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Acta Phys. -Chim. Sin.
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中文
Current Issue
2010 Vol. 26, No. 11
Published online: 2010-10-29
Current column
Table of Contents
Invited Aticle
Review
THERMODYNAMICS,THERMOCHEMISTRY AND SOLUTION CHEMISTRY
ELECTROCHEMISTRY
COLLOID AND INTERFACE CHEMISTRY
CATALYSIS AND SURFACE STRUCTURE
PHOTOCHEMISTRY AND SPECTROSCOPY
QUANTUM CHEMISTRY AND COMPUTATION CHEMISTRY
PHYSICAL CHEMISTRY OF MATERIALS
Table of Contents
Cover and Table of Contents for Vol.26 No. 11
Acta Phys. -Chim. Sin. 2010, 26 (11), 0.
2222
Abstract/Metrics
2192
PDF(4420KB)
Invited Aticle
Simple Chemical Model for Facilitated Transport with an Application to Wyman-Murray Facilitated Diffusion
COLE Christine Lind, QIAN Hong
A simple chemical kinetic model is developed which describes the behavior of small ligands that can bind reversibly with...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2857-2864.
DOI: 10.3866/PKU.WHXB20101129
5358
Abstract/Metrics
Supporting Info
1940
PDF(795KB)
Review
Solution Synthesis Strategies for Hierarchical Nanostructures
ZHANG Dong-Feng, NIU Li-Ya, GUO Lin
The coupling and synergistic effects of the unique structure of multi-level, multi-dimension, and multi- components allo...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2865-2876.
DOI: 10.3866/PKU.WHXB20101104
8050
Abstract/Metrics
4285
PDF(4476KB)
Progress of Investigations on Structures and Interactions of Ionic Liquids by Infrared Spectroscopy and Raman Spectroscopy
ZHANG Li-Qun, LI Hao-Ran
Experimental methods, theoretical calculations as well as computer simulations are the three most often used approaches ...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2877-2889.
DOI: 10.3866/PKU.WHXB20101123
12767
Abstract/Metrics
4650
PDF(1343KB)
THERMODYNAMICS,THERMOCHEMISTRY AND SOLUTION CHEMISTRY
Thermodynamics and Kinetics of Adsorption of Diclofenac on Magnetic Multiwalled Carbon Nanotubes in an Aqueous Solution
XIONG Zhen-Hu, WANG Lu, ZHOU Jian-Guo, LIU Jian-Ming
We investigated the adsorption of diclofenac (an anti-inflammatory drug) in aqueous solutions by magnetic multiwalled ca...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2890-2898.
DOI: 10.3866/PKU.WHXB20101130
8614
Abstract/Metrics
6266
PDF(1697KB)
Thermodynamic Analysis of Low Temperature Methane Wet-Air Reforming in a Microcombustor
RAN Jing-Yu, ZHAO Liu-Jie
We studied the effects of reaction pressure, molar ratios of air to methane and steam to methane on the reforming proces...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2899-2906.
DOI: 10.3866/PKU.WHXB20101121
5876
Abstract/Metrics
1815
PDF(1021KB)
Molecular Simulation of Dilute Polyacrylamide Solutions
LIU Yan-Yan, CHEN Pan-Ke, LUO Jian-Hui, ZHOU Ge, JIANG Bo
Polyacrylamide (PAM) applied to various fields is an important class of linear water-soluble polymers. Therefore, it is ...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2907-2914.
DOI: 10.3866/PKU.WHXB20101110
7878
Abstract/Metrics
3311
PDF(1281KB)
Thermal Decomposition Kinetics of Poly(propylene carbonate maleate)
WU Wei-Kang, WANG Jia-Li, LIU Su-Qin, HUANG Ke-Long, LIU Yan-Fei
The thermal decomposition kinetics of the novel terpolymer, poly(propylene carbonate maleate) (PPCMA), was investigated ...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2915-2919.
