Acta Phys. -Chim. Sin. ›› 2022, Vol. 38 ›› Issue (11): 2204049.doi: 10.3866/PKU.WHXB202204049
Special Issue: Special Issue of Emerging Scientists
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Research Progress in Regulation Strategies of High-Performance Antimony-Based Anode Materials for Sodium Ion Batteries
Ying Li1,2, Xueqi Lai1,2, Jinpeng Qu1,2, Qinzhi Lai1,2, Tingfeng Yi1,2,3,*(
)
- 1 School of Materials Science and Engineering, Northeastern University, Shenyang 110819, China
2 School of Resources and Materials, Northeastern University at Qinhuangdao, Qinhuangdao 066004, Hebei Province, China
3 Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province, Qinhuangdao 066004, Hebei Province, China
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Received:2022-04-26Accepted:2022-05-20Published:2022-05-25 -
Contact:Tingfeng Yi E-mail:tfyihit@163.com -
About author:Tingfeng Yi, Email: tfyihit@163.com
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Supported by:the National Natural Science Foundation of China(U1960107);the National Natural Science Foundation of China(22179019);the "333" Talent Project of Hebei Province(A202005018);the Natural Science Foundation of Hebei Province, China(B2020501003);the Fundamental Research Funds for the Central Universities, China(N2123001)
Cite this article
Ying Li, Xueqi Lai, Jinpeng Qu, Qinzhi Lai, Tingfeng Yi. Research Progress in Regulation Strategies of High-Performance Antimony-Based Anode Materials for Sodium Ion Batteries[J]. Acta Phys. -Chim. Sin. 2022, 38(11), 2204049. doi: 10.3866/PKU.WHXB202204049
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Fig 1
Sodium storage mechanisms and efficient strategies to enhance the electrochemical performance of Sb-based anode materials. All insets come from the literature."
Fig 2
(a) Crystal structures of Sb; (b) schematic diagram of electrochemical reaction mechanism of Sb materials 53. (c) ex-situ 23Na-NMR and PDF spectra of the cycled antimony electrodes and (d) electrochemical reaction mechanism of Sb obtained from PDF and NMR 54. (b) Adapted with permission from Ref. 53. Copyright 2016, American Chemical Society; (c, d) adapted with permission from Ref. 54. Copyright 2016, American Chemical Society."
Fig 3
(a) Rate capability tests and (b) cycling performance of Sb NCs 59. (c) Schematic diagram of synthesis process for Sb HNS 60. (d) Schematic diagram of the volume change during the Na+/Li+ insertion of Sb HNSs and NSs 60. (e) Schematic illustration of the synthesis, (f) SEM image and (g) rate capability of Sb NTs 63. (a, b) Adapted with permission from Ref. 59. Copyright 2014, American Chemical Society; (c) adapted with permission from Ref. 60. Copyright 2014, American Chemical Society; (d) adapted with permission from Ref. 60. Copyright 2014, American Chemical Society; (e–g) adapted with permission from Ref. 63. Copyright 2019, American Chemical Society."
Fig 4
Schematic diagram of (a) the crystalline phase evolution, (b) ex-situ SAED patterns and (c) electrochemical reaction mechanism for antimonene during the sodiation/desodiation 70. (d) Schematic diagram of synthesis mechanism for porous antimonene 71. (a–c) Adapted with permission from Ref. 70. Copyright 2018, American Chemical Society; (d) adapted with permission from Ref. 71. Copyright 2021, Elsevier."
Fig 5
(a) Schematic illustration of the preparation process and (b) cycling performance of the Sb/MLG hybrid 77. (c) Schematic illustration of synthesis process for Sb/graphene composites by using strong alkali electrolysis process, (d) cyclic voltammograms, and (e) cycling performance for the Sb/graphene composites 80. (a, b) Adapted with permission from Ref. 77. Copyright 2015, American Chemical Society; (c–e) adapted with permission from Ref. 80. Copyright 2019, Elsevier."
Fig 6
(a) Schematic illustration of the synthesis procedure for the Sb/N-C + CNT composite 85. (b) Charge-discharge profiles and (c) cycling performance of Sb/CNT 86. (d) Schematic illustration of the synthesis procedure of Sb NP-MWCNT composite 87. (e) Schematic illustration of the synthesis procedure for the Sb/CNTs composites 88. (a) Adapted with permission from Ref. 85. Copyright 2016, American Chemical Society; (b, c) adapted with permission from Ref. 86. Copyright 2020, Elsevier; (d) adapted with permission from Ref. 87. Copyright 2020, Elsevier; (e) adapted with permission from Ref. 88. Copyright 2021, Elsevier."
