聚多巴胺封装液态金属的Janus液态金属@MXene/Fe3O4纳米纤维膜：用于电磁干扰屏蔽与红外调控

doi:10.1016/j.actphy.2026.100281

物理化学学报 >> 2026, Vol. 42 >> Issue (10): 100281.doi: 10.1016/j.actphy.2026.100281

聚多巴胺封装液态金属的Janus液态金属@MXene/Fe₃O₄纳米纤维膜：用于电磁干扰屏蔽与红外调控

方春月¹^,†, 谭晓璇¹^,†, 王春红¹^,³^,⁸^,*(), 何洋²^,*(), 裴晓园¹, 张钰¹, Sarani binti Zakaria⁶, 伏广伟⁴, 王建刚⁵, 陈利⁸, 刘坤⁷, 徐婷⁷, 司传领⁷^,*()

¹ 天津工业大学纺织科学与工程学院, 天津 300387
² 天津工业大学材料科学与工程学院, 分离膜材料先进技术国家重点实验室, 天津 300387
³ 天津工业大学绍兴柯桥研究院, 浙江绍兴 312030
⁴ 中国纺织工程学会, 北京 100025
⁵ 绍兴市质量技术监督检测院, 浙江绍兴 312366
⁶ UKM-YSD Chair for Sustainability, Faculty of Engineering and Built Environment, Universiti Kebangsaan Malaysia 43600, Selangor, Malaysia
⁷ 天津科技大学生物基纤维材料全国重点实验室, 天津市制浆造纸重点实验室, 中国轻工业造纸与生物质精炼重点实验室, 天津 300457
⁸ 天津工业大学先进纺织复合材料学科交叉中心, 天津 300387

收稿日期:2026-02-02 修回日期:2026-03-05 录用日期:2026-03-05 发布日期:2026-09-03
通讯作者: Email: wangchunhong@tiangong.edu.cn (王春红)heyang@tiangong.edu.cn (何洋)sichli@tust.edu.cn (司传领)
作者简介:
^†这些作者对本工作做出了同等贡献

Janus liquid metal@Mxene/Fe₃O₄ nanofiber membranes with polydopamine-confined liquid metal for electromagnetic interference shielding and infrared control

Chunyue Fang¹, Xiaoxuan Tan¹, Chunhong Wang¹^,³^,⁸^,*(), Yang He²^,*(), Xiaoyuan Pei¹, Yu Zhang¹, Sarani binti Zakaria⁶, Guangwei Fu⁴, Jiangang Wang⁵, Li Chen⁸, Kun Liu⁷, Ting Xu⁷, Chuanling Si⁷^,*()

¹ School of Textile Science and Engineering, Tiangong University, Tianjin 300387, China
² State Key Laboratory of Advanced Separation Membrane Materials, School of Materials Science and Engineering, Tiangong University, Tianjin 300387, China
³ Shaoxing Keqiao Institute of Tiangong University, Shaoxing 312030, Zhejiang Province, China
⁴ China Textile Engineering Society, Beijing 100025, China
⁵ Shaoxing Testing Institute of Quality Technical Supervision, Shaoxing 312366, Zhejiang Province, China
⁶ UKM-YSD Chair for Sustainability, Faculty of Engineering and Built Environment, Universiti Kebangsaan Malaysia 43600, Selangor, Malaysia
⁷ State Key Laboratory of Bio-based Fiber Materials, Tianjin Key Laboratory of Pulp and Paper, China Light Industry Key Laboratory of Papermaking and Biorefinery, Tianjin University of Science and Technology, Tianjin 300457, China
⁸ Interdisciplinary Research Center for Advanced Textile Composites, Tiangong University, Tianjin 300387, China

Received:2026-02-02 Revised:2026-03-05 Accepted:2026-03-05 Published:2026-09-03
Contact: Email: wangchunhong@tiangong.edu.cn (Chunhong Wang)heyang@tiangong.edu.cn (Yang He)sichli@tust.edu.cn (Chunwen Sun)