DOI: 10.3866/PKU.WHXB20101028
6958
Abstract/Metrics
2073
PDF(257KB)
ELECTROCHEMISTRY
Mathematical Model and Circuit Realization to Improve Chronoamperometry
CHEN Xu-Hai, CHEN Jing-Hua, PAN Hai-Bo, LI Yu-Rong, DU Min, LIN Xin-Hua
To overcome the disadvantages of chronoamperometry we report a novel electrochemical method where a peak current is quic...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2920-2926.
DOI: 10.3866/PKU.WHXB20101117
5499
Abstract/Metrics
3315
PDF(2237KB)
Preparation and Photoeletrochemical Performance of CdS Quantum Dot Sensitized ZnO Nanorod Array Electrodes
ZHANG Qiao-Bao, FENG Zeng-Fang, HAN Nan-Nan, LIN Ling-Ling, ZHOU Jian-Zhang, LIN Zhong-Hua
We sensitized CdS quantum dots on a ZnO nanorod array electrode by the successive ionic layer adsorption and reaction me...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2927-2934.
DOI: 10.3866/PKU.WHXB20101113
8220
Abstract/Metrics
3195
PDF(2014KB)
Kinetics and Electrochemical Impedance Properties of TiO
2
Nanotube Array Photoelectrode
ZHANG Zhi-Yu, SANG Li-Xia, SUN Biao, ZHANG Xiao-Min, MA Chong-Fang
The 2μm and 650 nm TiO2 nanotube (TNT) arrays were fabricated by sonoelectrochemical anodic oxidation in ethylene gly...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2935-2940.
DOI: 10.3866/PKU.WHXB20101131
5792
Abstract/Metrics
2253
PDF(1346KB)
Evaluation of Metal Corrosion under Defective Coatings by WBE and EIS Technique
ZHANG Wei, WANG Jia, LI Yu-Nan, WANG Wei
We investigated the corrosion of steel under defective coatings in 3.5% (mass fraction) NaCl solution by the wire beamel...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2941-2950.
DOI: 10.3866/PKU.WHXB20101102
5915
Abstract/Metrics
2627
PDF(2976KB)
Improved Capacitive Performance of Polypyrrole Doped with 9,10-Anthraquinone-2-sulfonic Acid Sodium Salt
WAN Qun-Yi, FAN Shuan-Shi, YUE Xian-Jun, LANG Xue-Mei, XU Wen-Dong, LI Jing, FENG Chun-Hua
A polypyrrole(PPy)/9,10-anthraquinone-2-sulfonic acid sodium salt (AQS) composite electrode was prepared by constant-pot...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2951-2956.
DOI: 10.3866/PKU.WHXB20101107
5876
Abstract/Metrics
2372
PDF(2003KB)
Pt/FTO Counter Electrode for Dye-Sensitized Solar Cells Prepared by Sputtering-Displacement
WANG Yao-Qiong, WEI Zi-Dong, CAI Hong-Ying, ZHANG Qian, ZHAO Qiao-Ling
APt/FTOelectrode for dye-sensitized solar cells (DSSC) was prepared by the sputtering (Cu) -displacement (Pt) (SD) metho...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2957-2961.
DOI: 10.3866/PKU.WHXB20101026
6817
Abstract/Metrics
2510
PDF(3362KB)
Preparation and Electrochemical Performance of H
2
Ti
2
O
5
·H
2
O/Cr
2
O
3
Nanotubes as AnodeMaterials for Lithium-Ion Batteries
HE Yong, TANG Zi-Long, ZHANG Zhong-Tai
One problem that limits the rate capabilities of lithium-ion batteries is that despite the small size of the nanocrystal...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2962-2966.
DOI: 10.3866/PKU.WHXB20101101
5339
Abstract/Metrics
2195
PDF(865KB)
Properties of SPES/PWA/SiO
2
Composite Proton Exchange Membranes
GONG Chun-Li, ZHOU Yi, YAN Li-Cheng, WEN Sheng, ZHENG Gen-Wen
Novel sulfonated poly(ether sulfone) (SPES)/phosphotungstic acid (PWA)/silica organic-inorganic composite membranes for ...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2967-2974.
