二维光催化材料电子结构和性能调控策略研究进展

doi:10.3866/PKU.WHXB202010010

物理化学学报 >> 2021, Vol. 37 >> Issue (8): 2010010.doi: 10.3866/PKU.WHXB202010010

所属专题：二维光催化材料

二维光催化材料电子结构和性能调控策略研究进展

陈鹏¹^,², 周莹¹, 董帆¹^,²^,*()

¹ 西南石油大学新能源与材料学院，成都 610500
² 电子科技大学基础与前沿研究院环境与能源催化研究中心，成都 611731

收稿日期:2020-10-08 录用日期:2020-11-10 发布日期:2020-11-17
通讯作者: 董帆 E-mail:dfctbu@126.com; dongfan@uestc.edu.cn
作者简介:董帆，电子科技大学基础与前沿研究院教授、博士生导师。于2010年在浙江大学获得博士学位。现为国家青年拔尖人才，国家优秀青年科学基金获得者，国务院特殊津贴专家。主要研究方向包括环境与能源催化材料、空气污染控制技术和催化材料模拟计算等
基金资助:
国家自然科学基金(21822601);国家自然科学基金(21777011)

Advances in Regulation Strategies for Electronic Structure and Performance of Two-Dimensional Photocatalytic Materials

Peng Chen¹^,², Ying Zhou¹, Fan Dong¹^,²^,*()

¹ School of New Energy and Materials, Southwest Petroleum University, Chengdu 610500, China
² Research Center for Environmental and Energy Catalysis, Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 611731, China

Received:2020-10-08 Accepted:2020-11-10 Published:2020-11-17
Contact: Fan Dong E-mail:dfctbu@126.com; dongfan@uestc.edu.cn
About author:Fan Dong, Email: dfctbu@126.com; dongfan@uestc.edu.cn
Supported by:
the National Natural Science Foundation of China(21822601);the National Natural Science Foundation of China(21777011)

摘要/Abstract

摘要：

二维光催化材料具有丰富的表面活性位点、独特的几何结构、可调的电子结构和良好的光催化活性，在环境净化和能源转化等领域具有潜在的应用价值。鉴于此，二维光催化材料的合成方法和性能调控策略得到了快速发展。以往的策略主要集中在形貌和几何结构特征的调节上，实际上并不能完全满足高效稳定的光催化剂的设计需求。通过表面设计构建丰富的活性位点和调整电子结构，可以提高光催化性能及其稳定性。本文从光吸收、电荷分离和活性位点三个方面综述了二维光催化材料的表面设计和电子结构调控策略的研究进展，包括元素掺杂、异质结设计、缺陷构造、单原子修饰、等离子体金属负载等方法，总结了电子结构调控对二维光催化材料净化典型空气污染物反应机理的影响机制。最后，对二维光催化材料研究中存在的问题和挑战进行了分析和展望。

关键词: 二维光催化材料, 表面设计, 电子结构, 反应机理, 活性位点

Abstract:

Two-dimensional photocatalytic materials have potential applications in the fields of environmental purification and energy conversion owing to their rich surface active sites, unique geometric structures, adjustable electronic structures, and good photocatalytic activities. At present, the main two-dimensional photocatalytic materials include metal oxides, metal composite oxides, metal hydroxides, metal sulfides, bismuth-based materials, and non-metallic photocatalytic materials. The absorption of photons in bulk materials or nanoparticles is often limited by the transmittance and reflection at the grain boundary, while the two-dimensional structure can provide a large specific surface area and abundant surface low-coordination atoms to obtain more UV visible light. In addition, the smaller atomic thickness of two-dimensional photocatalytic materials can shorten the carrier migration distance. Thus, in two-dimensional photocatalytic materials, the carriers generated in the interior migrate to the surface faster than that in the bulk materials, which can reduce the recombination of photogenerated carriers and facilitate the photocatalytic reaction. For the surface redox reaction, the two-dimensional structure can provide more abundant surface-active sites to accelerate the reaction process. Additionally, when the thickness is reduced to the atomic scale, the escape energy of atoms is relatively small, thereby increasing the surface defects, which is helpful for the adsorption and activation of target molecules. Thus, the synthesis methods and performance enhancement strategies of two-dimensional photocatalytic materials have been developed rapidly. The former strategies mainly focus on the adjustment of morphology and geometric structure characteristics, which cannot fully meet the design requirements of efficient and stable photocatalysts. The photocatalytic performance and stability can be improved by surface design to construct abundant active sites and adjust the electronic structure. Research on the reaction mechanism of photocatalysis can help us understand the demand for photocatalytic structure characteristics in different reactions, thereby guiding the design of photocatalysts. In this paper, the advances in surface design and electronic structure regulation strategies of two-dimensional photocatalytic materials are reviewed from three aspects: light absorption; charge separation; and active sites, including element doping, heterojunction design, defect construction, single atom modification, and plasmonic metal loading. The effects on the reaction mechanism for typical air pollutant purification by regulating the electronic structure of two-dimensional photocatalytic materials are summarized. Finally, the problems and challenges associated with the development of two-dimensional photocatalytic materials are analyzed and discussed.

