非水溶剂Li-O2电池锂负极研究进展

doi:10.3866/PKU.WHXB201611181

Abstract

Abstract:

The aprotic Li-O₂ battery has attracted considerable interest in recent years because of its high theoretical specific energy that is far greater than that achievable with state-of-the-art Li-ion technologies. To date, most Li-O₂ studies, based on a cell configuration with a Li metal anode, aprotic Li⁺ electrolyte and porous O₂ cathode, have focused on O₂ reactions at the cathode. However, these reactions might be complicated by the use of Li metal anode. This is because both the electrolyte and O₂ (from cathode) can react with the Li metal and some parasitic products could cross over to the cathode and interfere with the O₂ reactions occurring therein. In addition, the possibility of dendrite formation on the Li anode, during its multiple plating/stripping cycles, raises serious safety concerns that impede the realization of practical Li-O₂ cells. Therefore, solutions to these issues are urgently needed to achieve a reversible and safety Li anode. This review summarizes recent advances in this field and strategies for achieving high performance Li anode for use in aprotic Li-O₂ batteries. Topics include alternative counter/reference electrodes, electrolytes and additives, composite protection layers and separators, and advanced experimental techniques for studying the Li anode|electrolyte interface. Future developments in relation to Li anode for aprotic Li-O₂ batteries are also discussed.

Key words: Lithium-oxygen battery, Lithium metal anode, Li anode stability, Solid electrolyte interphase layer

Yan-Tao ZHANG,Zhen-Jie LIU,Jia-Wei WANG,Liang WANG,Zhang-Quan PENG. Recent Advances in Li Anode for Aprotic Li-O₂ Batteries[J]. Acta Phys. -Chim. Sin. 2017, 33(3), 486-499. doi: 10.3866/PKU.WHXB201611181

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Recent Advances in Li Anode for Aprotic Li-O₂ Batteries

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