DOI: 10.3866/PKU.WHXB20101124
6055
Abstract/Metrics
2932
PDF(1169KB)
Highly Stable Solid Alkaline ElectrolyteMembranes fromPoly(vinyl alcohol)/Poly(vinyl pyrrolidone) Based on Chemical Cross-Linking
FU Jing, QIAO Jin-Li, MA Jian-Xin
The stability of alkaline electrolyte membranes is recognized as a key factor that affects their electrochemical applica...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2975-2981.
DOI: 10.3866/PKU.WHXB20101014
6706
Abstract/Metrics
2675
PDF(1535KB)
COLLOID AND INTERFACE CHEMISTRY
Effect of Hydrophobically Modified Polyacrylamide on Interfacial Dilational Rheological Properties of Crude Oil Components
ZONG Hua, WANG Lei, FANG Hong-Bo, MAO Lei-Ting, WANG Yu-Hui, ZHANG Lu, ZHAO Sui, YU Jia-Yong
The effect of hydrophobically modified polyacrylamide (HMPAM) on the dilational rheological properties of interfacial fi...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2982-2988.
DOI: 10.3866/PKU.WHXB20101105
6148
Abstract/Metrics
2279
PDF(312KB)
Effect of Hierarchical Architecture of Super-Hydrophobic Surface on the Condensed Drop's Final State
LIU Tian-Qing, SUN Wei, SUN Xiang-Yu, AI Hong-Ru
The interface free energy of a local condensate from the growth and combination of numerous initial condensation nuclei ...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2989-2996.
DOI: 10.3866/PKU.WHXB20101025
7649
Abstract/Metrics
2165
PDF(3342KB)
Interactions between
N
-Alkyl-
N
,
N
-di(2-hydroxyethyl)-
N
-methylammonium Bromide and Bovine Serum Albumin
SHAO Shuang, HU Xiao-Huan, YOU Jin-Zong, LEI Qun-Fang
Interactions between a series of N-alkyl-N,N-di(2-hydroxyethyl)-N-methylammonium bromides with alkyl chain from dodecyl ...
Acta Phys. -Chim. Sin. 2010, 26 (11), 2997-3001.
DOI: 10.3866/PKU.WHXB20101008
6086
Abstract/Metrics
2202
PDF(743KB)
CATALYSIS AND SURFACE STRUCTURE
Cataluminescence Performance on Catalysts of Graphene Supported Platinum
WU Xiao-Qin, ZONG Rui-Long, MU Hao-Jie, ZHU Yong-Fa
Platinum nanoparticles supported by graphene were prepared by the colloid deposition process. The effects of particle si...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3002-3008.
DOI: 10.3866/PKU.WHXB20101010
6881
Abstract/Metrics
3624
PDF(1991KB)
Deactivation of MnO
x
-CeO
x
/ACF Catalysts for Low-Temperature NH
3
-SCR in the Presence of SO
2
SHEN Bo-Xiong, LIU Ting
The low-temperature selective catalytic reduction of NO with NH3 (NH3-SCR) over MnOx-CeOx/ACF (activated carbon fiber) m...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3009-3016.
DOI: 10.3866/PKU.WHXB20101120
5162
Abstract/Metrics
2455
PDF(1038KB)
Carbon Deposition on a Toluene Disproportionation and Transalkylation Catalyst
MENG Gen, KONG De-Jin, QI Xiao-Lan, XU Zhong-Qiang
The nature of carbon deposition on a toluene disproportionation and transalkylation catalyst was characterized using the...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3017-3022.
DOI: 10.3866/PKU.WHXB20101118
6981
Abstract/Metrics
2352
PDF(1056KB)
Dynamic Performance of CO
2
Adsorption with Amine-Modified SBA-16
SHI Jing-Jin, LIU Ya-Min, CHEN Jie, ZHANG Yu, SHI Yao
Novel CO2 adsorbents for CO2 removal were prepared by introducing tetraethylenepentamine (TEPA) into SBA-16 type mesopor...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3023-3029.