Key words: Two dimensional photocatalytic materials, Surface design, Electronic structure, Reaction mechanism, Active sites

陈鹏, 周莹, 董帆. 二维光催化材料电子结构和性能调控策略研究进展[J]. 物理化学学报, 2021, 37(8), 2010010. doi: 10.3866/PKU.WHXB202010010

Peng Chen, Ying Zhou, Fan Dong. Advances in Regulation Strategies for Electronic Structure and Performance of Two-Dimensional Photocatalytic Materials[J]. Acta Phys. -Chim. Sin. 2021, 37(8), 2010010. doi: 10.3866/PKU.WHXB202010010

链接本文: https://www.whxb.pku.edu.cn/CN/10.3866/PKU.WHXB202010010

https://www.whxb.pku.edu.cn/CN/Y2021/V37/I8/2010010

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参考文献 124

1	Feng J. ; Zhang Y. ; Song W. ; Deng W. ; Zhu M. ; Fang Z. ; Ye Y. ; Fang H. ; Wu Z. ; Lowther S. ; et al Environ. Pollut. 2020, 267, 115623. doi: 10.1016/j.envpol.2020.115623
2	An J. ; Zou J. ; Wang J. ; Lin X. ; Zhu B. Environ. Sci. Pollut. Res. 2015, 22, 19607. doi: 10.1007/s11356-015-5177-0
3	Glasius M. ; Goldstein A. H. Environ. Sci. Technol. 2016, 50, 2754. doi: 10.1021/acs.est.5b05105
4	Li J. ; Dong X. A. ; Sun Y. ; Jiang G. ; Chu Y. ; Lee S. C. ; Dong F. Appl. Catal. B-Environ. 2018, 239, 187. doi: 10.1016/j.apcatb.2018.08.019
5	Deng Y. ; Li J. ; Li Y. ; Wu R. ; Xie S. J. Environ. Sci. 2019, 75, 334. doi: 10.1016/j.jes.2018.05.004
6	Muñoz V. ; Casado C. ; Suárez S. ; Sánchez B. ; Marugán J. Catal. Today 2019, 326, 82. doi: 10.1016/j.cattod.2018.09.001
7	Mo J. ; Zhang Y. ; Xu Q. ; Lamson J. J. ; Zhao R. Atmos. Environ. 2009, 43, 2229. doi: 10.1016/j.atmosenv.2009.01.034
8	Wang S. ; Ang H. M. ; Tade M. O. Environ. Int. 2007, 33, 694. doi: 10.1016/j.envint.2007.02.011
9	Gao X. ; An L. ; Qu D. ; Jiang W. ; Chai Y. ; Sun S. ; Liu X. ; Sun Z. Sci. Bull. 2019, 64, 918. doi: 10.1016/j.scib.2019.05.009
10	Li S. ; Wang D. ; Wu X. ; Chen Y. Chin. J. Catal. 2020, 41, 550. doi: 10.1016/S1872-2067(19)63446-7
11	Luo J. ; Zhang S. ; Sun M. ; Yang L. ; Luo S. ; Crittenden J. C. ACS Nano 2019, 13, 9811. doi: 10.1021/acsnano.9b03649
12	Wang Q. ; Hisatomi T. ; Jia Q. ; Tokudome H. ; Zhong M. ; Wang C. ; Pan Z. ; Takata T. ; Nakabayashi M. ; Shibata N. ; et al Nat. Mater. 2016, 15, 611. doi: 10.1038/nmat4589
13	Ong W. J. ; Tan L. L. ; Ng Y. H. ; Yong S. T. ; Chai S. P. Chem. Rev. 2016, 116, 7159. doi: 10.1021/acs.chemrev.6b00075
14	Li Y. ; Zhang D. ; Fan J. ; Xiang Q. Chin. J. Catal. 2021, 42, 627. doi: 10.1016/S1872-2067(20)63684-1
