2016,32(1): 201-213
16. HOU Li-Mei, WEN Zhi, LI Yin-Xiang, HU Hua-You, KAN Yu-He, SU Zhong-Min.Molecular Design of Indolizine Derivative as Sensitizers for Organic Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2015,31(8): 1504-1512
17. LI Hui, LIU Xiang-Xin, ZHANG Yu-Feng, DU Zhong-Ming, YANG Biao, HAN Jun-Feng, BESLAND Marie-Paule.Synthesis of CdS with Large Band Gap Values by a Simple Route at Room Temperature[J]. Acta Phys. -Chim. Sin., 2015,31(7): 1338-1344
18. WU Na, LUO Qun, WU Zhen-Wu, MA Chang-Qi.Influence of Electrode Interfacial Buffer Layers on Thermal Stability of P3HT:PC61BM Solar Cells[J]. Acta Phys. -Chim. Sin., 2015,31(7): 1413-1420
19. KOU Yan-Lei, QU Sheng-Chun, LIU Kong, CHI Dan, LU Shu-Di, LI Yan-Pei, YUE Shi-Zhong.Development of Cd-Based Compound Nanocrystal-Organic Polymer Hybrid Solar Cells[J]. Acta Phys. -Chim. Sin., 2015,31(5): 807-816
20. WANG Yu-Qiao, WANG Pan-Pan, LU Jing, BAI Yi-Chao, GU Yun-Liang, SUN Yue-Ming.Dye-Sensitized Solar Cells Based on MWCNT/TiO2 Counter Electrode and Thiolate/Disulfide Non-Iodine Redox Couple[J]. Acta Phys. -Chim. Sin., 2015,31(3): 448-456
21. BAI Xiao-Gong, SHI Yan-Tao, WANG Kai, DONG Qing-Shun, XING Yu-Jin, ZHANG Hong, WANG Liang, MA Ting-Li.Synthesis of CH3NH3SrxPb(1-x)I3 with Less Pb Content and Its Application in All-Solid Thin Film Solar Cells[J]. Acta Phys. -Chim. Sin., 2015,31(2): 285-290
22. ZHANG Jing-Bo, LI Pan, YANG Hui, ZHAO Fei-Yan, TANG Guang-Shi, SUN Li-Na, LIN Yuan.Preparation of a Highly Efficient PbS Electrode and Its Application in Quantum Dots-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2014,30(8): 1495-1500
23. GAO Su-Wen, LAN Zhang, WU Wan-Xia, QUE Lan-Fang, WU Ji-Huai, LIN Jian-Ming, HUANG Miao-Liang.Fabrication and Photovoltaic Performance of High Efficiency Front-Illuminated Dye-Sensitized Solar Cell Based on Ordered TiO2 Nanotube Arrays[J]. Acta Phys. -Chim. Sin., 2014,30(3): 446-452
24. CHEN Xi-Ming, JIA Chun-Yang, WAN Zhong-Quan, YAO Xiao-Jun.Theoretical Investigations of Tetrathiafulvalene Derivative as Electron Donor in Organic Dye for Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2014,30(2): 273-280
25. ZHU De-Hua, ZHONG Rong, CAO Yu, PENG Zhi-Hui, FENG Ai-Xin, XIANG Wei-Dong, ZHAO Jia-Long.Size-Dependent Electron Injection and Photoelectronic Properties of CuInS2 Quantum Dot Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2014,30(10): 1861-1866
26. ZHU Lei, QIANG Ying-Huai, ZHAO Yu-Long, GU Xiu-Quan, SONG Duan-Ming, SONG Chang-Bin.Facile Synthesis of Cu2SnSe3 as Counter Electrodes for Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2013,29(11): 2339-2344
27. LI Wen-Zhe, WANG Li-Duo, GAO Rui, DONG Hao-Peng, NIU Guang-Da, GUO Xu-Dong, QIU Yong.Transforming Organic Ligands into a ZnS Protective Layer through the S2- Intermediate State in ex situ CdSe Quantum Dot Devices[J]. Acta Phys. -Chim. Sin., 2013,29(11): 2345-2353
28. GUO Xu-Dong, Ma Bei-Bei, WANG Li-Duo, GAO Rui, DONG Hao-Peng, QIU Yong.Electron Injection and Photovoltaic Properties in CdSe/ZnS Quantum Dot Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2013,29(06): 1240-1246