DOI: 10.3866/PKU.WHXB20101109
6202
Abstract/Metrics
2200
PDF(1349KB)
PHOTOCHEMISTRY AND SPECTROSCOPY
XPS Study of the Thickness Nanosize Effect for Ultrathin SiO
2
on Si Substrate
ZHAO Zhi-Juan, LIU Fen, ZHAO Liang-Zhong
X-ray photoelectron spectroscopy (XPS) was used to record the Si 2p and valence band spectra for a series of ultrathin S...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3030-3034.
DOI: 10.3866/PKU.WHXB20101111
6652
Abstract/Metrics
2497
PDF(201KB)
Effect ofWater Ligation on the Redox Potential and Infrared Spectra of Chlorophyll-
a
HU Qiong, WANG Guo-Ying, OU Jia-Ming, WANG Rui-Li
In the reaction center of photosystem I the accessory electron transfer cofactors are two monomeric chlorophyll-a molecu...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3035-3040.
DOI: 10.3866/PKU.WHXB20101116
6926
Abstract/Metrics
2127
PDF(704KB)
QUANTUM CHEMISTRY AND COMPUTATION CHEMISTRY
Molecular Dynamics Simulation of Corrosive Medium Diffusion in Corrosion Inhibitor Membrane
QIAO Gui-Min, REN Zhen-Jia, ZHANG Jun, HU Song-Qing, YAN You-Guo, TI Yang
The corrosion inhibition mechanism of four 1-R1-2-undecyl-imidazoline inhibitors (R1: CH2COOH (A), CH2CH2OH (B), CH2CH2N...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3041-3046.
DOI: 10.3866/PKU.WHXB20101020
6357
Abstract/Metrics
2586
PDF(1573KB)
Adsorption Behavior of NO on Cu
3
Pt(111) Surface
XIE Xiu-Juan, CHEN Wen-Kai, SUN Bao-Zhen, GUO Xin, ZHANG Yong-Fan
The adsorption behavior of NOonto a Cu3Pt (111) surface was studied using a periodic slab model and the PW91 generalized...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3047-3051.
DOI: 10.3866/PKU.WHXB20101122
7205
Abstract/Metrics
2443
PDF(1308KB)
Electronic Structure and Optical Properties of the Novel Nonlinear LiAsSe
2
Crystal
NI Bi-Lian, ZHOU He-Gen, JIANG Jun-Quan, LI Yi, ZHANG Yong-Fan
We used density functional theory based on the pseudo-potential plane wave basis set to investigate the electronic struc...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3052-3060.
DOI: 10.3866/PKU.WHXB20101115
6192
Abstract/Metrics
2464
PDF(2296KB)
Geometric and Electronic Structures of Hexanuclear Binary Ta/Rh Mixed Clusters
CAO Fei, TAN Kai, LIN Meng-Hai
Density functional theory (DFT) was employed to investigate the geometric and electronic properties of a series of hexan...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3061-3066.
DOI: 10.3866/PKU.WHXB20101112
5749
Abstract/Metrics
2119
PDF(3987KB)
Effects of CH
3
OH and NH
3
on the Hydrolytic Deamination Mechanismof Adenine
LIU Hai-Ying, MENG Fan-Cui, LI Ping, DING Shi-Liang
The effects of CH3OH and NH3 on the hydrolytic deamination mechanism of adenine were studied by density functional theor...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3067-3072.
DOI: 10.3866/PKU.WHXB20101106
5436
Abstract/Metrics
1712
PDF(1146KB)
PHYSICAL CHEMISTRY OF MATERIALS
Synthesis and Nonlinear Optical Properties of Fluorinated Polyimides Containing Benzothiazole
HE Man, ZHOU Yu-Ming, MIAO Jun-Liang, LIU Cheng, FANG Cheng, CUI Yi-Ping, ZHANG Tong
Hetarylazo chromophores were incorporated into fluorinated polyimide matrices to prepare novel nonlinear optical (NLO) s...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3073-3079.