15	Cui W. ; Li J. ; Chen L. ; Dong X. A. ; Wang H. ; Sheng J. ; Sun Y. ; Zhou Y. ; Dong F. Sci. Bull. 2020, 65, 1626. doi: 10.1016/j.scib.2020.05.024
16	Wang H. ; Zhang L. ; Chen Z. ; Hu J. ; Li S. ; Wang Z. ; Liu J. ; Wang X. Chem. Soc. Rev. 2014, 43, 5234. doi: 10.1039/C4CS00126E
17	Wu W. Q. ; Feng H. L. ; Rao H. S. ; Xu Y. F. ; Kuang D. B. ; Su C. Y. Nat. Commun. 2014, 5, 3968. doi: 10.1038/ncomms4968
18	Luo B. ; Liu G. ; Wang L. Nanoscale 2016, 8, 6904. doi: 10.1039/C6NR00546B
19	Xiong J. ; Di J. ; Xia J. ; Zhu W. ; Li H. Adv. Funct. Mater. 2018, 28, 1801983. doi: 10.1002/adfm.201801983
20	Wang L. ; Zhang Y. ; Chen L. ; Xu H. ; Xiong Y. Adv. Mater. 2018, 30, 1801955. doi: 10.1002/adma.201801955
21	Liu G. ; Zhen C. ; Kang Y. ; Wang L. ; Cheng H.-M. Chem. Soc. Rev. 2018, 47, 6410. doi: 10.1039/C8CS00396C
22	Xiang Q. ; Yu J. ; Jaroniec M. Chem. Soc. Rev. 2012, 41, 782. doi: 10.1039/C1CS15172J
23	Gogotsi Y. J. Phys. Chem. Lett. 2011, 2, 2509. doi: 10.1021/jz201145a
24	Meng N. ; Ren J. ; Liu Y. ; Huang Y. ; Petit T. ; Zhang B. Energy Environ. Sci. 2018, 11, 566. doi: 10.1039/C7EE03592F
25	Safaei J. ; Mohamed N. A. ; Mohamad Noh M. F. ; Soh M. F. ; Ludin N. A. ; Ibrahim M. A. ; Roslam Wan Isahak W. N. ; Mat Teridi M. A. J. Mater. Chem. A 2018, 6, 22346. doi: 10.1039/C8TA08001A
26	Ding F. ; Yang D. ; Tong Z. ; Nan Y. ; Wang Y. ; Zou X. ; Jiang Z. Environ. Sci. Nano 2017, 4, 1455. doi: 10.1039/C7EN00255F
27	Low J. ; Cao S. ; Yu J. ; Wageh S. Chem. Commun. 2014, 50, 10768. doi: 10.1039/C4CC02553A
28	Li X. ; Dai Y. ; Ma Y. ; Han S. ; Huang B. Phys. Chem. Chem. Phys. 2014, 16, 4230. doi: 10.1039/C3CP54592J
29	Di J. ; Xiong J. ; Li H. ; Liu Z. Adv. Mater. 2018, 30, 1704548. doi: 10.1002/adma.201704548
30	Sun Y. ; Gao S. ; Lei F. ; Xie Y. Chem. Soc. Rev. 2015, 44, 623. doi: 10.1039/C4CS00236A
31	Zhang J. ; Chen Y. ; Wang X. Energy Environ. Sci. 2015, 8, 3092. doi: 10.1039/C5EE01895A
32	Zhao Z. ; Sun Y. ; Dong F. Nanoscale 2015, 7, 15. doi: 10.1039/C4NR03008G
33	Chen P. ; Liu H. ; Cui W. ; Lee S. C. ; Wang L. A. ; Dong F. EcoMat 2020, 2, e12047. doi: 10.1002/eom2.12047
34	Di J. ; Xiong J. ; Li H. ; Liu Z. Adv. Mater. 2018, 30, 1704548. doi: 10.1002/adma.201704548
35	Ong W. J. ; Tan L. L. ; Ng Y. H. ; Yong S. T. ; Chai S. P. Chem. Rev. 2016, 116, 7159. doi: 10.1021/acs.chemrev.6b00075