1. ACTPHY-2026.100281-SI-5p.pdf(483KB)

摘要/Abstract

摘要：

电磁干扰(EMI)日益制约着柔性多功能电子材料的发展，但非对称结构设计与功能集成仍存在局限。本文报道了一种Janus层级膜材料——液态金属@聚多巴胺-MXene/Fe₃O₄@纤维素聚丙烯腈纳米纤维(LM@PDA-MXene/Fe₃O₄@CPNF)，通过静电纺丝制备Fe₃O₄掺杂的纤维素/聚丙烯腈纳米纤维支架，并采用真空辅助组装法构筑插层有核壳结构LM@PDA纳米颗粒的MXene层制得。该多尺度结构耦合了三种损耗机制：MXene渗流网络实现导电损耗，LM@PDA间隔物抑制堆叠并形成微电容器引发界面与偶极极化，多孔磁性入口改善阻抗匹配。在X波段，70 μm单层膜的平均电磁屏蔽效能(SET)达45.1 dB，厚度归一化比屏蔽效能(SSE/t)达8.87 × 10³ dB cm² g⁻¹；四层堆叠后SET提升至70.8 dB。该膜还具有取向依赖性热功能，这种超薄、环保、轻质膜在单一平台集成了吸收主导型EMI屏蔽与双向热管理功能，为下一代可穿戴电子设备的电磁防护与红外调控提供了实用化路径。

关键词: 电磁干扰屏蔽, 磁性纳米纤维, MXene, 结构调控, 多功能性

Abstract:

Electromagnetic interference (EMI) increasingly constrains the development of flexible and multifunctional electronics materials, yet asymmetric structural design and functional integration remain limited. Here we report a Janus hierarchical membrane, liquid metal@polydopamine-MXene/Fe₃O₄@cellulose polyacrylonitrile nanofibers (LM@PDA-MXene/Fe₃O₄@CPNF), fabricated by electrospinning a Fe₃O₄-doped cellulose/Polyacrylonitrile nanofiber scaffold and vacuum-assisted assembly of MXene intercalated with core–shell LM@PDA nanoparticles. The multiscale architecture couples three loss pathways: a percolated MXene network for conductive loss, LM@PDA spacers that suppress restacking and form microcapacitors for interfacial and dipolar polarization, and a porous magnetic entrance that improves impedance matching. In the X-band, a single 70 μm layer achieved an average EMI shielding effectiveness (SET) of 45.1 dB and a thickness-normalised specific shielding effectiveness (SSE/t) = 8.87 × 10³ dB·cm² g⁻¹, stacking four layers raised SET to 70.8 dB. The membrane also provided orientation-dependent thermal functions, this ultrathin, eco-friendly, and lightweight membrane integrates absorption-dominant EMI shielding with bidirectional thermal management in a single platform, offering a practical route toward electromagnetic protection and infrared control in next-generation wearable electronics.

Key words: Electromagnetic interference shielding, Magnetic nanofiber, MXene, Structure regulation, Multifunctional

方春月, 谭晓璇, 王春红, 何洋, 裴晓园, 张钰, Sarani binti Zakaria, 伏广伟, 王建刚, 陈利, 刘坤, 徐婷, 司传领. 聚多巴胺封装液态金属的Janus液态金属@MXene/Fe₃O₄纳米纤维膜：用于电磁干扰屏蔽与红外调控[J]. 物理化学学报, 2026, 42(10), 100281. doi: 10.1016/j.actphy.2026.100281

Chunyue Fang, Xiaoxuan Tan, Chunhong Wang, Yang He, Xiaoyuan Pei, Yu Zhang, Sarani binti Zakaria, Guangwei Fu, Jiangang Wang, Li Chen, Kun Liu, Ting Xu, Chuanling Si. Janus liquid metal@Mxene/Fe₃O₄ nanofiber membranes with polydopamine-confined liquid metal for electromagnetic interference shielding and infrared control[J]. Acta Phys. -Chim. Sin. 2026, 42(10), 100281. doi: 10.1016/j.actphy.2026.100281

链接本文: https://www.whxb.pku.edu.cn/CN/10.1016/j.actphy.2026.100281

https://www.whxb.pku.edu.cn/CN/Y2026/V42/I10/100281

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Janus liquid metal@Mxene/Fe₃O₄ nanofiber membranes with polydopamine-confined liquid metal for electromagnetic interference shielding and infrared control

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