29. YANG Gui-Jun, WANG Shen-Rui, ZHANG Yong-Chang, WANG Gang, CHEN Hui-Yuan, NAN Hui, LIN Hong.Effect of pH Values on Performance of Trollius Chinensis Pigment Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2013,29(03): 539-545
30. WANG Hai, XU Xue-Qing, SHI Ji-Fu, XU Gang.Application of Ionic Liquids with Carboxyl and Aromatic Ring Conjugated Anions in Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2013,29(03): 525-532
31. WANG Sha-Sha, LU Shan, SU Jia, GUO Zheng-Kai, LI Xue-Min, ZHANG Xue-Hua, HE Sheng-Tai, HE Tao.Influences of Polymerization Time on Structure and Properties of Polyaniline Counter Electrodes in Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2013,29(03): 516-524
32. ZHAN Wei-Shen, LI Rui, PAN Shi, GUO Ying-Nan, ZHANG Yi.Extension of Conjugate π Bridge in Dye Molecules for Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2013,29(02): 255-262
33. GUO Wei, WANG Kai, SHEN Yi-Hua, ZHANG He, WENG Tao, MA Ting-Li.A Simple Template Synthesis of Hierarchically Mesoporous TiO2 Microsphere for Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2013,29(01): 82-88
34. DAI Yu-Hua, LI Xiao-Jie, FANG Yan-Yan, SHI Qiu-Fei, LIN Yuan, YANG Ming-Shan.Influence of Polymer Gel Electrolyte on the Performance of Dye-Sensitized Solar Cells Analyzed by Electrochemical Impedance Spectroscopy[J]. Acta Phys. -Chim. Sin., 2012,28(11): 2669-2675
35. JIANG Li-Lin, LU Xi-Yin, SONG Yun-Fei, LIU Wei-Long, YANG Yan-Qiang.Effects of Excited State Vibrational Coherence on Photo-Induced Electron Transfer Rates in Dye-Sensitized Nanocrystalline TiO2[J]. Acta Phys. -Chim. Sin., 2012,28(11): 2589-2596
36. JIAO Shu-Hong, XU Dong-Sheng, XU Li-Fen, ZHANG Xiao-Guang.Recent Progress in Electrochemical Synthesis and Morphological Control of Metal Oxide Nanostructures[J]. Acta Phys. -Chim. Sin., 2012,28(10): 2436-2446
37. LIANG Gui-Jie, ZHONG Zhi-Cheng, XU Jie, XU Wei-Lin, CHEN Mei-Hua, ZHANG Zeng-Chang, LI Wen-Lian.Formation Mechanism, Structure Model and Electrochemical Performance of an In situ Cross Linking Hybrid Polymer Electrolyte Membrane[J]. Acta Phys. -Chim. Sin., 2012,28(09): 2057-2064
38. LIANG Gui-Jie, ZHONG Zhi-Cheng, CHEN Mei-Hua, XU Jie, XU Wei-Lin, HE Ping, HOU Qiu-Fei, LI Zai-Fang.Effect of Donor Moieties on the Electronic Structures and Absorption Spectra of Indoline Dyes[J]. Acta Phys. -Chim. Sin., 2012,28(08): 1885-1891
39. CHU Ling-Ling, GAO Yu-Rong, WU Ming-Xing, WANG Lin-Lin, MA Ting-Li.Fabrication and Application of a Carbon Counter Electrode with Excellent Adhesion Properties for Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2012,28(07): 1739-1744
40. LI Xiao-Ning, BAI Shou-Li, YANG Wen-Sheng, CHEN Ai-Fan, SUN Li-Na, LIN Yuan, ZHANG Jing-Bo.Electron Transport Properties of One-Dimensional Structural SnO2 Belts[J]. Acta Phys. -Chim. Sin., 2012,28(07): 1797-1802
41. CHANG Meng-Lei, LI Xin-Jun.Fabrication of Nanosheet/Nestlike Nanoarray Hierarchical TiO2 Film for Dye-Sensitized Solar Cell[J]. Acta Phys. -Chim. Sin., 2012,28(06): 1368-1372