36	Xu M. ; Yang J. ; Sun C. ; Liu L. ; Cui Y. ; Liang B. Chem. Eng. J. 2020, 389, 124402. doi: 10.1016/j.cej.2020.124402
37	Li S. ; Sun J. ; Guan J. Chin. J. Catal. 2021, 42, 511. doi: 10.1016/S1872-2067(20)63693-2
38	Ran J. ; Zhang J. ; Yu J. ; Jaroniec M. ; Qiao S. Z. Chem. Soc. Rev. 2014, 43, 7787. doi: 10.1039/C3CS60425J
39	Li X. ; Yu J. ; Jaroniec M. Chem. Soc. Rev. 2016, 45, 2603. doi: 10.1039/C5CS00838G
40	Dong X. ; Li J. ; Xing Q. ; Zhou Y. ; Huang H. ; Dong F. Appl. Catal. B-Environ. 2018, 232, 69. doi: 10.1016/j.apcatb.2018.03.054
41	Cui W. ; Li J. ; Cen W. ; Sun Y. ; Lee S. C. ; Dong F. J. Catal. 2017, 352, 351. doi: 10.1016/j.jcat.2017.05.017
42	Chen P. ; Sun Y. ; Liu H. ; Zhou Y. ; Jiang G. ; Lee S. C. ; Zhang Y. ; Dong F. Nanoscale 2019, 11, 2366. doi: 10.1039/c8nr09147a
43	Li J. ; Dong X. ; Zhang G. ; Cui W. ; Cen W. ; Wu Z. ; Lee S. C. ; Dong F. J. Mater. Chem. 2019, 7, 3366. doi: 10.1039/C8TA11627J
44	Kabir E. ; Kumar P. ; Kumar S. ; Adelodun A. A. ; Kim K. -H. Renew. Sust. Energ. Rev. 2018, 82, 894. doi: 10.1016/j.rser.2017.09.094
45	Xu Z. ; Quintanilla M. ; Vetrone F. ; Govorov A. O. ; Chaker M. ; Ma D. Adv. Funct. Mater. 2015, 25, 2950. doi: 10.1002/adfm.201500810
46	Meng X. ; Liu L. ; Ouyang S. ; Xu H. ; Wang D. ; Zhao N. ; Ye J. Adv. Mater. 2016, 28, 6781. doi: 10.1002/adma.201600305
47	Wang X. ; Wang F. ; Sang Y. ; Liu H. Adv. Energy Mater. 2017, 7, 1700473. doi: 10.1002/aenm.201700473
48	Osterloh F. E. Chem. Soc. Rev. 2013, 42, 2294. doi: 10.1039/C2CS35266D
49	Dong F. ; Ho W.-K. ; Lee S. C. ; Wu Z. ; Fu M. ; Zou S. ; Huang Y. J. Mater. Chem. 2011, 21, 12428. doi: 10.1039/C1JM11840D
50	Liu Y. ; Wang Z. ; Huang B. ; Yang K. ; Zhang X. ; Qin X. ; Dai Y. Appl. Surf. Sci. 2010, 257, 172. doi: 10.1016/j.apsusc.2010.06.058
51	Yu L. ; Zhang X. ; Li G. ; Cao Y. ; Shao Y. ; Li D. Appl. Catal. B: Environ. 2016, 187, 301. doi: 10.1016/j.apcatb.2016.01.045
52	Chen L. ; Yin S. -F. ; Luo S. -L. ; Huang R. ; Zhang Q. ; Hong T. ; Au P. C. T. Ind. Eng. Chem. Res. 2012, 51, 6760. doi: 10.1021/ie300567y
53	Wang J. -J. ; Zhai X. -Y. ; Zhang G. -Y. ; Zhang J. -B. ; Zhao Y.-F. Solid State Sci. 2020, 105, 106288. doi: 10.1016/j.solidstatesciences.2020.106288
54	Tian N. ; Huang H. ; Guo Y. ; He Y. ; Zhang Y. Appl. Surf. Sci. 2014, 322, 249.
