Acta Phys. -Chim. Sin. ›› 2026, Vol. 42 ›› Issue (8): 100308.doi: 10.1016/j.actphy.2026.100308

• ARTICLE • Previous Articles     Next Articles

La2O3 decorated Ti3C2Tx MXene: temperature regulation and frequency selective surface synergy for enhanced X-Band microwave absorption

Qiang Wang1, Jifan Yang2, Xiaolei Su2,*(), Yi Liu2,*()   

  1. 1 School of Textile Science and Engineering, Xi'an Polytechnic University, Xi'an 710048, Shaanxi Province, China
    2 School of Materials Science & Engineering, Xi'an Polytechnic University, Xi'an 710048, Shaanxi Province, China
  • Received:2026-02-22 Revised:2026-04-20 Accepted:2026-04-21 Published:2026-06-11
  • Contact: Email: suxiaolei@xpu.edu.cn (Xiaolei Su)yiliu1021@xpu.edu.cn (Yi Liu)

Abstract:

MXene possesses high dielectric loss and a distinctive layered structure, yet its single-component characteristic gives rise to intense electromagnetic wave reflection, which severely restricts its microwave absorption efficiency. In this study, La2O3@Ti3C2Tx nanocomposites were fabricated by immobilizing La2O3 nanoparticles onto exfoliated Ti3C2Tx nanosheets via amino-bond linkage, with temperature adopted as a pivotal parameter to modulate the absorption performance. Ti3C2Tx was derived from the Ti3AlC2 precursor through LiF-assisted wet etching, ultrasonication and centrifugation. The phase composition and microstructure of the composites were characterized by XRD, SEM and TEM, while their electromagnetic parameters in the X-band were measured using a vector network analyzer. The optimal absorption performance was attained at a temperature of 60 ℃. At a thickness of 3.8 mm, the minimum reflection loss reaches −50.5 dB at 9.2 GHz, and the effective absorption bandwidth fully covers the X-band (8.2–12.4 GHz). Furthermore, the microwave absorption performance is further optimized by simulating the loaded frequency selective surface, with the reflection loss in the X-band all below −10 dB at a thickness of 3.2 mm. Mechanistic analysis based on electromagnetic field simulation confirms that the exceptional absorption behavior originates from LC resonance. This work provides a novel and feasible strategy for designing and fabricating high-performance Ti3C2Tx-based microwave absorbing materials, which shows promising application prospects in the field of electromagnetic protection.

Key words: La2O3@Ti3C2Tx, Reflection loss, Frequency selective surface, Polarization loss