Fig 7
(a) Schematic illustration of the synthesis process for the SbNP@C electrode 93. (b) Schematic illustration of the synthesis process for the SbNPs@3D-C 98. (c) Schematic illustration of the synthesis process, (d) cycling performance, and (e) rate capability of Sb|P-S@C foam 99. (a) Adapted with permission from Ref. 93. Copyright 2013, American Chemical Society; (b) adapted with permission from Ref. 98. Copyright 2016, Elsevier; (c–e) adapted with permission from Ref. 99. Copyright 2019, Elsevier."
Fig 8
Schematic illustration for the fabrication of (a) Sb⊂3DPC anode 100, (b) Sb@C yolk-shell structure 102, (c) Sb⊂CTHNs 109 and (d) Sb@PC 110. (a) Adapted with permission from Ref. 100. Copyright 2019, Elsevier; (b) adapted with permission from Ref. 102. Copyright 2017, Elsevier; (c) adapted with permission from Ref. 109. Copyright 2021, Elsevier; (d) adapted with permission from Ref. 110. Copyright 2021, American Chemical Society."
Fig 9
Schematic illustration of the fabrication for (a) Sb@S, N-3DPC 111 and (b) hollow Sb@C yolk-shell spheres 112. (c, d) TEM and SEM images of Sb@S, N-3DPC 111. (e) TEM image of Sb@C yolk-shell spheres 67. (f) Combination styles of 0D active nanoparticles and 2D current-collectors and (g) SEM image of Sb-NDs⊂CNs113. (h) Schematic illustration of sodium storage mechanism for Sb@(N, S?C) 114. (i) Schematic illustration of the fabrication of Sb@NS-3DPCMSs116 and (j) the preparation process of the a-Sb/NC 115. (a) Adapted with permission from Ref. 111. Copyright 2015, Elsevier; (b) adapted with permission from Ref. 112. Copyright 2017, American Chemical Society; (c, d) adapted with permission from Ref. 111. Copyright 2015, Elsevier; (e) adapted with permission from Ref. 112. Copyright 2017, American Chemical Society; (f, g) adapted with permission from Ref. 113. Copyright 2018, Elsevier; (h) adapted with permission from Ref. 114. Copyright 2019, American Chemical Society; (i) adapted with permission from Ref. 116. Copyright 2021, Elsevier; (j) adapted with permission from Ref. 115. Copyright 2019, Elsevier."
Table 1
Effect of carbon coating with different carbon sources on the electrochemical performance of Sb (n: the nth cycle)"
| Anode | Carbon source | Rate capability Capacity [mAh?g?1] (current density) | Cycling stability Capacity [mAh?g?1] (n, current density) | Ref. |
| Sb-N/C | Urea and citric acid | 142 (10 A?g?1) | 220 (180, 2 A?g?1) | |
| Sb@C microsphere | Furfural | 228 (7C) | 456 (300, 0.3C) | |
| peapod-like Sb@C | Glucose | 206 (10 A?g?1) | 305 (3000, 1 A?g?1) | |
| Sb@C | Bio-oil | 303 (5 A?g?1) | 391 (500, 1 A?g?1) | |
| Sb@NC | 1-Ethyl-3-methylimidazolium dicyanamide | 237 (5 A?g?1) | 395 (100, 0.1 A?g?1) | |
| Sb/NPC | Phenylamine | 357 (1.6 A?g?1) | 530 (100, 0.1 A?g?1) | |
| Sb@NCs | Diethylenetriaminepentaacetic acid | 240 (2 A?g?1) | 360 (250, 0.1 A?g?1) | |
| Sb/NPC | Nitrilotriacetic acid | 114 (2 A?g?1) | 401 (100, 0.1 A?g?1) | |
| Sb-CNC | 1-methylimidazole and ClCH2CN | 203 (5 A?g?1) | 475 (150, 0.1 A?g?1) | |
| a-Sb/C | CaC2 | 164 (10 A?g?1) | 283 (3000, 5 A?g?1) |
Fig 10
(a) SEM image of Sb/Cu2Sb 123. (b) Schematic diagram of fabrication process of Cu2Sb/Cu 124. (c) NiSb hollow nanospheres 121. (d) 3-D Sb/NiSb/Ni composite 125. (e) rGO@Sb-Ni composite 126 and (f) FeSb@NC composite 127. (a) Adapted with permission from Ref. 123. Copyright 2014, Elsevier; (b) adapted with permission from Ref. 124. Copyright 2016, American Chemical Society; (c) adapted with permission from Ref. 121. Copyright 2015, Elsevier; (d) adapted with permission from Ref. 125. Copyright 2015, Elsevier; (e) adapted with permission from Ref. 126. Copyright 2018, American Chemical Society; (f) adapted with permission from Ref. 127. Copyright 2020, Elsevier."