55	Hu J. ; Chen D. ; Li N. ; Xu Q. ; Li H. ; He J. ; Lu J. Appl. Catal. B: Environ. 2017, 217, 224. doi: 10.1016/j.apcatb.2017.05.088
56	Dong F. ; Xiong T. ; Wang R. ; Sun Y. ; Jiang Y. Dalton Trans. 2014, 43, 6631. doi: 10.1039/C3DT53383B
57	Hou W. ; Cronin S. B. Adv. Funct. Mater. 2013, 23, 1612. doi: 10.1002/adfm.201202148
58	Atay T. ; Song J.-H. ; Nurmikko A. V. Nano Letters 2004, 4, 1627. doi: 10.1021/nl049215n
59	Kolwas K. ; Derkachova A. ; Shopa M. J. Quant. Spectrosc. Radiat. Trans. 2009, 110, 1490. doi: 10.1016/j.jqsrt.2009.03.020
60	Mock J. J. ; Barbic M. ; Smith D. R. ; Schultz D. A. ; Schultz S. J. Chem. Phys. 2002, 116, 6755. doi: 10.1063/1.1462610
61	Kelly K. L. ; Coronado E. ; Zhao L. L. ; Schatz G. C. J. Phys. Chem. B 2003, 107, 668. doi: 10.1021/jp026731y
62	Li Q. ; Hao X. ; Guo X. ; Dong F. ; Zhang Y. Dalton Trans. 2015, 44, 8805. doi: 10.1039/c5dt00844a
63	Dong F. ; Li Q. ; Zhou Y. ; Sun Y. ; Zhang H. ; Wu Z. Dalton Trans. 2014, 43, 9468. doi: 10.1039/c4dt00427b
64	Dong F. ; Li P. ; Zhong J. ; Liu X. ; Zhang Y. ; Cen W. ; Huang H. Appl. Catal. A-Gen. 2016, 510, 161. doi: 10.1016/j.apcata.2015.11.022
65	Dong F. ; Li Q. ; Sun Y. ; Ho W. ACS Catal. 2014, 4, 4341. doi: 10.1021/cs501038q
66	Dong X. ; Zhang W. ; Cui W. ; Sun Y. ; Huang H. ; Wu Z. ; Dong F. Catal. Sci. Technol. 2017, 7, 1324. doi: 10.1039/C6CY02444K
67	Guo L. ; Yang Z. ; Marcus K. ; Li Z. ; Luo B. ; Zhou L. ; Wang X. ; Du Y. ; Yang Y. Energy Environ. Sci. 2018, 11, 106. doi: 10.1039/C7EE02464A
68	Chen Y. ; Ji S. ; Chen C. ; Peng Q. ; Wang D. ; Li Y. Joule 2018, 2, 1242. doi: 10.1016/j.joule.2018.06.019
69	Zhang J. Z. J. Phys. Chem. B 2000, 104, 7239. doi: 10.1021/jp000594s
70	Kubacka A. ; Fernández-García M. ; Colón G. Chem. Rev. 2012, 112, 1555. doi: 10.1021/cr100454n
71	Shao W. ; Wang H. ; Zhang X. Dalton Trans. 2018, 47, 12642. doi: 10.1039/C8DT02613K
72	Wang Y. Q. ; Shen S. H. Acta Phys. -Chim. Sin. 2020, 36, 1905080.
	王亦清; 沈少华. 物理化学学报, 2020, 36, 1905080. doi: 10.3866/pku.whxb201905080
73	Park H. S. ; Kweon K. E. ; Ye H. ; Paek E. ; Hwang G. S. ; Bard A. J. J. Phys. Chem. C 2011, 115, 17870. doi: 10.1021/jp204492r
74	Zhao Z. ; Sun Y. ; Dong F. ; Zhang Y. ; Zhao H. Rsc Adv. 2015, 5, 39549. doi: 10.1039/C5RA03433G
75	Chen P. ; Wang H. ; Liu H. ; Ni Z. ; Li J. ; Zhou Y. ; Dong F. Appl. Catal. B-Environ. 2019, 242, 19. doi: 10.1016/j.apcatb.2018.09.078