DOI: 10.3866/PKU.WHXB20101127
5160
Abstract/Metrics
1890
PDF(1024KB)
Purification of Multiwalled Carbon Nanotubes and Characterization of Their Oxygen-Containing Surface Groups
ZHOU Jin-Mei, LI Hai-Yan, LIN Guo-Dong, ZHANG Hong-Bin
We conveniently removed the Ni-MgO catalyst components from an as-grown multiwalled carbon nanotube (CNT) using an aqueo...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3080-3086.
DOI: 10.3866/PKU.WHXB20101108
6743
Abstract/Metrics
3115
PDF(961KB)
Preparation and Characterization of One-Dimensional TiO
2
Nanowire Films on a Flexible Stainless Steel Substrate
WU Tao, TAO Jie, DENG Jie, TANG Yu-Xin, ZHU Hong, GAO Peng
We synthesized a one dimensional (1D) TiO2 nanowire with a large aspect ratio on non-Ti substrate in NaOH aqueous soluti...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3087-3094.
DOI: 10.3866/PKU.WHXB20101103
6007
Abstract/Metrics
2875
PDF(5380KB)
Synthesis, Formation Mechanism and Surface-Enhanced Raman Scattering Properties of Silver Tangled Nanowires and Dendritic Structures
WU Xin-Zhou, PEI Mei-Shan, WANG Lu-Yan, LI Xiao-Nan, TAO Xu-Tang
Silver tangled nanowires and dendritic structures were readily synthesized in high yield by reducing silver nitrate with...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3095-3100.
DOI: 10.3866/PKU.WHXB20101132
6505
Abstract/Metrics
2735
PDF(5769KB)
Preparation and Triethylamine Sensing Properties of Ce-Doped In
2
O
3
Nanofibers
WANG Jin-Xing, YU Lian-Xiang, WANG Hao-Ming, RUAN Sheng-Ping, LI Jia-Jing, WU Feng-Qing
Ce-doped In2O3 nanofibers were synthesized by a simple and effective electrospinning method. The morphology and crystal ...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3101-3105.
DOI: 10.3866/PKU.WHXB20101126
6022
Abstract/Metrics
2312
PDF(1230KB)
Fabrication of Al
2
O
3
Nanoparticles by Cathodic Plasma Electrolysis
LI Zhao-Hu, ZHANG Zhi-Kun, GUO Deng-Zhu
We used aluminum as the cathodic material and an aqueous solution of 3 mol·L-1 NH4NO3 as the electrolyte in our w...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3106-3112.
DOI: 10.3866/PKU.WHXB20101114
5267
Abstract/Metrics
2462
PDF(1133KB)
Synthesis, Characterization and Surface Functionalization of Novel Spindle-Like α-Fe
2
O
3
Nanocrystals
ZHAN Yong-Gong, CHEN Qi-Yuan, YIN Zhou-Lan, LI Li-Li, CAI Bing-Xin
We synthesized novel α-Fe2O3 nanocrystals (NFO-1) with single crystalline structure. In our synthetic strategy, th...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3113-3119.
DOI: 10.3866/PKU.WHXB20101119
5516
Abstract/Metrics
Supporting Info
2052
PDF(1756KB)
Magnetite Sub-Microspheres with Controlled Diameter and Magnetic Properties Synthesized by the Citrate-Assisted Polyol Process
YAN Gong-Qin, WANG Wei, SUN Zhi-Gang, GUAN Jian-Guo
Monodispersed superparamagnetic magnetite (Fe3O4) sub-microspheres with controlled grain sizes and diameters were obtain...
Acta Phys. -Chim. Sin. 2010, 26 (11), 3120-3126.
DOI: 10.3866/PKU.WHXB20101027
5151
Abstract/Metrics
2644
PDF(2661KB)