Fig 11
(a) Sodium storage mechanism of Bi2Sb6 133. (b) Sodiation/desodiation processes for the Sb/C and BiSb3/C nanofibers 134. (c, d) SEM images of the ZnSb nanowire 135. (e) Schematic diagram of synthesis process for SnSb@SnOx/SbOx@C 145. (f) Schematic diagram of preparation procedure and (g–i) TEM images and elemental mapping images for SnSb/3D-NPC 146. (a) Adapted with permission from Ref. 133. Copyright 2018, American Chemical Society; (b) adapted with permission from Ref. 134. Copyright 2020, Elsevier; (c, d)adapted with permission from Ref. 135. Copyright 2016, Elsevier; (e) adapted with permission from Ref. 145. Copyright 2019, Elsevier; (f–i) adapted with permission from Ref. 146. Copyright 2021, Elsevier."
Fig 12
Schematic diagram of synthesis process for (a) PNS@SnSb 147, (b) porous carbon-free SnSb 149 and (c) NP-SnSb alloy 150. (d) Operando XRD patterns of SnSb alloy in the initial charge-discharge processes and (e) change of diffraction peaks at different ranges 150. (a) Adapted with permission from Ref. 147. Copyright 2017, American Chemical Society; (b) adapted with permission from Ref. 149. Copyright 2018, Elsevier; (c–e) adapted with permission from Ref. 150. Copyright 2018, Elsevier."
Table 2
Electrochemical performance and synthesis methods of other Sb-based alloy anodes for SIBs (n: the nth cycle)."
| Anode | Synthesis method | Rate capability [mAh?g?1] (current density) | Cycling stability [mAh?g?1] (n, current density) | Ref. |
| MS_Fe-Sb alloy | Melt-spinning process | 300 (1 A?g?1) | 466 (80, 0.05 A?g?1) | |
| FeSb2 | Ball milling | 490 (0.3 A?g?1) | 440 (150, 0.3 A?g?1) | |
| FeSb-TiC-C | High energy mechanical milling | 155 (10 A?g?1) | 215 (100, 0.1 A?g?1) | |
| Cu2Sb-Al2O3-C | Mechanochemical reaction | 160 (10 A?g?1) | 198 (70, 0.1 A?g?1) | |
| NiSb⊂3DCM | Cross-linking and galvanic replacement reaction | 248 (5 A?g?1) | 345 (400, 1 A?g?1) | |
| Bi0.2Sb0.8 | Mechanical alloying method | 270 (1.5 A?g?1) | 520 (200, 0.05 A?g?1) | |
| Bi0.25Sb1.75Te3/C | Ball milling | 331 (2 A?g?1) | 406 (100, 2 A?g?1) | |
| SnSb/NC | One-pot process | 85 (2 A?g?1) | 244 (200, 0.1 A?g?1) | |
| SnSb-TiC-C | High energy mechanical milling | 200 (3 A?g?1) | 210 (30, 0.1 A?g?1) | |
| CNF-SnSb | Electrospun | 110 (20C) | 345 (200, 0.2C) | |
| SnSb@rGO@CMFs | Centrifugally-spun | 190 (0.8 A?g?1) | 325 (200, 0.05 A?g?1) | |
| SnSb/CNT@graphene | Hydrothermal method | 268 (1 A?g?1) | 360 (100, 0.1 A?g?1) | |
| SnSb NCs | Colloidal synthesis | 230 (20C) | 345 (100, 0.5C) | |
| Sn-Sb | Replacement reaction route | 367 (2 A?g?1) | 451 (150, 0.5 A?g?1) | |
| SnSb | Ball milling | 400 (4C) | 525 (125, 0.5C) | |
| SnS/SnSb@C | Electrospinning | 159 (2 A?g?1) | 495 (100, 0.05 A?g?1) | |
| SnSb | Electrodeposited | 440 (4C) | 300 (100, 0.5C) |
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