76	Yuan C. ; Cui W. ; Sun Y. ; Wang J. ; Chen R. ; Zhang J. ; Zhang Y. ; Dong F. Chin. Chem. Lett. 2020, 31, 751. doi: 10.1016/j.cclet.2019.09.033
77	Lei F. ; Zhang L. ; Sun Y. ; Liang L. ; Liu K. ; Xu J. ; Zhang Q. ; Pan B. ; Luo Y. ; Xie Y. Angew. Chem. Int. Edit. 2015, 54, 9266. doi: 10.1002/anie.201503410
78	Mi Y. ; Wen L. ; Wang Z. ; Cao D. ; Xu R. ; Fang Y. ; Zhou Y. ; Lei Y. Nano Energy 2016, 30, 109. doi: 10.1016/j.nanoen.2016.10.001
79	Xiong T. ; Cen W. ; Zhang Y. ; Dong F. ACS Catal. 2016, 6, 2462. doi: 10.1021/acscatal.5b02922
80	Li J. ; Cui W. ; Sun Y. ; Chu Y. ; Cen W. ; Dong F. J. Mater. Chem. A 2017, 5, 9358. doi: 10.1039/C7TA02183F
81	Liu G. ; Niu P. ; Sun C. ; Smith S. C. ; Chen Z. ; Lu G. Q. ; Cheng H. -M. J. Am. Chem. Soc. 2010, 132, 11642. doi: 10.1021/ja103798k
82	Zai J. ; Cao F. ; Liang N. ; Yu K. ; Tian Y. ; Sun H. ; Qian X. J. Hazard. Mater. 2017, 321, 464. doi: 10.1016/j.jhazmat.2016.09.034
83	Wu D. ; Yue S. ; Wang W. ; An T. ; Li G. ; Yip H. Y. ; Zhao H. ; Wong P. K. Appl. Catal. B-Environ. 2016, 192, 35. doi: 10.1016/j.apcatb.2016.03.046
84	Yang W. ; Zhang L. ; Xie J. ; Zhang X. ; Liu Q. ; Yao T. ; Wei S. ; Zhang Q. ; Xie Y. Angew. Chem. Int. Edit. 2016, 55, 6716. doi: 10.1002/anie.201602543
85	Huang H. ; Li X. ; Wang J. ; Dong F. ; Chu P. K. ; Zhang T. ; Zhang Y. ACS Catal. 2015, 5, 4094. doi: 10.1021/acscatal.5b00444
86	Cui W. ; Li J. ; Sun Y. ; Wang H. ; Jiang G. ; Lee S. C. ; Dong F. Appl. Catal. B-Environ. 2018, 237, 938. doi: 10.1016/j.apcatb.2018.06.071
87	Li J. ; Zhang Z. ; Cui W. ; Wang H. ; Cen W. ; Johnson G. ; Jiang G. ; Zhang S. ; Dong F. ACS Catal. 2018, 8, 8376. doi: 10.1021/acscatal.8b02459
88	Marschall R. Adv. Funct. Mater. 2014, 24, 2421. doi: 10.1002/adfm.201303214
89	An X. ; Wang Y. ; Lin J. ; Shen J. ; Zhang Z. ; Wang X. Sci. Bull. 2017, 62, 599. doi: 10.1016/j.scib.2017.03.025
90	Zhou H. ; Qu Y. ; Zeid T. ; Duan X. Energy Environ. Sci. 2012, 5, 6732. doi: 10.1039/C2EE03447F
91	Wang Y. ; Wang Q. ; Zhan X. ; Wang F. ; Safdar M. ; He J. Nanoscale 2013, 5, 8326. doi: 10.1039/C3NR01577G
92	He W. ; Wu X. ; Li Y. ; Xiong J. ; Tang Z. ; Wei Y. ; Zhao Z. ; Zhang X. ; Liu J. Chin. Chem. Lett. 2020, 31, 2774. doi: 10.1016/j.cclet.2020.07.019
93	Ao Y. ; Wang K. ; Wang P. ; Wang C. ; Hou J. Appl. Catal. B: Environ. 2016, 194, 157. doi: 10.1016/j.apcatb.2016.04.050
