(Ta2/3Ti1/3)2CTx MXene/硫化物异质结构中的多尺度介电损耗工程及其电磁波衰减性能

doi:10.1016/j.actphy.2026.100374

Abstract

Abstract: The rational regulation of dielectric loss behavior and impedance matching remains a critical challenge for developing high-performance electromagnetic wave absorbers. Herein, a novel solid-solution (Ta_2/3Ti_1/3)₂CT_x MXene/CuInS₂ (TTC/CS) heterostructure was successfully fabricated through a microwaveassisted solvothermal strategy. Benefiting from the intimate coupling nanosheets and semiconductive CuInS₂, a multi-scale dielectric loss engineering platform was established to simultaneously optimize electromagnetic attenuation capability and impedance matching characteristics. Structural analyses demonstrate the successful formation of abundant TTC/CS heterointerfaces accompanied by significant interfacial charge redistribution. The synergistic effects originating from intrinsic vacancies, surface functional groups, multi-cation configurations, and heterojunction interfaces generate abundant polarization centers and multiple dielectric relaxation processes. Meanwhile, the interconnected layered architecture promotes charge transport, conduction loss, and multiple reflections/scattering of incident electromagnetic waves. As a result, the optimized TTC/CS-3 composite exhibits superior electromagnetic wave absorption performance, delivering a broad effective absorption bandwidth (EAB) of 4.56 GHz at a thickness of only 1.9 mm. Electromagnetic parameter analysis reveals that the outstanding performance originates from the cooperative optimization of attenuation capability and impedance matching. Furthermore, radar cross-section simulations demonstrate significantly suppressed electromagnetic scattering behavior for the optimized composite. This work provides an effective strategy for constructing MXene-based heterostructures through multi-scale dielectric configuration and offers new insights into the design of lightweight, broadband, and highly efficient electromagnetic protection materials.

Key words: (Ta_2/3Ti_1/3)₂CT_x, Heterojunctions, Dielectric relaxation, Balanced impedance matching, Electromagnetic protection

Shijie Zhang, Ruiqi Wang, Shun Wang, Li Tian, Panpan Wang, Xiaowei Liang, Airong Wang, Yupeng Shi, Zhiwei Zhao. Multi-scale dielectric loss engineering in (Ta_2/3Ti_1/3)₂CT_x MXene/sulfide heterostructures for electromagnetic wave attenuation[J]. Acta Phys. -Chim. Sin. 2026, (), 100374. doi: 10.1016/j.actphy.2026.100374

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Multi-scale dielectric loss engineering in (Ta_2/3Ti_1/3)₂CT_x MXene/sulfide heterostructures for electromagnetic wave attenuation

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Multi-scale dielectric loss engineering in (Ta2/3Ti1/3)2CTx MXene/sulfide heterostructures for electromagnetic wave attenuation

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Multi-scale dielectric loss engineering in (Ta_2/3Ti_1/3)₂CT_x MXene/sulfide heterostructures for electromagnetic wave attenuation