物理化学学报 >> 2025, Vol. 41 >> Issue (11): 100132.doi: 10.1016/j.actphy.2025.100132
马浩桐1, 衡明宇1, 许杨1, 毕炜1, 缪应纯2,*, 肖舒宁1,*
收稿日期:2025-06-25
修回日期:2025-07-16
录用日期:2025-07-18
发布日期:2025-09-29
通讯作者:
Email: xiaosn@usst.edu.cn (肖舒宁) Email: xiaosn@usst.edu.cn (Shuning Xiao)Miaoyingchun1979@126.com (缪应纯)
基金资助:Haotong Ma1, Mingyu Heng1, Yang Xu1, Wei Bi1, Yingchun Miao2,*, Shuning Xiao1,*
Received:2025-06-25
Revised:2025-07-16
Accepted:2025-07-18
Published:2025-09-29
Contact:
Miaoyingchun1979@126.com (Yingchun Miao)
Supported by:摘要:
在大气浓度下进行光催化CO2还原极具挑战性,但对于实现碳中和技术应用却至关重要。本研究通过微波辅助熔盐法合成了一种负载铜(Cu)的碳(C)掺杂氮化硼(Cu/BCN)光催化剂。该方法能够同时将C引入BN晶格并选择性负载Cu纳米颗粒,形成高效的异质结构。C掺杂与Cu负载之间的协同作用调节了能带结构,增强了可见光吸收,促进了电荷分离,并改善了CO2吸附。优化后的Cu/BCN光催化剂在环境CO2条件下实现了30.62 μmol·g−1·h−1的CO产率,选择性为95.8%。结合实验和DFT分析证实,Cu/BCN界面促进了电荷转移,并降低了*COOH形成的能垒。这项工作展示了直接从空气中高效利用CO2的有前景途径,为大气中的碳转化提供了一种可扩展的策略。
马浩桐, 衡明宇, 许杨, 毕炜, 缪应纯, 肖舒宁. 微波合成铜负载的碳掺杂氮化硼光催化材料及其大气浓度下CO2还原性能研究[J]. 物理化学学报, 2025, 41(11), 100132. doi: 10.1016/j.actphy.2025.100132
Haotong Ma, Mingyu Heng, Yang Xu, Wei Bi, Yingchun Miao, Shuning Xiao. Synergistic carbon doping and Cu loading on boron nitride via microwave synthesis for enhanced atmospheric CO2 photoreduction[J]. Acta Phys. -Chim. Sin. 2025, 41(11), 100132. doi: 10.1016/j.actphy.2025.100132
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