94	Tian N. ; Huang H. ; Liu C. ; Dong F. ; Zhang T. ; Du X. ; Yu S. ; Zhang Y. J. Mater. Chem. A 2015, 3, 17120. doi: 10.1039/C5TA03669K
95	Zhang Y. ; Wang Q. ; Liu D. ; Wang Q. ; Li T. ; Wang Z. Appl. Surf. Sci. 2020, 521, 146434. doi: 10.1016/j.apsusc.2020.146434
96	Yu W. ; Chen J. ; Shang T. ; Chen L. ; Gu L. ; Peng T. Appl. Catal. B: Environ. 2017, 219, 693. doi: 10.1016/j.apcatb.2017.08.018
97	Di J. ; Chen C. ; Yang S. -Z. ; Ji M. ; Yan C. ; Gu K. ; Xia J. ; Li H. ; Li S. ; Liu Z. J. Mater. Chem. A 2017, 5, 14144. doi: 10.1039/C7TA03624H
98	Zhang N. ; Li X. ; Ye H. ; Chen S. ; Ju H. ; Liu D. ; Lin Y. ; Ye W. ; Wang C. ; Xu Q. ; et al J. Am. Chem. Soc. 2016, 138, 8928. doi: 10.1021/jacs.6b04629
99	Liu Y. ; Xiao C. ; Li Z. ; Xie Y. Adv. Energy Mater. 2016, 6, 1600436. doi: 10.1002/aenm.201600436
100	Wang H. ; He W. ; Dong X. a. ; Wang H. ; Dong F. Sci. Bull. 2018, 63, 117. doi: 10.1016/j.scib.2017.12.013
101	Huang J. J. ; D J. M. ; Du H. W. ; Xu G. S. ; Yuan Y. P. Acta Phys. -Chim. Sin. 2020, 36, 1905056.
	黄娟娟; 杜建梅; 杜海威; 徐更生; 袁玉鹏. 物理化学学报, 2020, 36, 1905056. doi: 10.3866/PKU.WHXB201905056
102	Niu P. ; Liu G. ; Cheng H.-M. J. Phys. Chem. C 2012, 116, 11013. doi: 10.1021/jp301026y
103	Yuan J. ; Liu X. ; Tang Y. ; Zeng Y. ; Wang L. ; Zhang S. ; Cai T. ; Liu Y. ; Luo S. ; Pei Y. ; Liu C. Appl. Catal. B-Environ. 2018, 237, 24. doi: 10.1016/j.apcatb.2018.05.064
104	Liao J. ; Cui W. ; Li J. ; Sheng J. ; Wang H. ; Dong X. a. ; Chen P. ; Jiang G. ; Wang Z. ; Dong F. Chem. Eng. J. 2020, 379, 122282. doi: 10.1016/j.cej.2019.122282
105	Liu H. ; Chen P. ; Yuan X. ; Zhang Y. ; Huang H. ; Wang L. A. ; Dong F. Chin. J. Catal. 2019, 40, 620. doi: 10.1016/S1872-2067(19)63279-1
106	Dong X. A. ; Cui W. ; Wang H. ; Li J. ; Sun Y. ; Wang H. ; Zhang Y. ; Huang H. ; Dong F. Sci. Bull. 2019, 64, 669. doi: 10.1016/j.scib.2019.04.020
107	Chen P. ; Liu H. ; Sun Y. ; Li J. ; Cui W. ; Wang L. A. ; Zhang W. ; Yuan X. ; Wang Z. ; Zhang Y. ; Dong F. Appl. Catal. B-Environ. 2020, 264, 118545. doi: 10.1016/j.apcatb.2019.118545
108	Wang H. ; Zhang W. ; Li X. ; Li J. ; Cen W. ; Li Q. ; Dong F. Appl. Catal. B-Environ. 2018, 225, 218. doi: 10.1016/j.apcatb.2017.11.079
109	Dong X. A. ; Zhang W. ; Sun Y. ; Li J. ; Cen W. ; Cui Z. ; Huang H. ; Dong F. J. Catal. 2018, 357, 41. doi: 10.1016/j.jcat.2017.10.004
