层状MoS2/Ti3C2Tx异质结光热转换材料用于太阳能驱动水蒸发

doi:10.1016/j.actphy.2025.100053

Abstract

Abstract:

Metallic 1T Molybdenum disulfide (1T-MoS₂) exhibits enhanced full spectral light absorption and prominent electrical conductivity, making it ideal for photothermal applications in conjunction with Ti₃C₂T_x MXene. Despite the challenges in increasing the 1T-MoS₂ proportion within MoS₂/Ti₃C₂T_x heterostructures and the incomplete understanding of the mechanisms governing their formation and properties, herein, a combined theoretical and experimental framework has been established, suggesting that the metallic characteristics of Ti₃C₂T_x and 1T-MoS₂ could significantly improve photothermal performance through strong interlayer interactions and efficient electron transport. The hierarchical MoS₂/Ti₃C₂T_x heterostructure has been fabricated through a one-step hydrothermal synthesis method with enhanced 1T-MoS₂ proportion, which achieves multilayered wrinkled architecture resulting from the in-situ growth of MoS₂ on Ti₃C₂T_x nanosheets. Notably, a remarkable peak photoheating temperature of 107 ℃ under an 808 nm laser with an intensity of 0.5 W·cm⁻² is realized, demonstrating its exceptional photothermal conversion capability. By incorporated into a polyvinylidene difluoride membrane, the MoS₂/Ti₃C₂T_x heterostructure functions as an efficient self-floating solar-driven steam generator, reaching an evaporation rate of 1.79 kg·m⁻²·h⁻¹ and an evaporation efficiency of 96.4% under one solar irradiance. This study proposes a versatile strategy for the MoS₂/Ti₃C₂T_x heterostructure, offering the potential for sustainable solar-driven vapor generation technologies.

Key words: MXene, Molybdenum disulfide, Heterostructure, Photothermal conversion, Solar-driven vapor generation

Kun Rong, Cuilian Wen, Jiansen Wen, Xiong Li, Qiugang Liao, Siqing Yan, Chao Xu, Xiaoliang Zhang, Baisheng Sa, Zhimei Sun. Hierarchical MoS₂/Ti₃C₂T_x heterostructure with excellent photothermal conversion performance for solar-driven vapor generation[J]. Acta Phys. -Chim. Sin. 2025, 41(6), 100053. doi: 10.1016/j.actphy.2025.100053

Figures/Tables 6

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Hierarchical MoS2/Ti3C2Tx heterostructure with excellent photothermal conversion performance for solar-driven vapor generation

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Hierarchical MoS₂/Ti₃C₂T_x heterostructure with excellent photothermal conversion performance for solar-driven vapor generation