一种新型等离子体共振效应调控的Ag/Ag3PO4/C3N5 S型异质结光催化材料高效降解左氧氟沙星抗生素

doi:10.3866/PKU.WHXB202310013

Abstract

Abstract:

The escalating presence of pharmaceutical antibiotics in natural water poses an overwhelming threat to the sustainable development of society. Photocatalysis technology stands out as a promising and cutting-edge environmental purification alternative. C₃N₅, identified as a distinctive nonprecious nonmetal photocatalyst, holds potential for environmental protection. However, challenges persist originating from the sluggish photoreaction kinetics and severe photo-carrier reunion. Currently, the design of a special S-scheme photosystem proves to be a reliable strategy for obtaining outstanding photocatalysts. In this context, a plasmonic S-scheme photosystem involving Ag/Ag₃PO₄/C₃N₅ was developed through a feasible route. The compactly connected 0D/0D/2D Ag/Ag₃PO₄/C₃N₅ heterostructure, benefitting from the synergy between the plasmonic effect and the S-scheme junction, facilitates the efficient utilization of appreciably reinforced sunlight absorption, effective photo-carrier disassociation, and notable photoredox capacity. Consequently, this system generates •OH and •O₂⁻ effectively. Ag/Ag₃PO₄/C₃N₅ demonstrates a superb photocatalytic levofloxacin eradication rate of 0.0362 min⁻¹, marking a substantial advancement of 24.8, 1.1, and 0.7 folds compared to C₃N₅, Ag₃PO₄, and Ag₃PO₄/C₃N₅, respectively. Impressively, Ag/Ag₃PO₄/C₃N₅ delivers remarkable anti-interference performance and reusability. This achievement signifies a significant step toward developing potent C₃N₅-involved photosystems for environmental purification.

Key words: Plasmonic effect, C₃N₅, S-scheme heterojunction, Synergistic effect, Antibiotic removal, Internal electric field

Kexin Dong, Chuqi Shen, Ruyu Yan, Yanping Liu, Chunqiang Zhuang, Shijie Li. Integration of Plasmonic Effect and S-Scheme Heterojunction into Ag/Ag₃PO₄/C₃N₅ Photocatalyst for Boosted Photocatalytic Levofloxacin Degradation[J]. Acta Phys. -Chim. Sin. 2024, 40(10), 2310013. doi: 10.3866/PKU.WHXB202310013

Figures/Tables 6

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Integration of Plasmonic Effect and S-Scheme Heterojunction into Ag/Ag₃PO₄/C₃N₅ Photocatalyst for Boosted Photocatalytic Levofloxacin Degradation

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Integration of Plasmonic Effect and S-Scheme Heterojunction into Ag/Ag3PO4/C3N5 Photocatalyst for Boosted Photocatalytic Levofloxacin Degradation

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Integration of Plasmonic Effect and S-Scheme Heterojunction into Ag/Ag₃PO₄/C₃N₅ Photocatalyst for Boosted Photocatalytic Levofloxacin Degradation