铋基光催化剂在太阳能转换中的合理设计

doi:10.3866/PKU.WHXB202405016

物理化学学报 >> 2024, Vol. 40 >> Issue (12): 2405016.doi: 10.3866/PKU.WHXB202405016

所属专题：太阳燃料制备

铋基光催化剂在太阳能转换中的合理设计

崔元映¹^,²^,†, 张金锋²^,†, 褚海亮¹^,*(), 孙立贤¹^,*(), 代凯²^,*()

¹ 桂林电子科技大学材料科学与工程学院, 广西电子信息材料构效关系重点实验室, 广西新能源材料结构与性能协同创新中心, 广西桂林 541004
² 淮北师范大学物理与电子信息学院, 安徽省污染物敏感材料与环境修复重点实验室, 安徽淮北 235000

收稿日期:2024-05-20 修回日期:2024-07-07 录用日期:2024-07-08 发布日期:2024-11-09
通讯作者: Email: daikai940@chnu.edu.cn (代凯)sunlx@guet.edu.cn (孙立贤)chuhailiang@guet.edu.cn (褚海亮)
作者简介:
^† These authors contributed equally to this work.
基金资助:
国家自然科学基金(22278169, 51973078), 安徽省高校优秀科研创新团队(2022AH010028), 安徽省教育厅重大项目(2022AH040068)和安徽省质量工程项目(2022sx134), 桂林市创新平台与人才项目(20210102-4), 桂林漓江学者和广西八桂学者

Rational Design of Bismuth Based Photocatalysts for Solar Energy Conversion

Yuanyin Cui¹^,², Jinfeng Zhang², Hailiang Chu¹^,*(), Lixian Sun¹^,*(), Kai Dai²^,*()

¹ Guangxi Key Laboratory of Information Materials, Guangxi Collaborative Innovation Centre of Structure and Property for New Energy Materials, School of Materials Science and Engineering, Guilin University of Electronic Technology, Guilin 541004, Guangxi Zhuang Autonomous Region, China
² Laboratory of Green and Precise Synthetic Chemistry and Applications, Ministry of Education, College of Physics and Electronic Information, Huaibei Normal University, Huaibei 235000, Anhui Province, China

Received:2024-05-20 Revised:2024-07-07 Accepted:2024-07-08 Published:2024-11-09
Contact: Email: daikai940@chnu.edu.cn (Kai Dai)sunlx@guet.edu.cn (Lixian Sun)chuhailiang@guet.edu.cn (Hailiang Chu)
Supported by:
This work was supported by the National Natural Science Foundation of China (22278169, 51973078, 22179026), the Excellent Scientific Research and Innovation Team of Education Department of Anhui Province (2022AH010028), the Major Projects of Education Department of Anhui Province (2022AH040068), and Anhui Provincial Quality Engineering Project (2022sx134), the Innovation Platform and Talent Program Project of Guilin (20210102-4), the Guilin Lijiang Scholar Foundation and the Guangxi Bagui Scholar Foundation

摘要/Abstract

摘要：

作为一种清洁的太阳能转换技术，半导体光催化为应对世界能源危机和环境污染治理提供了重要技术途径。而在不同类型的光催化剂中，铋基材料凭借其特有的晶体结构、可调的能带宽度、多样的化学组成，以及在光催化领域所具有的广泛前景而备受关注。尽管如此，当前关于铋基光催化剂的开发还不够完善，仍需要大量研究和讨论。为了提高铋基材料的催化性能，并克服目前低光利用效率、选择性差和成本高的挑战，对其结构、合成和结构调控方法的全面理解必不可少。因此本文系统论述了在太阳能应用领域，铋基光催化剂的合理设计与最新进展。这篇文章首先概述了多种铋基光催化剂的近期科研动态，包括层状铋化合物、铋元素、BiVO₄、Bi₂S₂和Bi₂O₃等材料。其次，归纳了铋基光催化剂的主要合成方案，并介绍了提高催化活性的结构调控方法。接着，强调了铋基材料在CO₂还原、光解水、N₂固定、NO_X去除、H₂O₂生产以及选择性有机反应等多种领域潜力巨大。此外，文章还深入探讨了用于铋基光催化剂的先进原位分析手段。最后，本综述明确了现存的发展障碍，并预测了铋基光催化剂的未来发展前景。本综述有望为深入理解和合理设计高性能铋基材料提供全面指导，推动环境与能源领域的创新应用，助力实现双碳目标和可持续发展。

关键词: 光催化, 铋, 异质结, 电荷分离, 应用

Abstract:

Semiconductor photocatalysis makes full use of solar energy, serving as a potent tactic to solve the worldwide energy deficit and safeguard the environment. Bismuth-based photocatalysts stand out among various photocatalysts as a significant area, due to their unique crystal structure, favorable mixed electron band structure, diverse composition, and huge potential for solar catalytic conversion. This document reviews the rational design of Bi-based photocatalysts for solar energy. Recent advancements in diverse Bi-based photocatalysts such as Layered Bi, Bismuth element, BiVO₄, Bi₂S₂, and Bi₂O₃ are highlighted. Secondly, the synthesis strategies of Bi-based catalysts, including hydrothermal/solvothermal, chemical precipitation, and solid-state reaction, are summarized. Third, various structural regulation methods to improve the photocatalytic performance, including defect regulation, heteroatom doping, morphology, SPR effect utilization, and heterojunction construction, are systematically introduced. Additionally, a focus is given to the exclusive applications of Bi-based photocatalysts, including CO₂ reduction, water decomposition, N₂ fixation, NO_x removal, H₂O₂ production, and selective organic synthesis, followed by an introduction of advanced in situ characterization techniques of the Bi-based photocatalysts. Ultimately, the forthcoming obstacles are underscored, and a future outlook for Bi-based photocatalysts is anticipated. This review aims to offer detailed instructions for comprehensively understanding and logically crafting effective bismuth-based photocatalysts, while also encouraging novel ideas and advances in energy and environmental fields, contributing to the goals of green chemistry and sustainable development.

Key words: Photocatalysis, Bi, Heterojunction, Charge separation, Application

崔元映, 张金锋, 褚海亮, 孙立贤, 代凯. 铋基光催化剂在太阳能转换中的合理设计[J]. 物理化学学报, 2024, 40(12), 2405016. doi: 10.3866/PKU.WHXB202405016

Yuanyin Cui, Jinfeng Zhang, Hailiang Chu, Lixian Sun, Kai Dai. Rational Design of Bismuth Based Photocatalysts for Solar Energy Conversion[J]. Acta Phys. -Chim. Sin. 2024, 40(12), 2405016. doi: 10.3866/PKU.WHXB202405016

链接本文: https://www.whxb.pku.edu.cn/CN/10.3866/PKU.WHXB202405016

https://www.whxb.pku.edu.cn/CN/Y2024/V40/I12/2405016

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铋基光催化剂在太阳能转换中的合理设计

Rational Design of Bismuth Based Photocatalysts for Solar Energy Conversion

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