42. LI Dan, LIANG Ran, YUE He, WANG Peng, FU Li-Min, ZHANG Jian-Ping, AI Xi-Cheng.Influence of Donor and Acceptor Mass Ratios on P3HT:PCBM Film Structure and Device Performance[J]. Acta Phys. -Chim. Sin., 2012,28(06): 1373-1379
43. WANG Hui, XI Yan-Yan, ZHOU Jian-Zhang, LIN Zhong-Hua.Electrochemical Synthesis of CdS Nanocrystals on a Gold Electrode Modified with a p-Aminothiophenol Self-Assembled Monolayer[J]. Acta Phys. -Chim. Sin., 2012,28(06): 1398-1404
44. ZHANG Ren-Kai, SUN Zhe, XIE Huan-Huan, LIANG Mao, XUE Song.New Comb-Like Copolymer for Quasi-Solid Electrolyte Based Dye-Sensitized Solar Cells and Its Effects on Electron Recombination[J]. Acta Phys. -Chim. Sin., 2012,28(05): 1139-1145
45. ZHOU Wei, HUANG Qi-Yu, WANG Xiao-Chen, QI Fang-Yi, JIAO Fang, ZHENG Yi-Zhou.Fabrication and Characterization of Quasi-Solid-State Electrolyte Films Based on Polyvinyl Butyral[J]. Acta Phys. -Chim. Sin., 2012,28(05): 1134-1138
46. SHI Ji-Fu, FAN Ye, XU Xue-Qing, XU Gang, CHEN Li-Hua.Influence of Preparation Conditions on the Properties of Cu2S Photocathodes[J]. Acta Phys. -Chim. Sin., 2012,28(04): 857-864
47. GUO Xue-Yi, YI Peng-Fei, WANG Wei-Jia, YANG Ying.Electrochemical Properties of an Agarose-Based Magnetic Polymer Electrolyte in Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2012,28(03): 585-590
48. XIAO Yao-Ming, WU Ji-Huai, YUE Gen-Tian, LIN Jian-Ming, HUANG Miao-Liang, FAN Le-Qing, LAN Zhang.Preparation of Single-Crystalline TiO2 Nanowires and Their Application in Flexible Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2012,28(03): 578-584
49. ZHAN Wei-Shen, PAN Shi, WANG Qiao, LI Hong, ZHANG Yi.Comparison of D-SS and D-ST Dyes as Photo Sensitizers in Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2012,28(01): 78-84
50. WANG Xin-Chun, HU Bin-Bin, WANG Guang-Jun, YANG Guang-Hong, WAN Shao-Ming, DU Zu-Liang.Preparation of CIGS Thin Films by Electrodeposition Method Using Ethanol as a Solvent[J]. Acta Phys. -Chim. Sin., 2011,27(12): 2826-2830
51. CAI Qian, LIANG Xiao-Juan, ZHONG Jia-Song, SHAO Ming-Guo, WANG Yun, ZHAO Xiao-Wei, XIANG Wei-Dong.Synthesis and Characterization of Sphere-Like Cu2ZnSnS4 Nanocrystals by Solvothermal Method[J]. Acta Phys. -Chim. Sin., 2011,27(12): 2920-2926
52. LIN Xiao, WU Ming-Xing, AN Jiang, MIAO Qing-Qing, QIN Da, MA Ting-Li.Optimization of the Photoelectric Performance of Large-Scale All-Flexible Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2011,27(11): 2577-2582
53. LI Jing, SUN Ming-Xuan, ZHANG Xiao-Yan, CUI Xiao-Li.Counter Electrodes for Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2011,27(10): 2255-2268
54. SHI Ji-Fu, WAN Qing-Cui, XU Gang, XU Xue-Qing, FAN Ye.Influence of Temperature on the Properties of Polysulfide Electrolyte and Quantum Dot Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2011,27(10): 2360-2366
55. LIU Run-Hua, ZHANG Sen, XIA Xin-Yuan, YUN Da-Qin, BIAN Zu-Qiang, ZHAO Yong-Liang.DSSCs Using a Nanoparticle/Nanorod Composite TiO2 Film as a Photoanode[J]. Acta Phys. -Chim. Sin., 2011,27(07): 1701-1706