110	Liao J. ; Li K. ; Ma H. ; Dong F. ; Zeng X. ; Sun Y. Chin. Chem. Lett. 2020, doi: 10.1016/j.cclet.2020.03.081
111	Gao S. ; Gu B. ; Jiao X. ; Sun Y. ; Zu X. ; Yang F. ; Zhu W. ; Wang C. ; Feng Z. ; Ye B. ; Xie Y. J. Am. Chem. Soc. 2017, 139, 3438. doi: 10.1021/jacs.6b11263
112	Zhu C. ; Liu T. ; Qian F. ; Han T. Y. -J. ; Duoss E. B. ; Kuntz J. D. ; Spadaccini C. M. ; Worsley M. A. ; Li Y. Nano Lett. 2016, 16, 3448. doi: 10.1021/acs.nanolett.5b04965
113	Li S. ; Shi M. ; Yu J. ; Li S. ; Lei S. ; Lin L. ; Wang J. Chin. Chem. Lett. 2020, doi: 10.1016/j.cclet.2020.09.056
114	Liu J. ACS Catal. 2017, 7, 34. doi: 10.1021/acscatal.6b01534
115	Yang S. ; Gong Y. ; Zhang J. ; Zhan L. ; Ma L. ; Fang Z. ; Vajtai R. ; Wang X. ; Ajayan P. M. Adv. Mater. 2013, 25, 2452. doi: 10.1002/adma.201204453
116	Niu P. ; Zhang L. ; Liu G. ; Cheng H.-M. Adv. Funct. Mater. 2012, 22, 4763. doi: 10.1002/adfm.201200922
117	Ovchinnikov D. ; Allain A. ; Huang Y. -S. ; Dumcenco D. ; Kis A. ACS Nano 2014, 8, 8174. doi: 10.1021/nn502362b
118	Parzinger E. ; Miller B. ; Blaschke B. ; Garrido J. A. ; Ager J. W. ; Holleitner A. ; Wurstbauer U. ACS Nano 2015, 9, 11302. doi: 10.1021/acsnano.5b04979
119	Lei F. ; Sun Y. ; Liu K. ; Gao S. ; Liang L. ; Pan B. ; Xie Y. J. Am. Chem. Soc. 2014, 136, 6826. doi: 10.1021/ja501866r
120	Liu J. ; Wang D. ; Wang M. ; Kong D. ; Zhang Y. ; Chen J.-F. ; Dai L. Chem. Eng. Technol. 2016, 39, 891. doi: 10.1002/ceat.201500542
121	Xie J. ; Zhang X. ; Zhang H. ; Zhang J. ; Li S. ; Wang R. ; Pan B. ; Xie Y. Adv. Mater. 2017, 29, 1604765. doi: 10.1002/adma.201604765
122	Li X. ; Bi W. ; Zhang L. ; Tao S. ; Chu W. ; Zhang Q. ; Luo Y. ; Wu C. ; Xie Y. Adv. Mater. 2016, 28, 2427. doi: 10.1002/adma.201505281
123	Chen Z. ; Mitchell S. ; Vorobyeva E. ; Leary R. K. ; Hauert R. ; Furnival T. ; Ramasse Q. M. ; Thomas J. M. ; Midgley P.A. ; Dontsova D. ; et al Adv. Funct. Mater. 2017, 27, 1605785. doi: 10.1002/adfm.201605785
124	Liu G. ; Robertson A. W. ; Li M. M.-J. ; Kuo W. C. H. ; Darby M. T. ; Muhieddine M. H. ; Lin Y. -C. ; Suenaga K. ; Stamatakis M. ; Warner J. H. ; Tsang S. C. E. Nat. Chem. 2017, 9, 810. doi: 10.1038/nchem.2740

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二维光催化材料电子结构和性能调控策略研究进展

Advances in Regulation Strategies for Electronic Structure and Performance of Two-Dimensional Photocatalytic Materials

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