3D-2D-1D混合微结构的ZIF-8@Fe3O4/GNs复合材料电磁波吸收性能优化研究

doi:10.1016/j.actphy.2026.100418

Abstract

Abstract: With the intensification of electromagnetic pollution, high-performance microwave absorbing materials featuring thin thickness, light weight, broad bandwidth and strong absorption are in urgent demand. In this work, a ternary ZIF-8@Fe₃O₄/graphite nanosheet (GNs) composite with a unique 3D-2D-1D hierarchical microstructure was rationally designed and synthesized. Different from most reported ZIF-8-based absorbers with a single polyhedral structure, this work realized controllable modulation of ZIF-8 morphology between two-dimensional (2D) leaf-like nanosheets and three-dimensional (3D) rhombic dodecahedra by tuning the molar ratio of Zn²⁺ to 2-methylimidazole. Furthermore, one-dimensional (1D) short carbon nanotubes were in-situ grown on the composite surface through the catalytic effect of reduced metal particles during high-temperature calcination, constructing a cross-dimensional hierarchical structure. The optimized composite exhibited excellent electromagnetic wave absorption performance: the maximum effective absorption bandwidth (EAB) reached 5.12 GHz at a matching thickness of only 1.6 mm. CST numerical simulations verified that the composite still maintained satisfactory absorption performance when applied as a functional coating. The superior absorption performance originates from good impedance matching, as well as the synergistic effect of multiple polarization mechanisms, conduction loss and magnetic loss enabled by the 3D-2D-1D hierarchical structure. This work provides a new structural design strategy for the development of high-performance ZIF-based microwave absorbing materials.

Key words: ZIF-8, GNs, Hierarchical microstructure, Electromagnetic wave absorption, Impedance matching

Luohan Wang, Hanhong Deng, Liyuan Sun, Haifeng Li, Nan Sun. Electromagnetic wave absorbing properties of ZIF-8@Fe₃O₄/GNs composites optimized by 3D-2D-1D microstructure[J]. Acta Phys. -Chim. Sin. 2026, (), 100418. doi: 10.1016/j.actphy.2026.100418

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Electromagnetic wave absorbing properties of ZIF-8@Fe₃O₄/GNs composites optimized by 3D-2D-1D microstructure

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Electromagnetic wave absorbing properties of ZIF-8@Fe3O4/GNs composites optimized by 3D-2D-1D microstructure

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Electromagnetic wave absorbing properties of ZIF-8@Fe₃O₄/GNs composites optimized by 3D-2D-1D microstructure