56. SHI Ji-Fu, XU Gang, MIAO Lei, XU Xue-Qing.p-Type and pn-Type Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2011,27(06): 1287-1299
57. LI Huan-Huan, CHEN Run-Feng, MA Cong, ZHANG Sheng-Lan, AN Zhong-Fu, HUANG Wei.Titanium Oxide Nanotubes Prepared by Anodic Oxidation and Their Application in Solar Cells[J]. Acta Phys. -Chim. Sin., 2011,27(05): 1017-1025
58. ZHUO Zu-Liang, ZHANG Fu-Jun, XU Xiao-Wei, WANG Jian, LU Li-Fang, XU Zheng.Photovoltaic Performance Improvement of P3HT:PCBM Polymer Solar Cells by Annealing Treatment[J]. Acta Phys. -Chim. Sin., 2011,27(04): 875-880
59. LAO Chun-Feng, CHU Zeng-Ze, ZOU De-Chun.Self-Assembly of 3-Aminopropyltrimethoxysilane to Improve the Efficiency of Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2011,27(02): 419-424
60. CHEN Dong-Po, ZHANG Xiao-Dan, WEI Chang-Chun, LIU Cai-Chi, ZHAO Ying.Effect of Blocking Layers Prepared by the Hydrolysis of TiCl4 Solution on the Photovoltaic Performance of a Dye-Sensitized Solar Cell[J]. Acta Phys. -Chim. Sin., 2011,27(02): 425-431
61. GAO Rui, MA Bei-Bei, WANG Li-Duo, SHI Yan-Tao, DONG Hao-Peng, QIU Yong.Photovoltaic Properties and Mechanism Analysis of a Dye/Al2O3 Alternating Assembly Structure by Electrochemical Impedance Spectroscopy[J]. Acta Phys. -Chim. Sin., 2011,27(02): 413-418
62. LIU Jia, YANG Hao-Tian, ZHANG Jing-Bo, ZHOU Xiao-Wen, LIN Yuan.Room Temperature Synthesis of Rutile TiO2 and Its Application in Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2011,27(02): 408-412
63. WANG Yao-Qiong, WEI Zi-Dong, CAI Hong-Ying, ZHANG Qian, ZHAO Qiao-Ling.Pt/FTO Counter Electrode for Dye-Sensitized Solar Cells Prepared by Sputtering-Displacement[J]. Acta Phys. -Chim. Sin., 2010,26(11): 2957-2961
64. QIAN Di-Feng, ZHANG Qing-Hong, WAN Jun, LI Yao-Gang, WANG Hong-Zhi.Enhancing the Photovoltaic Performance of Dye Sensitized Solar Cells with the TiO2 Sol Infiltrated Nanocrystalline Electrode[J]. Acta Phys. -Chim. Sin., 2010,26(10): 2745-2751
65. WANG Wen-Li, LIN Hong, ZHANG Luo-Zheng, LI Xin, CUI Bai, LI Jian-Bao.Electrochemical Impedance Spectroscopy Analysis of an Electrophoretic Titania Nanotube/Nanoparticle Composite Film[J]. Acta Phys. -Chim. Sin., 2010,26(05): 1249-1253
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67. ZHAN Wei-Shen, PAN Shi, LI Yuan-Zuo, CHEN Mao-Du.A Comparison of Indoline Dyes as Photosensitizers in Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin., 2009,25(10): 2087-2092
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69. Li Wei-Hua, Hao Yan-Zhong, Qiao Xue-Bin, Zhang Li, Yang Mai-Zhi, Cai Sheng-Min.Photoelectrochemical Studies on the Nanostructured ZnO/Dye/PPy Electrode[J]. Acta Phys. -Chim. Sin., 1999,15(10): 905-910
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71. ZHOU Shichao, FENG Guitao, XIA Dongdong, LI Cheng, WU Yonggang, LI Weiwei.Star-Shaped Electron Acceptor based on Naphthalenediimide-Porphyrin for Non-Fullerene Organic Solar Cells[J]. Acta Phys. -Chim. Sin., 0,(): 0-0
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