染料敏化太阳电池中TiO2/染料/电解质界面的修饰

doi:10.3866/PKU.WHXB201306172

Abstract

Abstract:

Dye-sensitized solar cell (DSC), a new type of solar cell, have attracted widespread attention since they were first reported. The internal contact interfaces of DSC, especially TiO₂/dye/electrolyte interfaces, have always been a focus of research in this field. The adsorption of photosensitizers, and the injection, transport, and recombination of photoelectrons, which occur at the interface, have a significant effect on the DSC performance. Modification of the TiO₂/dye/electrolyte interface of DSC can effectively reduce dye aggregation, surpress electronic recombination, enhance electronic injection efficiency, and improve the transport rate, so it improves the photovoltaic performance and stability of the DSC. Modification can also affect the position of TiO₂ conduction band, the adsorption behavior of the dye, and other parameters. In this article, researches on the methods and mechanism of TiO₂/dye/electrolyte interface modification are reviewed. These include modification of TiO₂ photoanodes by various methods, the introduction of co-adsorbents into the dye bath, the co-sensitization by different dyes, and the use of electrolyte additives with different functional mechanisms in the electrolyte. Finally, problems existed in application of these modification methods and future development directions are discussed.

Key words: Dye-sensitized solar cell, Interface modification, Electronic recombination, Photoanode, Co-sensitization, Electrolyte additive, Coadsorbent

LI Jing-Zhe, KONG Fan-Tai, WU Guo-Hua, HUANG Yang, CHEN Wang-Chao, DAI Song-Yuan. TiO₂/Dye/Electrolyte Interface Modification for Dye-Sensitized Solar Cells[J]. Acta Phys. -Chim. Sin. 2013, 29(09), 1851-1864. doi: 10.3866/PKU.WHXB201306172

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TiO₂/Dye/Electrolyte Interface Modification for Dye-Sensitized Solar Cells

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TiO₂/Dye/Electrolyte Interface Modification for Dye-Sensitized Solar Cells